The thermodynamics of interstitial-vacancy interactions in solid solutions
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2016, Journal of Alloys and CompoundsCitation Excerpt :These models have been formulated on the base of the thermodynamic equilibrium involving the solution energy of H incorporation in the interstitial sites of a perfect crystal and the formation energy of H-vacancy clusters. The distribution of the H atoms and the vacancies has been taken into account from the Maxwell–Boltzmann statistics [59], the Fermi–Dirac distribution function [25,42,60–62] or from a linear mixing of the Ni–H solid solution [40]. However, no non-configurational entropic contributions have been taken into account in these models and no clear correlations have been made between the presence of vacancies and the macroscopic solubility of hydrogen in nickel so far.
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