Skip to main content
Erschienen in: Environmental Earth Sciences 12/2015

01.06.2015 | Thematic Issue

Combination of MIEX® resin and ozonation for reduction of dissolved organic matter during aquifer recharge using municipal effluent

verfasst von: Xue Zhang, Xuan Zhao, Yutuan Gao, Meng Zhang

Erschienen in: Environmental Earth Sciences | Ausgabe 12/2015

Einloggen

Aktivieren Sie unsere intelligente Suche um passende Fachinhalte oder Patente zu finden.

search-config
loading …

Abstract

Magnetic anion exchange resin treatment (MIEX®), as well as ozonation, was applied as pretreatment for soil aquifer treatment (SAT). The removal of dissolved organic matter (DOM) derived from municipal effluent was characterized during these treatments. The DOM removal ratio increased with the increasing of MIEX® resin dosage (5–20 mL/L), and a dosage of 5–10 mL/L was suggested for the SAT pretreatment. Under this dosage, 30 % DOC was removed from secondary effluent, which was much lower than those found with drinking water resources. The aromatic DOM with apparent molecular weight (AMW) ranging 2–5 kDa was preferentially removed by MIEX®, especially for aromatic proteins. Differently, ozonation preferentially destroyed larger AMW (>10 kDa) DOM, especially for fulvic and humic acid-like materials. Better purifucation was achieved by combining the two technologies. With pretreatments (MIEX®, ozonation, and combined MIEX®/ozonation), the DOM removals by SAT were significantly improved. The DOC and UV254 values were reduced by 40–77 % in SAT combined with pretreatments, compared with 20–30 % reduction by only SAT. Around 50% of the fluorescent DOM was reduced in SAT and MIEX/SAT systems, while higher reductions (76-84%) were achieved in ozonation/SAT and MIEX/Ozonation/SAT systems. Different modes were identified: ozonation improved SAT on removing DOM of 1.7–5.3 kDa, whereas MIEX® treatment attributed to the removal of small AMW (0.5–1.7 kDa) DOM responsible for the absorbance peak at 300 nm. Based on the results, DOM removed by MIEX® treatment is complementary with those removed by SAT and ozonation, and the best DOM purification was found in combined MIEX®/ozonation/SAT.

Sie haben noch keine Lizenz? Dann Informieren Sie sich jetzt über unsere Produkte:

Springer Professional "Wirtschaft+Technik"

Online-Abonnement

Mit Springer Professional "Wirtschaft+Technik" erhalten Sie Zugriff auf:

  • über 102.000 Bücher
  • über 537 Zeitschriften

aus folgenden Fachgebieten:

  • Automobil + Motoren
  • Bauwesen + Immobilien
  • Business IT + Informatik
  • Elektrotechnik + Elektronik
  • Energie + Nachhaltigkeit
  • Finance + Banking
  • Management + Führung
  • Marketing + Vertrieb
  • Maschinenbau + Werkstoffe
  • Versicherung + Risiko

Jetzt Wissensvorsprung sichern!

Springer Professional "Technik"

Online-Abonnement

Mit Springer Professional "Technik" erhalten Sie Zugriff auf:

  • über 67.000 Bücher
  • über 390 Zeitschriften

aus folgenden Fachgebieten:

  • Automobil + Motoren
  • Bauwesen + Immobilien
  • Business IT + Informatik
  • Elektrotechnik + Elektronik
  • Energie + Nachhaltigkeit
  • Maschinenbau + Werkstoffe




 

Jetzt Wissensvorsprung sichern!

