Skip to main content
Disciplines
Automotive Business IT + Informatics Construction + Real Estate Electrical Engineering + Electronics Energy + Sustainability Insurance + Risk Finance + Banking Management + Leadership Marketing + Sales Mechanical Engineering + Materials
Events
DE
EN
Books
Journals
Topic Page
Marketing
Start single access now
Access for companies
EXTENDED SEARCH
Log in
Top
Journal of Materials Science
Published in: Journal of Materials Science 17/2021

10-03-2021 | Chemical routes to materials

Preparation of polyvinylidene fluoride modified membrane by tannin and halloysite nanotubes for dyes and antibiotics removal

Authors: Rui Zhang, Yi Liu, Yu Li, Qiong Han, Tongqing Zhang, Kunlin Zeng, Chen Zhao

Published in: Journal of Materials Science | Issue 17/2021

Log in

Activate our intelligent search to find suitable subject content or patents.

search-config
loading …

Abstract

Separation of dyes and antibiotics is particularly important in wastewater treatment. In this work, the hydrophilic modified polyvinylidene fluoride (PVDF) membranes were prepared by deposition of halloysite nanotubes (HNTs), tannic acid (TA) and ferric chloride (FeCl3). The surface morphology of the modified membranes was studied using scanning electron microscopy (SEM) and atomic force microscopy (AFM). In addition, the Fourier transform infrared (FTIR) and X-ray photoelectron spectroscopy (XPS) were used to evaluate the chemical compositions of the membrane. The measurements of water contact angle (CA) and pure water flux (Jw) show that the PVDF membrane has excellent permeability and hydrophilicity. The PVDF modified membrane has good separation performance for dyes, and the rejection ratios of methyl orange, methylene blue and rhodamine B were 98.2%, 94.6% and 96.9%, respectively. In addition, the rejection ratios of modified membrane for tetracyclines and bisphenol A were significantly improved. Most important of all, the TA-Fe(III)/HNTs/PVDF membrane has excellent antifouling performance after cycles tests. These results indicate that the TA-Fe(III)/HNTs/PVDF modified membranes have a great application prospect in dye and antibiotic wastewater treatment.
previous article Polarization-induced phase structure transition and change of photoluminescence in Er3+-doped (Ba, Ca)(Ti, Sn)O3-based multifunctional ceramics
next article Self-healing polymeric ionic liquid hydrogels with high mechanical strength and ionic conductivity

Dont have a licence yet? Then find out more about our products and how to get one now:

Springer Professional "Wirtschaft+Technik"

Online-Abonnement

Mit Springer Professional "Wirtschaft+Technik" erhalten Sie Zugriff auf:

  • über 102.000 Bücher
  • über 537 Zeitschriften

aus folgenden Fachgebieten:

  • Automobil + Motoren
  • Bauwesen + Immobilien
  • Business IT + Informatik
  • Elektrotechnik + Elektronik
  • Energie + Nachhaltigkeit
  • Finance + Banking
  • Management + Führung
  • Marketing + Vertrieb
  • Maschinenbau + Werkstoffe
  • Versicherung + Risiko

Jetzt Wissensvorsprung sichern!

inform now

Springer Professional "Technik"

Online-Abonnement

Mit Springer Professional "Technik" erhalten Sie Zugriff auf:

  • über 67.000 Bücher
  • über 390 Zeitschriften

aus folgenden Fachgebieten:

  • Automobil + Motoren
  • Bauwesen + Immobilien
  • Business IT + Informatik
  • Elektrotechnik + Elektronik
  • Energie + Nachhaltigkeit
  • Maschinenbau + Werkstoffe




 

Jetzt Wissensvorsprung sichern!

