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Journal of Materials Science

Erschienen in:

13.04.2020 | Chemical routes to materials

H₃PW₁₂O₄₀-doped pyromellitic diimide prepared via thermal transformation as an efficient visible-light photocatalyst

verfasst von: Xiaoyi Huang, Wang Wang, Xia Liu

Erschienen in: Journal of Materials Science | Ausgabe 20/2020

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Abstract

We prepared the H₃PW₁₂O₄₀-doped pyromellitic diimide (PMDI) photocatalysts via thermal transformation using urea phosphotungstate and pyromellitic dianhydride as precursors (UPWPI) and calcination of PMDI with phosphotungstic acid directly (UPIPW). The influences of the strategies on the morphology, light absorption, and visible-light photocatalytic degradation efficiency of H₃PW₁₂O₄₀-doped PMDI are systematically investigated by various characterization methods. By comparing the structure of UPWPI and UPIPW, the adoption of urea phosphotungstate as precursors can promote the separation of PMDI into small particles and the inclusion of phosphotungstic acid. Moreover, the visible-light (λ > 420 nm) absorption efficiency of UPWPI is also enhanced compared with that of UPIPW because of the improved photogenerated electron transfer efficiency between PMDI and HPW. With a catalyst dosage of 100 mg and the degradation time of 3 h, the photocatalytic degradation efficiency of imidacloprid on UPWPI was 97.12% and the degradation rate constant was 0.93 h⁻¹.

Vorheriger Artikel Bond analysis of novel MnZrTa2O8 microwave dielectric ceramics with monoclinic structure

Nächster Artikel Characterization of discarded fruit waste as substitute for harmful synthetic fiber-reinforced polymer composites

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Titel: H3PW12O40-doped pyromellitic diimide prepared via thermal transformation as an efficient visible-light photocatalyst
verfasst von: Xiaoyi Huang
Wang Wang
Xia Liu
Publikationsdatum: 13.04.2020
Verlag: Springer US
Erschienen in: Journal of Materials Science / Ausgabe 20/2020
Print ISSN: 0022-2461
Elektronische ISSN: 1573-4803
DOI: https://doi.org/10.1007/s10853-020-04642-2

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