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19-12-2016 | Original Paper | Issue 7/2017

Journal of Materials Science 7/2017

Thin-film electrode based on zeolitic imidazolate frameworks (ZIF-8 and ZIF-67) with ultra-stable performance as a lithium-ion battery anode

Journal:
Journal of Materials Science > Issue 7/2017
Authors:
Zhen Li, Xiaoxiong Huang, Chuanling Sun, Xiangyu Chen, Jinbo Hu, Andreas Stein, Bohejin Tang

Abstract

Thin-film electrodes were prepared using a one-step drop-casting strategy without polymer binder and carbon black. The electrodes exhibit a thin-layer structure, which is an intriguing architecture for lithium-ion battery applications. A high reversible capacity (335.3 and 311.6 mAh g−1 for ZIF-8 and ZIF-67, respectively), good rate performance, and exceptionally cycling stability (about 95.5% initial capacity was retained after 100 cycles at a high current rate of 5 C) were observed in this study. Such an excellent electrochemical performance of the film electrodes is attributed to the thin-layer architecture, which provides easy access for Li+ ions to permeate the whole electrodes because of the shortened diffusion paths, and also to the unique property of the MOFs without the collapse of its structure.

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