Literatur
Zurück zum Zitat Allpike BP, Heitz A, Joll CA, Kagi RI, Abbt-Braun G, Frimmel FH, Brinkmann T, Her N, Amy G (2005) Size exclusion chromatography to characterize DOC removal in drinking water treatment. Environ Sci Technol 39(7):2334–2342CrossRef Allpike BP, Heitz A, Joll CA, Kagi RI, Abbt-Braun G, Frimmel FH, Brinkmann T, Her N, Amy G (2005) Size exclusion chromatography to characterize DOC removal in drinking water treatment. Environ Sci Technol 39(7):2334–2342CrossRef
Zurück zum Zitat Chen W, Westerhoff P, Leenheer JA, Booksh K (2003) Fluorescence excitation emission matrix regional integration to quantify spectra for dissolved organic matter. Environ Sci Technol 37:5701–5710CrossRef Chen W, Westerhoff P, Leenheer JA, Booksh K (2003) Fluorescence excitation emission matrix regional integration to quantify spectra for dissolved organic matter. Environ Sci Technol 37:5701–5710CrossRef
Zurück zum Zitat Chow CWK, Fabris R, van Leeuwen J, Wang DS, Drikas M (2008) Assessing natural organic matter treatability using high performance size exclusion chromatography. Environ Sci Technol 42:6683–6689CrossRef Chow CWK, Fabris R, van Leeuwen J, Wang DS, Drikas M (2008) Assessing natural organic matter treatability using high performance size exclusion chromatography. Environ Sci Technol 42:6683–6689CrossRef
Zurück zum Zitat Cordy GE, Duran NL, Bouwer H, Rice RC, Furlong ET, Zaugg SD, Meyer MT, Barber LB, Kolpin DW (2004) Do pharmaceuticals, pathogens, and other organic waste water compounds persist when waste water is used for recharge? Ground Water Monit Rem 24:58–69CrossRef Cordy GE, Duran NL, Bouwer H, Rice RC, Furlong ET, Zaugg SD, Meyer MT, Barber LB, Kolpin DW (2004) Do pharmaceuticals, pathogens, and other organic waste water compounds persist when waste water is used for recharge? Ground Water Monit Rem 24:58–69CrossRef
Zurück zum Zitat Drewes JE, Jekel M (1998) Behavior of DOC and AOX using advanced treated wastewater for groundwater recharge. Water Res 32:3125–3133CrossRef Drewes JE, Jekel M (1998) Behavior of DOC and AOX using advanced treated wastewater for groundwater recharge. Water Res 32:3125–3133CrossRef
Zurück zum Zitat Drikas M, Chow CWK, Cook D (2003) The impact of recalcitrant organic character on disinfection stability, trihalomethane formation and bacterial regrowth: an evaluation of magnetic ion exchange resin (MIEX®) and alum coagulation. J Water Supply Res Tech Aqua 52:475–487 Drikas M, Chow CWK, Cook D (2003) The impact of recalcitrant organic character on disinfection stability, trihalomethane formation and bacterial regrowth: an evaluation of magnetic ion exchange resin (MIEX®) and alum coagulation. J Water Supply Res Tech Aqua 52:475–487
Zurück zum Zitat Fox P, Aboshanp W, Alsamadi B (2005) Analysis of soils to demonstrate sustained organic carbon removal during soil aquifer treatment. J Environ Qual 34:156–163 Fox P, Aboshanp W, Alsamadi B (2005) Analysis of soils to demonstrate sustained organic carbon removal during soil aquifer treatment. J Environ Qual 34:156–163
Zurück zum Zitat Humbert H, Gallard H, Suty H, Croué JP (2005) Performance of selected anion exchange resins for the treatment of a high DOC content surface water. Water Res 39:1699–1708CrossRef Humbert H, Gallard H, Suty H, Croué JP (2005) Performance of selected anion exchange resins for the treatment of a high DOC content surface water. Water Res 39:1699–1708CrossRef
Zurück zum Zitat Johnson CJ, Singer PC (2004) Impact of a magnetic ion exchange resin on ozone demand and bromate formation during drinking water treatment. Water Res 38:3738–3750CrossRef Johnson CJ, Singer PC (2004) Impact of a magnetic ion exchange resin on ozone demand and bromate formation during drinking water treatment. Water Res 38:3738–3750CrossRef
Zurück zum Zitat Katsoyiannis A, Samara C (2007) The fate of dissolved organic carbon (DOC) in the wastewater treatment process and its importance in the removal of wastewater contaminants. Environ Sci Pollut Res 14:284–292CrossRef Katsoyiannis A, Samara C (2007) The fate of dissolved organic carbon (DOC) in the wastewater treatment process and its importance in the removal of wastewater contaminants. Environ Sci Pollut Res 14:284–292CrossRef
Zurück zum Zitat Kitis M, Harman BI, Yigit NO, Beyhan M, Nguyen H, Adams B (2007) The removal of natural organic matter from selected Turkish source waters using magnetic ion exchange resin (MIEX®). React Funct Polym 67(12):1495–1504CrossRef Kitis M, Harman BI, Yigit NO, Beyhan M, Nguyen H, Adams B (2007) The removal of natural organic matter from selected Turkish source waters using magnetic ion exchange resin (MIEX®). React Funct Polym 67(12):1495–1504CrossRef
Zurück zum Zitat Liu S, Lim M, Fabris R, Chow CWK, Drikas M, Korshin G, Amal R (2010) Multi-wavelength spectroscopic and chromatography study on the photocatalytic oxidation of natural organic matter. Water Res 44:2525–2532CrossRef Liu S, Lim M, Fabris R, Chow CWK, Drikas M, Korshin G, Amal R (2010) Multi-wavelength spectroscopic and chromatography study on the photocatalytic oxidation of natural organic matter. Water Res 44:2525–2532CrossRef
