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Journal of Materials Science
Erschienen in: Journal of Materials Science 24/2015

01.12.2015 | Original Paper

One-pot hydrothermal route to synthesize the ZnIn2S4/g-C3N4 composites with enhanced photocatalytic activity

verfasst von: Wei Chen, Tian-Yu Liu, Ting Huang, Xiao-Heng Liu, Jun-Wu Zhu, Guo-Rong Duan, Xu-Jie Yang

Erschienen in: Journal of Materials Science | Ausgabe 24/2015

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Abstract

Heterogeneous ZnIn2S4/g-C3N4 hybrid composites, as highly efficient visible-light-driven photocatalysts, were designed and fabricated by a simple one-step hydrothermal route for the first time, wherein the cubic ZnIn2S4 nanoparticles were in situ immobilized on the surface of porous g-C3N4 nanosheets (NSs). The resultant composites exhibit efficient photocatalytic activities, excellent photo-stability, and versatile photocatalytic abilities towards organic dye degradation, Cr(VI) reduction, and water splitting for H2 evolution. The significant enhancement of photocatalytic activity is attributed to the effective separation of photo-generated charge carrier pairs based on the construction of close heterogeneous interface and well-matched band structure, which can obviously lengthen the life span of holes and electrons pairs. Besides, the effective charge transfer from cubic ZnIn2S4 to ultrathin g-C3N4 NSs was confirmed by photoluminescence spectra, transient photocurrent–time (I–t) curves and electrochemical impedance spectroscopy Nyquist plots. This research provides a new sight in designing the highly efficient visible light responsive photocatalysts for environmental remediation and energy production.
Vorheriger Artikel Atomic scale modeling of shock response of fused silica and α-quartz
Nächster Artikel Surface-specific visible light luminescence from composite metal oxide nanocrystals

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Metadaten
Titel
One-pot hydrothermal route to synthesize the ZnIn2S4/g-C3N4 composites with enhanced photocatalytic activity
verfasst von
Wei Chen
Tian-Yu Liu
Ting Huang
Xiao-Heng Liu
Jun-Wu Zhu
Guo-Rong Duan
Xu-Jie Yang
Publikationsdatum
01.12.2015
Verlag
Springer US
Erschienen in
Journal of Materials Science / Ausgabe 24/2015
Print ISSN: 0022-2461
Elektronische ISSN: 1573-4803
DOI
https://doi.org/10.1007/s10853-015-9388-z

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