inform now
Literature
1.
Hashino M, Katagiri T, Kubota N, Ohmukai Y, Maruyama T, Matsuyama H (2011) Effect of surface roughness of hollow fiber membranes with gear-shaped structure on membrane fouling by sodium alginate. J Membr Sci 366:389–397
2.
Wang Z, Zhang P, Hu F, Zhao Y, Zhu L (2017) A crosslinked β-cyclodextrin polymer used for rapid removal of a broad-spectrum of organic micropollutants from water. Carbohyd Polym 177:224–231
3.
Oki T, Kanae S (2006) Global hydrological cycles and world water resources. Science 313:1068–1072
4.
Shannon MA, Bohn PW, Elimelech M, Georgiadis JG, Marinas BJ, Mayes AM (2008) Science and technology for water purification in the coming decades. Nature 452:301–310
5.
Zhu Y, Wang D, Jiang L, Jin J (2014) Recent progress in developing advanced membranes for emulsified oil/water separation. Npg Asia Mater 6:101–121
6.
Kangn GD, Cao YM (2014) Application and modification of poly(vinylidene fluoride) (PVDF) membranes-a review. J Membr Sci 63:145–165
7.
Cui Z, Hassankiadeh NT, Zhuang Y, Drioli E, Lee YM (2015) Crystalline polymorphism in poly (vinylidenefluoride) membranes. Prog Polym Sci 51:94–126
8.
Zhang Y, Wang J, Gao F, Chen Y, Zhang H (2016) A comparison study: the different impacts of sodium hypochlorite on PVDF and PSF ultrafiltration (UF) membranes. Water Res 109:227–236
9.
Liu J, Shen X, Zhao Y, Chen L (2013) Acryloylmorpholine-grafted PVDF membrane with improved protein fouling resistance. Ind Eng Chem Res 52:18392–18400
10.
11.
Zhao S, Wang Z (2017) A loose nano-filtration membrane prepared by coating HPAN UF membrane with modified PEI for dye reuse and desalination. J Membr Sci 524:214–224
12.
Ye Q, Zhou F, Liu W (2011) Bioinspired catecholic chemistry for surface modification. Chem Soc Rev 40:4244–4258
13.
Lee H, Dellatore SM, Miller WM, Messersmith PB (2007) Mussel-inspired surface chemistry for multifunctional coatings. Science 318:426–430
14.
Xu YC, Tang YP, Liu LF, Guo ZH, Shao L (2017) Nanocomposite organic solvent nanofiltration membranes by a highly-efficient mussel-inspired co-deposition strategy. J Membr Sci 526:32–42
15.
Gao S, Sun J, Liu P, Zhang F, Zhang W, Yuan S, Li J, Jin J (2016) A robust polyionized hydrogel with an unprecedented underwater anti-crude-oil-adhesion property. Adv Mater 28:5307–5314
16.
Barrett DG, Sileika TS, Messersmith PB (2014) Molecular diversity in phenolic and polyphenolic precursors of tannin-inspired nanocoatings. Chem Commun 50:7265–7268
17.
Ferreira D, Gross GG, Hagerman AE (2008) Tannins and related polyphenols: perspectives on their chemistry, biology, ecological effects, and human health protection. Phytochemistry 69:3006–3008
18.
Gulcin I, Huyut Z, Elmastas M, Aboul-Enein HY (2010) Radical scavenging and antioxidant activity of tannic acid. Arabian J Chem 3:43–53
19.
Annamalai J, Nallamuthu T (2015) Characterization of biosynthesized gold nanoparticles from aqueous extract of chlorella vulgaris and their anti-pathogenic properties. Appl Nanosci 5:603–607
20.
Sileika TS, Barrett DG, Zhang R, Lau HKA, Messersmith PB (2013) Colorless multifunctional coatings inspired by polyphenols found in tea, chocolate, and wine. Angew Chem Int Ed 52:10766–10770
21.
Cui Z, Hassankiadeh NT, Lee SY (2013) Poly(vinylidene fluoride) membrane preparation with an environmental diluent via thermally induced phase separation. J Membr Sci 444:223–236
22.
Chakrabarty T, Pérez-Manríquez L, Neelakanda P, Peinemann KV (2017) Bioinspired tannic acid-copper complexes as selective coating for nanofiltration membranes. Sep Purif Technol 184:188–194
23.
Zhang Y, Yu L, Wang H, Zhang B, Liu J (2016) Recent advances in halloysite nanotube derived composites for water treatment. Environ Sci 3:28–44
24.
He Q, Yang D, Deng X, Wu Q, Li R, Zhai Y, Zhang L (2013) Preparation, characterization and application of N-2-Pyridylsuccinamic acid-functionalized halloysite nanotubes for solid-phase extraction of Pb(II). Water Res 47:3976–3983
25.
Lvov YM, Shchukin DG, Möhwald H, Price RR (2008) Halloysite clay nanotubes for controlled release of protective agents. ACS Nano 2:814–820
26.
Zhang R, Zhu XY, Liu Y, Cai YF, Han Q, Zhang TQ (2019) The application of halloysite nanotubes/Fe3O4 composites nanoparticles in polyvinylidene fluoride membranes for dye solution removal. J Inorg Organomet P 29:1625–1636
27.
