Skip to main content
Top
Published in: Journal of Materials Science 27/2021

21-06-2021 | Metals & corrosion

Corrosion and wear resistance of micro-arc oxidation coating on glass microsphere reinforced Mg alloy composite

Authors: Lin Liu, Sirong Yu, Guang Zhu, Quan Li, Enyang Liu, Wei Xiong, Bingying Wang, Xizhen Yang

Published in: Journal of Materials Science | Issue 27/2021

Log in

Activate our intelligent search to find suitable subject content or patents.

search-config
loading …

Abstract

In this study, micro-arc oxidation (MAO) coatings were prepared on a novel glass microsphere reinforced Mg alloy composite to retard the degradation of the composite in the liquid environment containing Cl for degradable downhole tool applications. The microstructure and chemical composition of the coatings were characterized by SEM, EDS, XPS and XRD. The growth characteristics of the MAO coatings on different matrix regions were analyzed. The corrosion and wear resistance of the coatings were evaluated through the immersion test, electrochemical measurements and friction test. Results showed that the MAO coatings consisted primarily of Mg2SiO4, MgO, little amount of MgAl2O4 and amorphous SiO2. The current density influenced the thickness and structure via affecting the voltage response of the MAO process, afterward influencing the properties of the coatings. The termination voltage of the MAO process and thickness of the coatings increased with the current density. With the current density increased from 8 to 160 mA/cm2, the compactness and microhardness of the coatings were increased, thereby improving the corrosion and wear resistance of the coatings. However, as the current density increased to 200 mA/cm2, the generation of large through-cracks caused the friction coefficient to increase and the corrosion resistance to deteriorate.

Dont have a licence yet? Then find out more about our products and how to get one now:

Springer Professional "Wirtschaft+Technik"

Online-Abonnement

Mit Springer Professional "Wirtschaft+Technik" erhalten Sie Zugriff auf:

  • über 102.000 Bücher
  • über 537 Zeitschriften

aus folgenden Fachgebieten:

  • Automobil + Motoren
  • Bauwesen + Immobilien
  • Business IT + Informatik
  • Elektrotechnik + Elektronik
  • Energie + Nachhaltigkeit
  • Finance + Banking
  • Management + Führung
  • Marketing + Vertrieb
  • Maschinenbau + Werkstoffe
  • Versicherung + Risiko

Jetzt Wissensvorsprung sichern!

Springer Professional "Technik"

Online-Abonnement

Mit Springer Professional "Technik" erhalten Sie Zugriff auf:

  • über 67.000 Bücher
  • über 390 Zeitschriften

aus folgenden Fachgebieten:

  • Automobil + Motoren
  • Bauwesen + Immobilien
  • Business IT + Informatik
  • Elektrotechnik + Elektronik
  • Energie + Nachhaltigkeit
  • Maschinenbau + Werkstoffe




 

Jetzt Wissensvorsprung sichern!

