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Toward Practical All-solid-state Batteries with Sulfide Electrolyte: A Review

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Chemical Research in Chinese Universities Aims and scope

Abstract

Sulfide-based solid-state electrolytes with ultrahigh lithium ion conductivities have been considered as the most promising electrolyte system to enable practical all-solid-state batteries. However, the practical applications of the sulfide-based all-solid-state batteries are hindered by severe interfacial issues as well as large-scale material preparation and battery fabrication problems. Liquid-involved interfacial treatments and preparation processes compatible with current battery manufacturing capable of improving electrode/electrolyte interface contacts and realizing the mass production of sulfide electrolytes and the scalable fabrication of sulfide-based battery component have attracted considerable attention. In this perspective, the current advances in liquid-involved treatments and processes in sulfide-based all-solid-state batteries are summarized. Then relative chemical mechanisms and existing challenges are included. Finally, future guidance is also proposed for sulfide-based batteries. Focusing on the sulfide-based all-solid-state batteries, we aim at providing a fresh insight on understandings towards liquid-involved processes and promoting the development of all-solid-state batteries with higher energy density and better safety.

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Authors and Affiliations

  1. Advanced Research Institute of Multidisciplinary Science, Beijing Institute of Technology, Beijing, 100081, P. R. China

    Hong Yuan & Jiaqi Huang

  2. Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University, Beijing, 100084, P. R. China

    Hong Yuan, Jia Liu, Yang Lu, Chenzi Zhao, Xinbing Cheng & Qiang Zhang

  3. Beijing Key Laboratory of Lignocellulosic Chemistry, Beijing Forestry University, Beijing, 100083, P. R. China

    Jia Liu

  4. School of Chemical Engineering and Light Industry, Guangdong University of Technology, Guangzhou, 510006, P. R. China

    Haoxiong Nan & Quanbing Liu

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  1. Hong Yuan
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  8. Jiaqi Huang
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  9. Qiang Zhang
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Corresponding author

Correspondence to Qiang Zhang.

Additional information

Supported by the National Natural Science Foundation of China(Nos.21808124, 21825501, U1801257), the National Key Research and Development Program of China(Nos.2016YFA0202500, 2016YFA0200102) and the China Postdoctoral Science Foundation(No.2019T120098).

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Yuan, H., Liu, J., Lu, Y. et al. Toward Practical All-solid-state Batteries with Sulfide Electrolyte: A Review. Chem. Res. Chin. Univ. 36, 377–385 (2020). https://doi.org/10.1007/s40242-020-0103-5

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  • DOI: https://doi.org/10.1007/s40242-020-0103-5

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