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Electrospun Metal–Organic Framework Nanofiber Membranes for Energy Storage and Environmental Protection

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Abstract

Metal–organic frameworks (MOFs) are attractive in many fields due to their unique advantages. However, the practical applications of single MOF materials are limited. In recent years, a large number of MOF-based composites have been investigated to overcome the defects of single MOF materials to broaden the avenues for the practical applications of MOFs. Among them, MOF-based hybrid nanofiber membranes fabricated by electrospinning combine the advantages of polymer nanofibers and inorganic porous materials, receiving extensive attention and development in energy storage and environmental protection. This review systematically summarizes the recent progress of MOF-based hybrid nanofiber membranes prepared by electrospinning from the perspectives of preparation and application. Firstly, two main methods for preparing MOF/polymer nanofibrous membranes are discussed. Next, the applications of MOF/polymer nanofibrous membranes in energy storage and environmental protection are summarized at length. Finally, to fully tap the potential of MOF-based nanofiber membranes in more fields, the current challenges are proposed, and future research directions are discussed.

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Fig. 1
Fig. 2

Reproduced with permission from Ref [123]. Copyright 2012, the Royal Society of Chemistry. SEM pictures of c PI and d ZIF-8/PI membranes after filtering PM2.5 in the air; exhibition of ZIF-8/PI membrane e stiffness and f flexibility. Reproduced with permission from Ref [126]. Copyright 2019, American Chemical Society. g Schematic diagram of the in situ growth of ZIF-8 on electrospinning nanofibers; h formation mechanism of the in situ ZIF-8/PAN nanofibers; SEM images of i the in situ ZIF-8/PAN nanofibers and j PAN; k, l TEM images of the in situ ZIF-8/PAN nanofibers. Reproduced with permission from Ref [133]. Copyright 2018, American Chemical Society

Fig. 3

Reproduced with permission from Ref [134]. Copyright 2018, the Royal Society of Chemistry. k Schematic diagram of the fabrication procedures of PAN@ZIF-8 electrospinning fibers; SEM pictures of l ZIF-8 on the PAN and m, n the ZIF-8/PAN nanofibers. Reproduced with permission from Ref [105]. Copyright 2016, the Royal Society of Chemistry

Fig. 4

Reproduced with permission from Ref [135]. Copyright 2019, the Royal Society of Chemistry. Schematic diagram of the preparation of UiO-66-NH2/PAN fiber membranes by in situ growth of UiO-66-NH2 on electrospinning fibers: d control PAN sample; e PAN with ATA; f control PAN post-synthesis; g PAN with ATA post-synthesis. Reproduced with permission from Ref [136]. Copyright 2017, American Chemical Society

Fig. 5

Reproduced with permission from Ref [138]. Copyright 2014, the Royal Society of Chemistry. f Schematic sketch of the fabrication of PAN fiber membrane covered with UiO-66-NH2. Reproduced with permission from Ref [140]. Copyright 2019, Elsevier

Fig. 6

Reproduced with permission from Ref [115]. Copyright 2019, Elsevier. f Preparation of the CNT/Co3O4 microtubes; Electrochemical properties of the CNT/Co3O4 microtubes: g Charge–discharge voltage profiles at 0.1 A·g−1; h rate performance at different current densities. Reproduced with permission from Ref [163]. Copyright 2016, Wiley–VCH

Fig. 7

Reproduced with permission from Ref [175]. Copyright 2020, the Royal Society of Chemistry. f Schematic diagram of the fabrication route for C/Co9S8–C@S nanofiber; g cycle properties and coulombic efficiency of the C/Co9S8–C@S nanofibers at 1 C; h cycle properties and coulombic efficiency of C/Co9S8–C@S nanofibers, C/Co9S8@S polyhedron, C@S nanofibers and the sulfur cathode at 0.1 C. Reproduced with permission from Ref [176]. Copyright 2021, Elsevier

Fig. 8

Reproduced with permission from Ref [193]. Copyright 2020, Elsevier. f Schematic diagram of the synthetic process of Fe7S8/N-CNFs; g FESEM picture of Fe7S8/N-CNFs; h HRTEM picture and nanoparticle size distribution (the inset) of Fe7S8/N-CNFs; i charge/discharge curves of the Fe7S8/N-CNFs electrode for the first, second, 30th, 50th and 100th cycles at 0.1 A·g−1; j cycle performance and coulombic efficiency of the Fe7S8/N-CNFs electrode at 0.2 A·g−1. Reproduced with permission from ref [194]. Copyright 2021, Wiley–VCH

Fig. 9

Reproduced with permission from Ref [205]. Copyright 2020, American Chemical Society. d Schematic diagram of the fabrication of pearl-necklace-like composite fiber membranes; e adsorption capacity of all samples for Cr6+ and Cu2+; f effect of contact time on the adsorption of Cr6+ and Cu2+ on the ZIF/CA-24 (experimental condition: at room temperature, pH ≈ 6.5, without stirring). Reproduced with permission from Ref [206]. Copyright 2018, Wiley–VCH. g Preparation of bio-MOF/PAN membrane and its adsorption of cationic dyes; h adsorption capacity of bio-MOF/PAN filter for MB+ with different original concentrations; i adsorption capacity of bio-MOF/PAN filter for MB+ in five cycles. Reproduced with permission from Ref [212]. Copyright 2020, Elsevier. j Fabrication Process of the PLA/ZIF-8@GO composite nanofiber membranes; k mechanisms of photocatalytic degradation of MB on PLA/ZIF-8@GO nanofibers; l removal efficiency of MB on PLA/ZIF-8@GO nanofibers with three cycles. Reproduced with permission from Ref [213]. Copyright 2018, American Chemical Society

Fig. 10

Reproduced with permission from Ref [220]. Copyright 2019, the Royal Society of Chemistry. SEM images of d PI membranes and e ZIF-8/PI membranes; f PM2.5 removal efficiency of different membranes; g the concentration of PM2.5 captured by different membranes in harsh conditions. Reproduced with permission from Ref [126]. Copyright 2019, American Chemical Society

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Acknowledgements

This work was supported by the National Natural Science Foundation of China (NSFC-U1904215), Natural Science Foundation of Jiangsu Province (BK20200044), Changjiang scholars program of the Ministry of Education (Q2018270).

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  1. School of Chemistry and Chemical Engineering, Yangzhou University, Yangzhou, 225002, Jiangsu, People’s Republic of China

    Xiaoge Liu, Yi Zhang, Xiaotian Guo & Huan Pang

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  1. Xiaoge Liu
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  2. Yi Zhang
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  3. Xiaotian Guo
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Liu, X., Zhang, Y., Guo, X. et al. Electrospun Metal–Organic Framework Nanofiber Membranes for Energy Storage and Environmental Protection. Adv. Fiber Mater. 4, 1463–1485 (2022). https://doi.org/10.1007/s42765-022-00214-y

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