Literature
2.
go back to reference Zhang YZ, Wang XY, Kuang YF, Liu BS, Zhang KW, Fang DQ (2017) Enhanced mechanical properties and degradation rate of Mg-3Zn-1Y based alloy by Cu addition for degradable fracturing ball applications. Mater Lett 195:194–197CrossRef Zhang YZ, Wang XY, Kuang YF, Liu BS, Zhang KW, Fang DQ (2017) Enhanced mechanical properties and degradation rate of Mg-3Zn-1Y based alloy by Cu addition for degradable fracturing ball applications. Mater Lett 195:194–197CrossRef
4.
go back to reference Zheng C, Liu YH, Wang HX, Qin J, Chen C, Zhang SH (2017) Dissolvable fracturing tool based on a controlled electrolytic method. J Petrol Sci Eng 153:81–87CrossRef Zheng C, Liu YH, Wang HX, Qin J, Chen C, Zhang SH (2017) Dissolvable fracturing tool based on a controlled electrolytic method. J Petrol Sci Eng 153:81–87CrossRef
5.
go back to reference Du BD, He TT, Liu GL, Chen W, Wang YM, Wang W, Chen DM (2018) Al-water reactivity of Al-Mg-Ga-In-Sn alloys used for hydraulic fracturing tools. Int J Hydrogen Energ 43:7201–7215CrossRef Du BD, He TT, Liu GL, Chen W, Wang YM, Wang W, Chen DM (2018) Al-water reactivity of Al-Mg-Ga-In-Sn alloys used for hydraulic fracturing tools. Int J Hydrogen Energ 43:7201–7215CrossRef
6.
go back to reference Chen L, Wu Z, Xiao DH, Geng ZW, Zhou PF (2015) Effects of copper on the microstructure and properties of Mg-17Al-3Zn alloys. Mater Corros 66:1159–1168CrossRef Chen L, Wu Z, Xiao DH, Geng ZW, Zhou PF (2015) Effects of copper on the microstructure and properties of Mg-17Al-3Zn alloys. Mater Corros 66:1159–1168CrossRef
7.
go back to reference Xiao DH, Geng ZW, Chen L, Wu Z, Diao HY, Song M, Zhou PF (2015) Effects of alloying elements on microstructure and properties of magnesium alloys for tripling ball. Metall Mater Trans A 46:4793–4803CrossRef Xiao DH, Geng ZW, Chen L, Wu Z, Diao HY, Song M, Zhou PF (2015) Effects of alloying elements on microstructure and properties of magnesium alloys for tripling ball. Metall Mater Trans A 46:4793–4803CrossRef
8.
go back to reference Li XW, Shi T, Li B, Zhou XG, Zhang CW, He ZY, Zhang BB, Zhang QX (2020) Microstructures and electrochemical behaviors of as-cast magnesium alloys with enhanced compressive strengths and corrosion decomposition. Mater Corros 71:1989–1998CrossRef Li XW, Shi T, Li B, Zhou XG, Zhang CW, He ZY, Zhang BB, Zhang QX (2020) Microstructures and electrochemical behaviors of as-cast magnesium alloys with enhanced compressive strengths and corrosion decomposition. Mater Corros 71:1989–1998CrossRef
9.
go back to reference Wang JF, Gao SQ, Liu XY, Peng X, Wang K, Liu SJ, Jiang WY, Guo SF, Pan FS (2020) Enhanced mechanical properties and degradation rate of Mg-Ni-Y alloy by introducing LPSO phase for degradable fracturing ball applications. J Magnes Alloy 8:127–133CrossRef Wang JF, Gao SQ, Liu XY, Peng X, Wang K, Liu SJ, Jiang WY, Guo SF, Pan FS (2020) Enhanced mechanical properties and degradation rate of Mg-Ni-Y alloy by introducing LPSO phase for degradable fracturing ball applications. J Magnes Alloy 8:127–133CrossRef
10.
go back to reference Liu L, Yu SR, Niu YF, Liu EY (2020) Preparation and properties of hollow glass microspheres reinforced Mg alloy degradable composites. J Alloys Compd 835:155198CrossRef Liu L, Yu SR, Niu YF, Liu EY (2020) Preparation and properties of hollow glass microspheres reinforced Mg alloy degradable composites. J Alloys Compd 835:155198CrossRef
11.
go back to reference Liu L, Yu SR, Liu EY, Zhao Y, Wang BY, Niu YF (2021) Effect of Ni addition on the mechanical and degradation properties of hollow glass microsphere/Mg alloy composites. J Alloys Compd 853:157125CrossRef Liu L, Yu SR, Liu EY, Zhao Y, Wang BY, Niu YF (2021) Effect of Ni addition on the mechanical and degradation properties of hollow glass microsphere/Mg alloy composites. J Alloys Compd 853:157125CrossRef
12.
