Abstract
The dry and wet deposition of N and S compounds to the Baltic Sea Basin were assessed using daily concentration measurements of air and precipitation concentrations, and actual meteorological data on precipitation, daily wind speed and wind direction, as well as the buoyant fluxes at the air- sea interface. The data cover the period 1980–86. Both concentrations and deposition levels show distinct south-north gradients and strong seasonal variability. Dry deposition is an important contribution in the case of S (25 to 80%) but is less significant for the N compounds (10 to 30%). The contribution of particles to dry deposition is negligible for S, equivalent to the gaseous contribution for oxidized N and about 10 to 20% for reduced nitrogen compounds. The obtained total annual deposition of about 1.4 to 1.8 g(S) m−2 for the S compounds, and 1 g(N) m−2 for the N compounds are comparable with, but on the upper side of, previous empirical and model estimates.
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References
Areskoug, H.: 1989, Deposition Estimates to the Baltic Sea Area Based on Reported Data for 1986, Baltic Marine Environment Protection Commission — Helsinki Commission, Baltic Sea Environment Proceedings No. 32, pp. 34–58.
Bortkovskii, R. S.: 1987, Air-Sea Exchange of Heat and Moisture During Storms, Kluwer Acad. Publishers, p. 194.
Brutsaert, W.: 1975, J. Atmos. Sci. 32, 2028.
Buat-Ménard, P. (ed.): 1985, The Role of Air-Sea Exchange in Geochemical Cycling, Kluwer Acad. Publishers, p. 549.
Derwent, R. G.: 1988, Estimation of Inputs of Nitrogen Compounds from the Atmosphere to the North Sea, AERE Report-R13329, Harwell Laboratory, Oxon.
Ferm, M.: 1984, Compilation of Atmospheric Concentration Data and Estimation of the Wet and Dry Deposition to the Baltic Sea, Swedish Environmental Research Institute Publication IVL-EM 1573.
Fitzgerald, J. W.: 1975, J. Appl. Meteor. 14, 1044.
Garratt, J. R. and Hicks, B. B.: 1973, Quart. J. Roy. Meteor. Soc. 99, 680.
Granat, L.: 1988, A Comparative Study of Precipitation Chemistry at Inland, Coastal and Island Sites in the Bothnian Bay Area, University of Stockholm, International Meteorological Institute, Report CM-73.
Harrison, R. M. and Pio, C. A.: 1983, Atmos. Environ. 17, 1733.
Hillamo, R.: 1989, The Use of Low Pressure Impactor in Size Distribution Measurements of Atmospheric Aerosols, Report Series in Aerosol Science 9, Finnish Association or Aerosol Research Publication, Helsinki, p. 82 (in Finnish).
Iversen, T., Saltbones, J., Sandnes, H., Eliassen, A., and Hov, Ö.: 1989, Airborne Transboundary Transport of Sulphur and Nitrogen over Europe — Model Descriptions and Calculations, EMEP MSC-W Report 2/89, Norwegian Meteorological Institute, Oslo, Norway.
Iversen, T., Halvorsen, N. E., Saltbones, J., and Sandnes, H.: 1990, Calculated Budgets for Airborne Sulphur and Nitrogen in Europe, EMEP/MSC-W Report 2/90, Norwegian Meteorological Institute, Oslo, Norway.
Joffre, S. M.: 1982, Bound. Layer Meteor. 24, 211.
Joffre, S. M.: 1985, The Structure of the Marine Atmospheric Boundary Layer: A Review from the Point of View of Diffusivity, Transport and Deposition Processes, Technical Report No. 29, Finnish Meteorological Institute, Helsinki, p. 119.
Joffre, S. M.: 1988a, Atmos. Environ. 22, 1137.
Joffre, S. M.: 1988b, Parameterization and Assessment of Processes Affecting the Long-Range Transport of Airborne Pollutants over the Sea. Finnish Meteorological Institute Contributions No. 1, p. 49.
Joffre, S. M. and Lindfors, V.: 1990, Observations of Airborne Pollutants over the Baltic Sea and Assessment of Their Transport, Chemistry and Deposition, Finnish Meteorological Institute Contributions No. 3, p. 41.