Zurück zum Zitat Maeng SK, Sharma SK, Lekkerkerker-Teunissen K, Amy GL (2011) Occurrence and fate of bulk organic matter and pharmaceutically active compounds in managed aquifer recharge: a review. Water Res 45:3015–3033CrossRef Maeng SK, Sharma SK, Lekkerkerker-Teunissen K, Amy GL (2011) Occurrence and fate of bulk organic matter and pharmaceutically active compounds in managed aquifer recharge: a review. Water Res 45:3015–3033CrossRef
Zurück zum Zitat Miller GW (2006) Integrated concepts in water reuse: managing global water needs. Desalination 187:65–75CrossRef Miller GW (2006) Integrated concepts in water reuse: managing global water needs. Desalination 187:65–75CrossRef
Zurück zum Zitat Nguyen TV, Zhang R, Vigneswaran S, Ngo HH, Kandasamy J, Mathes P (2011) Removal of organic matter from effluents by Magnetic Ion Exchange (MIEX®). Desalination 276:96–102CrossRef Nguyen TV, Zhang R, Vigneswaran S, Ngo HH, Kandasamy J, Mathes P (2011) Removal of organic matter from effluents by Magnetic Ion Exchange (MIEX®). Desalination 276:96–102CrossRef
Zurück zum Zitat Quanrud DM, Hafer J, Karpiscak MM, Zhang HM, Lansey KE, Arnold RG (2003) Fate of organics during soil-aquifer treatment: sustainability of removals in the field. Water Res 37:3401–3411CrossRef Quanrud DM, Hafer J, Karpiscak MM, Zhang HM, Lansey KE, Arnold RG (2003) Fate of organics during soil-aquifer treatment: sustainability of removals in the field. Water Res 37:3401–3411CrossRef
Zurück zum Zitat Singer PC, Bilyk K (2002) Enhanced coagulation using a magnetic ion exchange resin. Water Res 36:4009–4022CrossRef Singer PC, Bilyk K (2002) Enhanced coagulation using a magnetic ion exchange resin. Water Res 36:4009–4022CrossRef
Zurück zum Zitat Wang S, Ma J, Liu B, Jiang Y, Zhang H (2008) Degradation characteristics of secondary effluent of domestic wastewater by combined process of ozonation and biofiltration. J Hazard Mater 150:109–114CrossRef Wang S, Ma J, Liu B, Jiang Y, Zhang H (2008) Degradation characteristics of secondary effluent of domestic wastewater by combined process of ozonation and biofiltration. J Hazard Mater 150:109–114CrossRef
Zurück zum Zitat Wu LL, Zhao X, Zhang M (2011) Removal of dissolved organic matter in municipal effluent with ozonation, slow sand filtration and nanofiltration as high quality pre-treatment option for artificial groundwater recharge. Chemosphere 83:693–699CrossRef Wu LL, Zhao X, Zhang M (2011) Removal of dissolved organic matter in municipal effluent with ozonation, slow sand filtration and nanofiltration as high quality pre-treatment option for artificial groundwater recharge. Chemosphere 83:693–699CrossRef
Zurück zum Zitat Xue S, Zhao QL, Wei LL, Ren NQ (2009) Behavior and characteristics of dissolved organic matter during column studies of soil aquifer treatment. Water Res 43:499–507CrossRef Xue S, Zhao QL, Wei LL, Ren NQ (2009) Behavior and characteristics of dissolved organic matter during column studies of soil aquifer treatment. Water Res 43:499–507CrossRef
Zurück zum Zitat Yi LL, Jiao W, Chen X, Chen W (2011) An overview of reclaimed water reuse in China. J Environ Sci 23:1585–1593CrossRef Yi LL, Jiao W, Chen X, Chen W (2011) An overview of reclaimed water reuse in China. J Environ Sci 23:1585–1593CrossRef
Zurück zum Zitat Zhang ZY, Lei ZF, Zhang ZY, Sugiura N, Xu XT, Yin DD (2007) Organics removal of combined wastewater through shallow soil infiltration treatment: a field and laboratory study. J Hazard Mater 149:657–665CrossRef Zhang ZY, Lei ZF, Zhang ZY, Sugiura N, Xu XT, Yin DD (2007) Organics removal of combined wastewater through shallow soil infiltration treatment: a field and laboratory study. J Hazard Mater 149:657–665CrossRef
Zurück zum Zitat Zhang X, Li FZ, Zhao X (2012) Application of a magnetic resin (MIEX®) in wastewater reclamation for managed aquifer recharge. Water Air Soil Poll 223:4687–4694CrossRef Zhang X, Li FZ, Zhao X (2012) Application of a magnetic resin (MIEX®) in wastewater reclamation for managed aquifer recharge. Water Air Soil Poll 223:4687–4694CrossRef
Zurück zum Zitat Zhao X, Zhang M, Cheng XZ (2009) Bulk organic matter and nitrogen removal from reclaimed water during groundwater recharge by enhanced direct injection well. Water Environ Res 81:69–75CrossRef Zhao X, Zhang M, Cheng XZ (2009) Bulk organic matter and nitrogen removal from reclaimed water during groundwater recharge by enhanced direct injection well. Water Environ Res 81:69–75CrossRef
Metadaten
Titel
Combination of MIEX® resin and ozonation for reduction of dissolved organic matter during aquifer recharge using municipal effluent
verfasst von
Xue Zhang
Xuan Zhao
Yutuan Gao
Meng Zhang
Publikationsdatum
01.06.2015
Verlag
Springer Berlin Heidelberg
Erschienen in
Environmental Earth Sciences / Ausgabe 12/2015
Print ISSN: 1866-6280
Elektronische ISSN: 1866-6299
DOI
https://doi.org/10.1007/s12665-014-3292-8

Weitere Artikel der Ausgabe 12/2015

Environmental Earth Sciences 12/2015 Zur Ausgabe