go back to reference Lei T, Ouyang C, Tang W, Li LF, Zhou L (2010) Enhanced corrosion protection of MgO coatings on magnesium alloy deposited by an anodic electrodeposition process. Corros Sci 52:3504–3508CrossRef Lei T, Ouyang C, Tang W, Li LF, Zhou L (2010) Enhanced corrosion protection of MgO coatings on magnesium alloy deposited by an anodic electrodeposition process. Corros Sci 52:3504–3508CrossRef
13.
go back to reference Ishizaki T, Shimada Y, Tsunakawa M, Lee H, Yokomizo T, Hisada S, Nakamura K (2017) Rapid fabrication of a crystalline myristic acid-based superhydrophobic film with corrosion resistance on magnesium alloys by the facile one-step immersion process. ACS Omega 2:7904–7915CrossRef Ishizaki T, Shimada Y, Tsunakawa M, Lee H, Yokomizo T, Hisada S, Nakamura K (2017) Rapid fabrication of a crystalline myristic acid-based superhydrophobic film with corrosion resistance on magnesium alloys by the facile one-step immersion process. ACS Omega 2:7904–7915CrossRef
14.
go back to reference Soliman H, Qian J, Tang S, Xian P, Wan G (2020) Hydroxyquinoline/nano-graphene oxide composite coating of self-healing functionality on treated Mg alloys AZ31. Surf Coat Technol 385:125393CrossRef Soliman H, Qian J, Tang S, Xian P, Wan G (2020) Hydroxyquinoline/nano-graphene oxide composite coating of self-healing functionality on treated Mg alloys AZ31. Surf Coat Technol 385:125393CrossRef
17.
go back to reference Yin ZZ, Qi WC, Zeng RC, Chen XB, Gu CD, Guang SK, Zheng YF (2020) Advances in coatings on biodegradable magnesium alloys. J Magnes Alloy 8:42–65CrossRef Yin ZZ, Qi WC, Zeng RC, Chen XB, Gu CD, Guang SK, Zheng YF (2020) Advances in coatings on biodegradable magnesium alloys. J Magnes Alloy 8:42–65CrossRef
18.
go back to reference Muhaffel F, Cimenoglu H (2019) Development of corrosion and wear resistant micro-arc oxidation coating on a magnesium alloy. Surf Coat Tech 357:822–832CrossRef Muhaffel F, Cimenoglu H (2019) Development of corrosion and wear resistant micro-arc oxidation coating on a magnesium alloy. Surf Coat Tech 357:822–832CrossRef
19.
go back to reference Liu EY, Niu YF, Yu SR, Liu L, Zhang K, Bi XJ, Liang JH (2020) Micro-arc oxidation behavior of fly ash cenospheres/magnesium alloy degradable composite and corrosion resistance of coatings. Surf Coat Tech 391:125693CrossRef Liu EY, Niu YF, Yu SR, Liu L, Zhang K, Bi XJ, Liang JH (2020) Micro-arc oxidation behavior of fly ash cenospheres/magnesium alloy degradable composite and corrosion resistance of coatings. Surf Coat Tech 391:125693CrossRef
20.
go back to reference Jia ZJ, Li M, Liu Q, Xu XC, Cheng Y, Zheng YF, Xi TF, Wei SC (2014) Micro-arc oxidization of a novel Mg-1Ca alloy in three alkaline KF electrolytes: corrosion resistance and cytotoxicity. Appl Surf Sci 292:1030–1039CrossRef Jia ZJ, Li M, Liu Q, Xu XC, Cheng Y, Zheng YF, Xi TF, Wei SC (2014) Micro-arc oxidization of a novel Mg-1Ca alloy in three alkaline KF electrolytes: corrosion resistance and cytotoxicity. Appl Surf Sci 292:1030–1039CrossRef
21.
go back to reference Kaseem M, Hoom J, Gun Ko Y (2017) Corrosion behavior of Al-1wt% Mg-0.85wt%Si alloy coated by microarc-oxidation using TiO2 and Na2MoO4 additives: Role of current density. J Alloys Compd 723:448–455CrossRef Kaseem M, Hoom J, Gun Ko Y (2017) Corrosion behavior of Al-1wt% Mg-0.85wt%Si alloy coated by microarc-oxidation using TiO2 and Na2MoO4 additives: Role of current density. J Alloys Compd 723:448–455CrossRef
22.
go back to reference Ghasemi A, Raja VS, Blawert C, Dietzel W, Kainer KU (2010) The role of anions in the formation and corrosion resistance of the plasma electrolytic oxidation coatings. Surf Coat Technol 204:1469–1478CrossRef Ghasemi A, Raja VS, Blawert C, Dietzel W, Kainer KU (2010) The role of anions in the formation and corrosion resistance of the plasma electrolytic oxidation coatings. Surf Coat Technol 204:1469–1478CrossRef
23.
