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30.06.2020

Assessment of the potential use of zeolites synthesized from power plant fly ash to capture CO₂ under post-combustion scenario

verfasst von: Rafael Morales-Ospino, Yan Goltzman, A. Eurico B. Torres, Enrique Vilarrasa-García, Moises Bastos-Neto, Celio L. Cavalcante Jr, Diana C. S. Azevedo, Carolina Resmini Melo Marques, Thiago Fernandes de Aquino, Vanessa Reich de Oliveira

Erschienen in: Adsorption | Ausgabe 7/2020

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Abstract

Two types of zeolites (type X and type A) were synthesized from fly ash of two Brazilian coal based power plants via hydrothermal treatment after ash fusion with NaOH. The synthesized zeolites were characterized by means of XRF, XRD, SEM and gas adsorption (N₂ and CO₂ adsorption/desorption at − 196 and 0 °C, respectively). Pure CO₂ and N₂ adsorption equilibrium isotherms were performed at 50, 70 and 90 °C to measure the CO₂ adsorption capacity and selectivity of CO₂ over N₂. CO₂/N₂ binary isotherms (15/85% v/v) were also obtained at the same temperatures. Commercial zeolitic materials used for CO₂/N₂ separation such as zeolite 13X and zeolite 4A underwent the same characterization and adsorption measurements as benchmarks to evaluate the performance of the synthesized zeolites. The synthesized materials from fly ash are promising low cost adsorbents for CO₂ separation, reaching ca. 83% of the CO₂ adsorption capacity of their commercial counterparts at 0.15 bar and 50 °C.

Vorheriger Artikel Coupled gravimetric, manometric and calorimetric study of CO2, N2 and CH4 adsorption on zeolites for the assessment of classical equilibrium models

Nächster Artikel Non-thermal plasma-assisted catalytic CO2 conversion over Zn-TCPP 2D catalyst

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Titel: Assessment of the potential use of zeolites synthesized from power plant fly ash to capture CO2 under post-combustion scenario
verfasst von: Rafael Morales-Ospino
Yan Goltzman
A. Eurico B. Torres
Enrique Vilarrasa-García
Moises Bastos-Neto
Celio L. Cavalcante Jr
Diana C. S. Azevedo
Carolina Resmini Melo Marques
Thiago Fernandes de Aquino
Vanessa Reich de Oliveira
Publikationsdatum: 30.06.2020
Verlag: Springer US
Erschienen in: Adsorption / Ausgabe 7/2020
Print ISSN: 0929-5607
Elektronische ISSN: 1572-8757
DOI: https://doi.org/10.1007/s10450-020-00245-0

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