Madaeni SS, Zinadini S, Vatanpour V (2013) Preparation of superhydrophobic nanofiltration membrane by embedding multiwalled carbon nanotube and polydimethylsiloxane in pores of microfiltration membrane. Sep Purif Technol 111:98–107
28.
29.
Shi Y, Liu J, Zhuo L, Yan X, Cai F, Luo W (2020) Antibiotics in wastewater from multiple sources and surface water of the Yangtze River in Chongqing in China. Environ Monit Assess 192:1–13
30.
Wang Z, Shao D, Westerhoff P (2017) Wastewater discharge impact on drinking water sources along the Yangtze River (China). Sci Total Environ 599–600:1399–1407
31.
32.
Wang KY, Chung TS, Gryta M (2008) Hydrophobic PVDF hollow fiber membranes with narrow pore size distribution and ultra-thin skin for the fresh water production through membrane distillation. Chem Eng Sci 63:2587–2594
33.
Teyssedre G, Bernes A, Lacabanne C (1993) Influence of the crystalline phase on the molecular mobility of PVDF. J Polym Sci Pol Phys 31:2027–2034
34.
Luo C, Liu Q (2017) Oxidant-induced high-efficient mussel-inspired modification on PVDF membrane with superhydrophilicity and underwater superoleophobicity characteristics for oil/water separation. Acs Appl Mater Inter 9:8297–8307
35.
Luo H, Gu C, Zheng W, Dai F, Wang X, Zheng Z (2015) Facile synthesis of novel size-controlled antibacterial hybrid spheres using silver nanoparticles loaded with poly-dopamine spheres. Rsc Advances 5:13470–13477
36.
Zhang Y, Xie Y, Tang A, Zhou Y, Yang H (2014) Precious-metal nanoparticles anchored onto functionalized halloysite nanotubes. Ind Eng Chem Res 53:5507–5514
37.
Xie Y, Qian D, Wu D, Ma X (2011) Magnetic halloysite nanotubes/iron oxide composites for the adsorption of dyes. Chem Eng J 168:959–963
38.
Kim HJ, Kim DG, Yoon H, Choi YS, Yoon J, Lee JC (2015) Polyphenol/Fe\r, III\r, complex coated membranes having multifunctional properties prepared by a one-step fast assembly. Adv Mater Interfaces 2:1500298–1500306
39.
Dreyer DR, Miller DJ, Freeman BD, Paul DR, Bielawski CW (2013) Perspectives on poly (dopamine). Chem Sci 4:3796–3802
40.
Xuan Y, Jiang G, Li Y, Wang J, Geng H (2013) Inhibiting effect of dopamine adsorption and polymerization on hydrated swelling of montmorillonite. Colloid Surf A 422:50–60
41.
Hegab HM, Elmekawy A, Barclay TG, Michelmore A, Zou L, Saint CP (2016) Single-step assembly of multifunctional poly (tannic acid)-graphene oxide coating to reduce biofouling of forward osmosis membranes. Acs Appl Mater Inter 8:17519–17528
42.
Yu L, Wang HX, Zhang YT, Zhang B, Liu JD (2016) Recent advances in halloysite nanotube derived composites for water treatment. Environ Sci Nano 3:28–44
43.
Liu M, Jia Z, Jia D, Zhou C (2014) Recent advance in research on halloysite nanotubes-polymer nanocomposite. Prog Polym Sci 39:1498–1525
44.
Sun H, Yang X, Zhang Y, Cheng X, Xu Y, Bai Y (2018) Segregation-induced in situ hydrophilic modification of poly (vinylidene fluoride) ultrafiltration membranes via sticky poly (ethylene glycol) blending. J Membr Sci 563:22–30
Metadata
Title
Preparation of polyvinylidene fluoride modified membrane by tannin and halloysite nanotubes for dyes and antibiotics removal
Authors
Rui Zhang
Yi Liu
Yu Li
Qiong Han
Tongqing Zhang
Kunlin Zeng
Chen Zhao
Publication date
10-03-2021
Publisher
Springer US
Published in
Journal of Materials Science / Issue 17/2021
Print ISSN: 0022-2461
Electronic ISSN: 1573-4803
DOI
https://doi.org/10.1007/s10853-021-05911-4

Other articles of this Issue 17/2021

Journal of Materials Science 17/2021 Go to the issue

Chemical routes to materials

Numerical study of thermal effect in silicone rubber filled with carbonyl iron powder under microwave radiation

Energy materials

Palladium phosphide nanoparticles embedded in 3D N, P co-doped carbon film for high-efficiency oxygen reduction

Energy materials

Ultra-high capacity dual-ion batteries realized by few-layered reduced graphene oxide and cathode structure design

Electronic materials

Optical temperature sensing based on upconversion nanoparticles with enhanced sensitivity via dielectric superlensing modulation

Composites & nanocomposites

Adjusting shell composition and content of Co-based bimetal core–shell microspheres toward the broadband microwave absorption

Ceramics

Tailoring the electromagnetic properties of perovskite La0.7Sr0.3MnO3 ceramics by Co doping

Premium Partners

    Image Credits