Abstract
Determination of sedimentary fluxes of222Rn via diffusion was required as an input for a mass balance model of radon in a freshwater lake. We obtained these fluxes by: (1) direct measurement in the laboratory using a simulated sediment bed and water column; (2) a “sediment equilibration” technique; and (3) porewater modeling. The first method, analogous to an in situ benthic chamber approach, uses direct observation of the increasing222Rn activity in water overlying a sediment bed packed in plastic columns. This allows one to directly measure the fluxes and determine the effective wet bulk sediment diffusion coefficient (D s). Radon flux estimates using these three techniques agreed to within approximately 10–15%.
Similar content being viewed by others
References
R. M. Key, N. L. Guinasso, Jr., D. R. Schink, Mar. Chem., 7 (1979) 221.
D. E. Hammond, H. J. Simpson, G. Mathieu, J. Geophys. Res., 82 (1977) 3913.
K. A. Gruebel, C. S. Martens, Limnol. Oceanogr., 29 (1984) 587.
C. S. Martens, J. P. Chanton, J. Geophys. Res., 94 (1989) 3451.
J. E. Cable, G. C. Bugna, W. C. Burnett, J. P. Chanton, Limnol. Oceanogr., 41 (1996) 1347.
D. R. Corbett, W. C. Burnett, P. H. Cable, S. B. Clark, J. Hydrology (1997) in press.
C. S. Martens, G. W. Kipphut, J. V. Klump, Science, 208 (1980) 285.
G. G. Mathieu, R. A. Lupton, D. E. Hammond, Health Phys., 55 (1988) 989.
R. H. Hesslein, Limnol. Oceanogr., 41 (1976) 1347.
T. H. Peng, T. Takahashi, W. S. Brocker, J. Geophys. Res., 79 (1974) 1772.
W. J. Ullman, R. C. Aller, Limnol. Oceanogr., 27 (1982) 552
R. A. Berner, Principles of chemical sedimentology, McGraw-Hill, New York, N.Y., 1971, p. 240.
W. S. Broecker, T. H. Peng, Tellus, 26 (1974) 21.
B. Hartman, D. E. Hammond, J. Geophys. Res., 89 (1984) 3593.
J. E. Cable, W. C. Burnett, J. P. Chanton, G. L. Weatherly, Estuarine, Coastal and Shelf Science, 144 (1996) 591.
R. A. Berner, Early Diagenesis: A Theoretical Approach, Princeton University Press, Princeton, N.J., 1980, p. 241.
Author information
Authors and Affiliations
Rights and permissions
About this article
Cite this article
Corbett, D.R., Burnett, W.C., Cable, P.H. et al. A multiple approach to the determination of radon fluxes from sediments. J Radioanal Nucl Chem 236, 247–253 (1998). https://doi.org/10.1007/BF02386351
Received:
Issue Date:
DOI: https://doi.org/10.1007/BF02386351