go back to reference Gao H, Zhang M, Yang X, Huang P, Xu K (2014) Effect of Na2SiO3 solution concentration of micro-arc oxidation process on lap-shear strength of adhesive-bonded magnesium alloys. Appl Surf Sci 314:447–452CrossRef Gao H, Zhang M, Yang X, Huang P, Xu K (2014) Effect of Na2SiO3 solution concentration of micro-arc oxidation process on lap-shear strength of adhesive-bonded magnesium alloys. Appl Surf Sci 314:447–452CrossRef
24.
go back to reference Yue Y, Hua W (2012) Effect of current density on corrosion resistance of micro-arc oxide coatings on magnesium alloy. Trans Nonferrous Met Soc China 20:688–692 Yue Y, Hua W (2012) Effect of current density on corrosion resistance of micro-arc oxide coatings on magnesium alloy. Trans Nonferrous Met Soc China 20:688–692
25.
go back to reference Duan HP, Yan CW, Wang FH (2007) Growth process of plasma electrolytic oxidation films formed on magnesium alloy AZ91D in silicate solution. Electrochim Acta 52:5002–5009CrossRef Duan HP, Yan CW, Wang FH (2007) Growth process of plasma electrolytic oxidation films formed on magnesium alloy AZ91D in silicate solution. Electrochim Acta 52:5002–5009CrossRef
26.
go back to reference Chai L, Xia Y, Yang Z, Wang Y, Okido M (2008) Anodizing of magnesium alloy AZ31 in alkaline solutions with silicate under continuous sparking. Corros Sci 50:3274–3279CrossRef Chai L, Xia Y, Yang Z, Wang Y, Okido M (2008) Anodizing of magnesium alloy AZ31 in alkaline solutions with silicate under continuous sparking. Corros Sci 50:3274–3279CrossRef
27.
go back to reference Li CY, Feng XL, Yu XT, Yin ZZ, Kannan MB, Chen XB, Guan SK, Zhang J, Zeng RC (2019) Corrosion and wear resistance of micro-arc oxidation composite coatings on magnesium alloy AZ31-the influence of inclusions of carbon spheres. Adv Eng Mater 21:1900446CrossRef Li CY, Feng XL, Yu XT, Yin ZZ, Kannan MB, Chen XB, Guan SK, Zhang J, Zeng RC (2019) Corrosion and wear resistance of micro-arc oxidation composite coatings on magnesium alloy AZ31-the influence of inclusions of carbon spheres. Adv Eng Mater 21:1900446CrossRef
28.
go back to reference Hussein RO, Nie X, Northwood DO (2013) An investigation of ceramic coating growth mechanisms in plasma electrolytic oxidation (PEO) processing. Electrochim Acta 112:111–119CrossRef Hussein RO, Nie X, Northwood DO (2013) An investigation of ceramic coating growth mechanisms in plasma electrolytic oxidation (PEO) processing. Electrochim Acta 112:111–119CrossRef
29.
go back to reference Nashrah N, Kamil MP, Yoon DK, Kim YG, Ko YG (2019) Formation mechanism of oxide layer on AZ31 Mg alloy subjected to microarc oxidation considering surface roughness. Appl Surf Sci 497:143772CrossRef Nashrah N, Kamil MP, Yoon DK, Kim YG, Ko YG (2019) Formation mechanism of oxide layer on AZ31 Mg alloy subjected to microarc oxidation considering surface roughness. Appl Surf Sci 497:143772CrossRef
30.
go back to reference Xue WB (2006) Features of film growth during plasma anodizing of Al 2024/SiC metal matrix composite. Appl Surf Sci 252:6195–6200CrossRef Xue WB (2006) Features of film growth during plasma anodizing of Al 2024/SiC metal matrix composite. Appl Surf Sci 252:6195–6200CrossRef
31.
go back to reference Guo HF, An MZ (2005) Growth of ceramic coatings on AZ91D magnesium alloys by microarc oxidation in aluminate-fluoride solutions and evaluation of corrosion resistance. Appl Surf Sci 246:229–238CrossRef Guo HF, An MZ (2005) Growth of ceramic coatings on AZ91D magnesium alloys by microarc oxidation in aluminate-fluoride solutions and evaluation of corrosion resistance. Appl Surf Sci 246:229–238CrossRef
32.
go back to reference Yin D, Niu X, Zhang K, Wang J, Cui D (2018) Preparation of MgO doped colloidal SiO2 abrasive and their chemical mechanical polishing performance on c-, r- and a-plane sapphire substrate. Ceram Int 44:14631–14637CrossRef Yin D, Niu X, Zhang K, Wang J, Cui D (2018) Preparation of MgO doped colloidal SiO2 abrasive and their chemical mechanical polishing performance on c-, r- and a-plane sapphire substrate. Ceram Int 44:14631–14637CrossRef
