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Journal of Nanoparticle Research
Erschienen in: Journal of Nanoparticle Research 9/2020

01.09.2020 | Research paper

Carbon-coated Co3O4 with porosity derived from zeolite imidazole framework-67 as a bi-functional electrocatalyst for rechargeable zinc air batteries

verfasst von: Qing Zhao, XiaoLong Xu, YuHong Jin, QianQian Zhang, JingBing Liu, Hao Wang

Erschienen in: Journal of Nanoparticle Research | Ausgabe 9/2020

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Abstract

The electro-catalytic performance of the bi-functional catalysts at the air cathode for the oxygen evolution reaction (OER) and oxygen reduction reaction (ORR) plays a significant role for the development of rechargeable zinc air batteries (ZABs). To obtain the high-performance electrocatalysts, a series of porous Co3O4 samples derived from zeolitic imidazolate framework-67 (ZIF-67) are prepared by one-step annealing process at different temperature (350, 450, and 550 °C) under air atmosphere. Compared with the commercial Co3O4, the optimized sample Co3O4 prepared at 450 °C (CO3O4/C-450) exhibits the lowest overpotential of 1.68 V and the highest half-wave potential of − 0.56 V because the porosity of as-prepared Co3O4 provides abundant reactive sites. Moreover, the high discharge potential of 1.33 V and long cycle life of more than 100 h at 20 mA cm−2 are achieved in ZABs with CO3O4/C-450 electrocatalyst, which are attributed to the better stability provided by the carbon coating.
Vorheriger Artikel CVD-diamond nanoparticle synthesis for DLC film application
Nächster Artikel Regulation of the size of metal iron nanoparticles in channels of mesoporous silica matrices (MCM-41, SBA-15) and structure and magnetic properties of the received nanocomposites МСМ-41/Fe0 and SBA-15/Fe0

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Metadaten
Titel
Carbon-coated Co3O4 with porosity derived from zeolite imidazole framework-67 as a bi-functional electrocatalyst for rechargeable zinc air batteries
verfasst von
Qing Zhao
XiaoLong Xu
YuHong Jin
QianQian Zhang
JingBing Liu
Hao Wang
Publikationsdatum
01.09.2020
Verlag
Springer Netherlands
Erschienen in
Journal of Nanoparticle Research / Ausgabe 9/2020
Print ISSN: 1388-0764
Elektronische ISSN: 1572-896X
DOI
https://doi.org/10.1007/s11051-020-05029-9

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