Large, W. G. and Pond, S.: 1981, J. Phys. Oceanogr. 11, 324.
Lindfors, V. and Joffre, S. M.: 1989, Transformation and Deposition of Airborne Gaseous and Paniculate Pollutants During Transport over the Baltic Sea. Finnish Meteorological Institute, Helsinki, Publications on Air Quality No. 5, p. 39 (in Finnish).
Lindfors, V., Joffre, S. M., and Damski, J.: 1991, Determination of the Wet and Dry Deposition of Sulphur and Nitrogen Compounds over the Baltic Sea Using Actual Meteorological Data, Finnish Meteorological Institute Contributions No. 4, p. 111.
Liss, P. S. and Slinn, W. G. N. (eds.): 1983, Air-Sea Exchange of Gases and Particles. Kluwer Acad. Publishers, Dordrecht, p. 561.
Meyers, T. P. and Yuen, T. S.: 1987, J. Geophys. Res. 92, 6705.
Monahan, E. C.: 1968, J. Geophys. Res. 73, 1127.
Petersen, G., Weber, H., and Grassl, H. 1989. ‘Modelling the Atmospheric Transport of Trace Metals from Europe to the North Sea and the Baltic Sea’, in J. M. Pacyna and B. Ottar (eds.), Control and Fate of Atmospheric Trace Metals, Kluwer Acad. Publishers, pp. 57–83.
Pierson, W. R. and Brachaczek, W. W.: 1988, Atmos. Environ. 22, 1665.
Rodhe, H., Söderlund, R., and Ekstedt, J.: 1980, Ambio 9, 168.
Schneider, B.: 1988, Input of Atmospheric Trace Metals to the Baltic Sea Area — An Estimate Based on the EGAP (HELCOM) — Monitoring Data, Contribution to the GESAMP-Meeting, October 1988, Rhode Island, USA.
Seinfeld, J. H.: 1986, Atmospheric Chemistry and Physics of Air Pollution, John Wiley & Sons, New York, p. 738.
Sirois, A. and Barrie, L. A.: 1988, Tellus 40B, 59.
Slinn, W. G. N.: 1983, ‘Air-to-Sea Transfer of Particles’, in Liss, P. S. and Slinn, W. G. N. (eds.), Air-Sea Exchange of Gases and Particles. Kluwer Acad. Publishers, p. 299–405.
Slinn, S. A. and Slinn, W. G. N.: 1980, Atmos. Environ. 14, 1013.
Söderlund, R. and Areskoug, H.: 1989, Deposition Estimates to the Baltic Sea Area Based on Reported Data for 1983–1985, Baltic Marine Environment Protection Commission — Helsinki Commission — 1989, Baltic Sea Environment Proceedings No. 32, p. 5–33.
Stull, R. B.: 1988, An Introduction to Boundary Layer Meteorology, Kluwer Acad. Publishers, Dordrecht, p. 666.
Van Aalst, R. M. van Ardenne, R. M., de Kreuk, J. F., and Lems, Th.: 1983, Pollution of the North Sea from the Atmosphere. Netherlands Organization for Applied Scientific Research. TNO Report CL 82/152.
Voipio, A. (ed.): 1981, The Baltic Sea, Elsevier Oceanography Series 30, Elsevier, Amsterdam.
Voldner, E. C., Barrie, L. A., and Sirois, A.: 1986, Atmos Environ. 20, 2101.
Wall, S. M., John, W., and Ondo, J. L.: 1988, Atmos. Environ. 22, 1649.
Williams, R. M.: 1982, Atmos. Environ. 16, 1933.
Wu, J.: 1979, J. Phys. Oceanogr. 9, 1064.
Wu, J.: 1988, J. Phys. Oceanogr. 18, 1448.
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Lindfors, V., Joffre, S.M. & Damski, J. Meteorological variability of the wet and dry deposition of sulphur and nitrogen compounds over the baltic sea. Water Air Soil Pollut 66, 1–28 (1993). https://doi.org/10.1007/BF00477058
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DOI: https://doi.org/10.1007/BF00477058