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A quantitative approach for sealing capacity evaluation of caprock in candidate of aquifer gas storage

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Abstract

The gas sealing capacity of caprock (SCC) is one of the key factors that determine whether aquifer trap can be constructed into underground gas storage (UGS). However, no standard protocol for evaluating SCC of candidate aquifers has been proposed. Based on the core observation, laboratory experiment, and well logging data, the sealing capacity of the target aquifer caprock of Permian mudstone in D5 block of Litan sag, China, is quantitatively evaluated. The important parameters of mineral brittleness, permeability, breakthrough pressure (BP), mechanical brittleness, thickness, and areal extent that affect the SCC are determined. The results of specific tests and data statistics show that the caprock of D5 block is a low permeability rock with a permeability of 10−4 mD, and the BP of undisturbed rock is greater than 38 MPa. Although the brittle mineral quartz is abundant with an average of 38.38%, the mechanical brittleness is not strong under formation conditions. The direct caprock has a thickness of greater than 50 m, and on the top of it is a high-quality indirect caprock that complements the physical closure. The results of a mathematical evaluation model show that except for the sealing index of sample 2, all the other samples have optimal sealing capacity. The field interference test shows that the optimal sealing capacity of the caprock meets the requirements of the construction of underground gas storage (UGS). The rationality of the comprehensive evaluation model can provide a reference for similar evaluation projects in the future.

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Data availability

The data used to support the findings of this study is included within the article.

Abbreviations

SCC:

Sealing capacity of caprock

UGS:

Underground gas storage

BP:

Breakthrough pressure

AGS:

Aquifer gas storage

AEC:

Areal extent of caprock

AESC:

Areal extent of structural closure

\({BRIT}_{\mathrm{t}}\) :

The mineral brittleness considering quartz, feldspar and carbonate

\({BRIT}_{\mathrm{q}}\) :

The mineral brittleness that only quartz is considered

\({B}_{1}^{^{\prime}}\) :

Relative post-peak stress drop

\({B}_{2}^{^{\prime}}\) :

Absolute rate of post-peak stress drop

\({B}_{3}^{^{\prime}}\) :

Yield influence coefficient

\({B}_{4}^{^{\prime}}\) :

Residual flow coefficient

\({BRIT}_{\mathrm{m}}\) :

Mechanical brittleness index

\({\sigma }_{p}\) :

Peak strength

\({\sigma }_{r}\) :

Residual strength

\({k}_{BC}\) :

Slope of the line connecting the starting points of the yield stage and residual stage

\({\varepsilon }_{p1}\) :

Strain at the starting point of yield stage

\({\varepsilon }_{p2}\) :

Strain at the ending point of yield stage

\({\varepsilon }_{r1}\) :

Strain at the starting point of residual stage

\({\varepsilon }_{r1}\) :

Strain at the ending point of the residual stage

\({I}_{c}\) :

Capillary sealing index

\(BR\) :

The normalized breakthrough pressure

\(PE\) :

The normalized permeability

\({p}_{d}\) :

Breakthrough pressure

\({p}_{d\mathrm{max}}\) :

Maximum breakthrough pressure

\(k\) :

Permeability

\({I}_{SEAL}\) :

Sealing capacity of mudstone

\({A}_{s}\) :

Covering area of caprock that is described by the ratio of AES to AESC

\(h\) :

Caprock thickness

\(TF\) :

Ratio of fault throw offset in the top seal to the caprock thickness

\(BRIT\) :

Brittleness of mudstone

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Funding

The authors gratefully acknowledge the support from the National Natural Science Foundation of China (Grant No. 42072166), the Natural Science Foundation of Heilongjiang Province (Grant No. LH2020D004), and State Key Laboratory for Geomechanics and Deep Underground Engineering (Grant No. SKLGDUEK2001).

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Shanpo Jia and Meng Xu: designed and performed the experiments, analyzed the data, and prepared the paper.

Caoxuan Wen and Zengqiang Xi: designed the experiments and revised the manuscript.

Borui Li, Tuanhui Liu, and Lin Han: participated to collect the materials related to the experiment. Designed the experiments and revised the manuscript.

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Correspondence to Caoxuan Wen.

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Jia, S., Xu, M., Wen, C. et al. A quantitative approach for sealing capacity evaluation of caprock in candidate of aquifer gas storage. Environ Sci Pollut Res 30, 63678–63690 (2023). https://doi.org/10.1007/s11356-023-26873-x

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