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Adsorption
Erschienen in: Adsorption 2-3/2017

08.10.2016

IAST predictions vs co-adsorption measurements for CO2 capture and separation on MIL-100 (Fe)

verfasst von: Pierre Billemont, Nicolas Heymans, Périne Normand, Guy De Weireld

Erschienen in: Adsorption | Ausgabe 2-3/2017

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Abstract

Metal–organic frameworks (MOFs) are considered since last decade as promising materials notably for the development of gas separation and purification by adsorption processes. Selectivity and working capacity are important parameters for adsorbent selection. Unfortunately, these parameters are mostly estimated from pure component isotherms without comparison with mixture experimental data because these measurements are time consuming and complicated. The aim of this study is to compare IAST mixture simulations from pure component isotherms with co-adsorption measurements considering promising industrial adsorption processes for a mesoporous MOF, MIL-100 (Fe). This adsorbent has a good selectivity for CO2 over permanent gases. Three adsorption processes have been studied (i) CO2 capture: a CO2/N2 separation by PSA or mixed membrane process, (ii) biogas and (iii) natural gas purification: a CO2/CH4 separation by PSA process. Pure component isotherms (CO2, CH4 and N2 at 303.15 K) and binary mixture equilibrium measurements (CO2/N2 at 1 and 4 bar and 303.15 K and CO2/CH4 at 303.15 K and 1 and 4 bar for biogas and 30 bar for natural gas) have been realized. A particular attention has been paid for the pure component representation in order to obtain IAST predictions as accurate as possible. The pressure ranges and the theoretical models are selected to get the best fitted curves of pure component adsorption measurements. In these conditions, the comparison between experimental and simulated values in terms of adsorbed quantities and selectivities allows us to conclude that in the case of mixtures studied in this work on MIL-100 (Fe), IAST is a suitable model for such applications.
Vorheriger Artikel Probing adsorption on a nanoscale: field desorption microspectroscopy
Nächster Artikel Development of carboxyl-layered double hydrotalcites of enhanced CO2 capture capacity by K2CO3 promotion

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Metadaten
Titel
IAST predictions vs co-adsorption measurements for CO2 capture and separation on MIL-100 (Fe)
verfasst von
Pierre Billemont
Nicolas Heymans
Périne Normand
Guy De Weireld
Publikationsdatum
08.10.2016
Verlag
Springer US
Erschienen in
Adsorption / Ausgabe 2-3/2017
Print ISSN: 0929-5607
Elektronische ISSN: 1572-8757
DOI
https://doi.org/10.1007/s10450-016-9825-6

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