Abstract
The world will need greatly increased energy supply in the future for sustained economic growth, but the related CO2 emissions and the resulting climate changes are becoming major concerns. CO2 is one of the most important greenhouse gases that is said to be responsible for approximately 60% of the global warming. Along with improvement of energy efficiency and increased use of renewable energy sources, carbon capture and sequestration (CCS) is expected to play a major role in curbing the greenhouse gas emissions on a global scale. This article reviews the various options and technologies for CO2 capture, specifically for stationary power generation sources. Many options exist for carbon dioxide capture from such sources, which vary with power plant types, and include post-combustion capture, pre-combustion capture, oxy fuel combustion capture, and chemical looping combustion capture. Various carbon dioxide separation technologies can be utilized with these options, such as chemical absorption, physical absorption, adsorption, and membrane separation. Most of these capture technologies are still at early stages of development. Recent progress and remaining challenges for the various CO2 capture options and technologies are reviewed in terms of capacity, selectivity, stability, energy requirements, etc. Hybrid and modified systems hold huge future potentials, but significant progress is required in materials synthesis and stability, and implementations of these systems on demonstration plants are needed. Improvements and progress made through applications of process systems engineering concepts and tools are highlighted and current gaps in the knowledge are also mentioned. Finally, some recommendations are made for future research directions.
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Jay H. Lee obtained his B.S. degree in Chemical Engineering from the University of Washington, Seattle, in 1986, and his Ph.D. degree in Chemical Engineering from California Institute of Technology, Pasadena, in 1991. From 1991 to 1998, he was with the Department of Chemical Engineering at Auburn University, AL, as an Assistant Professor and an Associate Professor. From 1998–2000, he was with School of Chemical Engineering at Purdue University, West Lafayette and then with the School of Chemical Engineering at Georgia Institute of Technology, Atlanta. Starting this fall, he is the Head of the Chemical and Biomolecular Engineering Department at KAIST, Korea. He has held visiting appointments at E. I. Du Pont de Numours, Wilmington, in 1994 and at Seoul National University, Seoul, Korea, in 1997. He was a recipient of the National Science Foundation’s Young Investigator Award in 1993 and was elected as an IEEE Fellow, an IFAC Fellow, and a full member of the Korean Academy of Science and Technology in 2011. He is also the recipient of the 2013 Computing in Chemical Engineering Award given by the AIChE’s CAST Division. He published over 130 manuscripts in SCI journals with more than 3200 ISI citations. His research interests are in the areas of system identification, state estimation, robust control, model predictive control and approximate dynamic programming.
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Zaman, M., Lee, J.H. Carbon capture from stationary power generation sources: A review of the current status of the technologies. Korean J. Chem. Eng. 30, 1497–1526 (2013). https://doi.org/10.1007/s11814-013-0127-3
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DOI: https://doi.org/10.1007/s11814-013-0127-3