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Journal of Materials Science: Materials in Electronics

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22-07-2019

Three-dimensional self-doped hierarchical porous mussel nacre-derived carbons for high performance supercapacitors

Authors: Song Lv, Liya Ma, Qin Zhou, Xinyu Shen, Hua Tong

Published in: Journal of Materials Science: Materials in Electronics | Issue 15/2019

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Abstract

A facile self-doping and self-templating strategy to prepare three-dimensional nitrogen-doped hierarchical porous carbons via direct carbonization of mussel nacre (MN) is developed. Self-templating can be effective to retain the origin structure and the volatile organic components can serve as carbon precursors for porous carbon. The typical MN-derived carbon (MNC) carbonized at 800 °C is endowed with high surface area of unique hierarchical porosity (consisting of macropores, mesopores and micropores), and high content of heteroatom functionalities (1.30 at.% N). Consequently, the performance in the alkaline KOH electrolyte system was particularly promising with the MNC-6 electrodes showing a high capacitance of 243.7 F g⁻¹ at a current density of 1.0 A g⁻¹ and a promising cycling stability with 85.7% capacitance retention at 1.0 A g⁻¹ after 10,000 cycles. The present work provides a new avenue for facile and high efficient construction of N-doped hierarchical porous carbons for potential supercapacitor.

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Title: Three-dimensional self-doped hierarchical porous mussel nacre-derived carbons for high performance supercapacitors
Authors: Song Lv
Liya Ma
Qin Zhou
Xinyu Shen
Hua Tong
Publication date: 22-07-2019
Publisher: Springer US
Published in: Journal of Materials Science: Materials in Electronics / Issue 15/2019
Print ISSN: 0957-4522
Electronic ISSN: 1573-482X
DOI: https://doi.org/10.1007/s10854-019-01807-x

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