33.
go back to reference Brambilla E, Radtke C, Dos Santos JHZ, Miranda MSL (2009) An investigation on structure and texture of silica-magnesia xerogels. J Sol-Gel Sci Technol 51:70–77CrossRef Brambilla E, Radtke C, Dos Santos JHZ, Miranda MSL (2009) An investigation on structure and texture of silica-magnesia xerogels. J Sol-Gel Sci Technol 51:70–77CrossRef
34.
go back to reference Tian N, Zhou Z, Tian X, Yang C, Li Y (2017) Superior capability of MgAl2O4 for selenite removal from contaminated groundwater during its reconstruction of layered double hydroxides. Sep Purif Technol 176:66–72CrossRef Tian N, Zhou Z, Tian X, Yang C, Li Y (2017) Superior capability of MgAl2O4 for selenite removal from contaminated groundwater during its reconstruction of layered double hydroxides. Sep Purif Technol 176:66–72CrossRef
35.
go back to reference Brambilla R, Pires GP, Dos Santos JHZ, Miranda MSL, Chornik B (2007) Octadecylsilane-modified silicas prepared by grafting and sol-gel methods. J Electron Spectrosc 156–158:413–420CrossRef Brambilla R, Pires GP, Dos Santos JHZ, Miranda MSL, Chornik B (2007) Octadecylsilane-modified silicas prepared by grafting and sol-gel methods. J Electron Spectrosc 156–158:413–420CrossRef
36.
go back to reference Sun C, Liu X, Zhou C, Wang C, Cao H (2019) Preparation and wear properties of magnetic assisted pulse electrodeposited Ni-SiC nano-coatings. Ceram Int 45:1348–1355CrossRef Sun C, Liu X, Zhou C, Wang C, Cao H (2019) Preparation and wear properties of magnetic assisted pulse electrodeposited Ni-SiC nano-coatings. Ceram Int 45:1348–1355CrossRef
37.
go back to reference Yang W, Xu DP, Wang JL, Yao XF, Chen J (2018) Microstructure and corrosion resistance of micro-arc oxidation plus electrostatic powder spraying composite coating on magnesium alloy. Corros Sci 136:174–179CrossRef Yang W, Xu DP, Wang JL, Yao XF, Chen J (2018) Microstructure and corrosion resistance of micro-arc oxidation plus electrostatic powder spraying composite coating on magnesium alloy. Corros Sci 136:174–179CrossRef
38.
go back to reference Tang H, Gao Y (2016) Preparation and characterization of hydroxyapatite containing coating on AZ31 magnesium alloy by micro-arc oxidation. J Alloys Compd 688:699–708CrossRef Tang H, Gao Y (2016) Preparation and characterization of hydroxyapatite containing coating on AZ31 magnesium alloy by micro-arc oxidation. J Alloys Compd 688:699–708CrossRef
39.
go back to reference Gu YH, Bandopadhyay B, Chen CF, Ning CY, Guo YJ (2013) Long-term corrosion inhibition mechanism of microarc oxidation coated AZ31 Mg alloys for biomedical applications. Mater Design 46:66–75CrossRef Gu YH, Bandopadhyay B, Chen CF, Ning CY, Guo YJ (2013) Long-term corrosion inhibition mechanism of microarc oxidation coated AZ31 Mg alloys for biomedical applications. Mater Design 46:66–75CrossRef
42.
go back to reference Cui LY, Zeng RC, Guan SK, Qi WC, Zhang F, Li SQ, Han EH (2017) Degradation mechanism of micro-arc oxidation coatings on biodegradable Mg-Ca alloys: The influence of porosity. J Alloys Compd 695:2464–2476CrossRef Cui LY, Zeng RC, Guan SK, Qi WC, Zhang F, Li SQ, Han EH (2017) Degradation mechanism of micro-arc oxidation coatings on biodegradable Mg-Ca alloys: The influence of porosity. J Alloys Compd 695:2464–2476CrossRef
Metadata
Title
Corrosion and wear resistance of micro-arc oxidation coating on glass microsphere reinforced Mg alloy composite
Authors
Lin Liu
Sirong Yu
Guang Zhu
Quan Li
Enyang Liu
Wei Xiong
Bingying Wang
Xizhen Yang
Publication date
21-06-2021
Publisher
Springer US
Published in
Journal of Materials Science / Issue 27/2021
Print ISSN: 0022-2461
Electronic ISSN: 1573-4803
DOI
https://doi.org/10.1007/s10853-021-06252-y

Other articles of this Issue 27/2021

Journal of Materials Science 27/2021 Go to the issue

Polymers & biopolymers

Microwave foaming of polymers

Premium Partners