Abstract
Control of spontaneously emitted light lies at the heart of quantum optics. It is essential for diverse applications ranging from miniature lasers and light-emitting diodes1,2,3,4,5, to single-photon sources for quantum information6,7,8, and to solar energy harvesting9. To explore such new quantum optics applications, a suitably tailored dielectric environment is required in which the vacuum fluctuations that control spontaneous emission can be manipulated10,11. Photonic crystals provide such an environment: they strongly modify the vacuum fluctuations, causing the decay of emitted light to be accelerated or slowed down12,13, to reveal unusual statistics14, or to be completely inhibited in the ideal case of a photonic bandgap1,15. Here we study spontaneous emission from semiconductor quantum dots embedded in inverse opal photonic crystals16. We show that the spectral distribution and time-dependent decay of light emitted from excitons confined in the quantum dots are controlled by the host photonic crystal. Modified emission is observed over large frequency bandwidths of 10%, orders of magnitude larger than reported for resonant optical microcavities17. Both inhibited and enhanced decay rates are observed depending on the optical emission frequency, and they are controlled by the crystals' lattice parameter. Our experimental results provide a basis for all-solid-state dynamic control of optical quantum systems18.
This is a preview of subscription content, access via your institution
Access options
Subscribe to this journal
Receive 51 print issues and online access
$199.00 per year
only $3.90 per issue
Buy this article
- Purchase on Springer Link
- Instant access to full article PDF
Prices may be subject to local taxes which are calculated during checkout
Similar content being viewed by others
References
Yablonovitch, E. Inhibited spontaneous emission in solid-state physics and electronics. Phys. Rev. Lett. 58, 2059–2062 (1987)
Painter, O. et al. Two-dimensional photonic band-gap defect mode laser. Science 284, 1819–1821 (1999)
Smith, C. J. M. et al. Near-infrared microcavities confined by two-dimensional photonic bandgap crystals. Electron. Lett. 35, 228–230 (1999)
Colombelli, R. et al. Quantum cascade surface-emitting photonic crystal laser. Science 302, 1374–1377 (2003)
Noda, S. et al. Polarization mode control of two-dimensional photonic crystal laser by unit cell structure design. Science 293, 1123–1125 (2001)
Kim, J., Benson, O., Kan, H. & Yamamoto, Y. A single-photon turnstile device. Nature 397, 500–503 (1999)
Michler, P. et al. A quantum dot single-photon turnstile device. Science 290, 2282–2285 (2000)
Kuhn, A., Hennrich, M. & Rempe, G. Deterministic single-photon source for distributed quantum networking. Phys. Rev. Lett. 89, 067901 (2002)
Grätzel, M. Photoelectrochemical cells. Nature 414, 338–344 (2001)
Scully, M. O. & Zubairy, M. S. Quantum Optics (Cambridge Univ. Press, Cambridge, 1997)
Loudon, R. The Quantum Theory of Light (Oxford Univ. Press, New York, 2000)
Bykov, V. P. Spontaneous emission from a medium with a band spectrum. Sov. J. Quant. Electron. 4, 861–871 (1975)
Lambropoulos, P., Nikolopoulos, G. M., Nielsen, T. R. & Bay, S. Fundamental quantum optics in structured reservoirs. Rep. Prog. Phys. 63, 455–503 (2000)
John, S. & Quang, T. Spontaneous emission near the edge of a photonic band gap. Phys. Rev. A 50, 1764–1769 (1994)
John, S. Strong localization of photons in certain disordered dielectric superlattices. Phys. Rev. Lett. 58, 2486–2489 (1987)
Wijnhoven, J. E. G. J. & Vos, W. L. Preparation of photonic crystals made of air spheres in titania. Science 281, 802–804 (1998)
Vahala, K. J. Optical microcavities. Nature 424, 839–846 (2003)
Mabuchi, H. & Doherty, A. C. Cavity quantum electrodynamics: coherence in context. Science 298, 1372–1377 (2002)
Sprik, R., van Tiggelen, B. A. & Lagendijk, A. Optical emission in periodic dielectrics. Europhys. Lett. 35, 265–270 (1996)
Busch, K. & John, S. Photonic band gap formation in certain self-organizing systems. Phys. Rev. E 58, 3896–3908 (1998)
Koenderink, A. F. & Vos, W. L. Light exiting from real photonic band gap crystals is diffuse and strongly directional. Phys. Rev. Lett. 91, 213902 (2003)
Fisher, B. R., Eisler, H.-J., Stott, N. E. & Bawendi, M. G. Emission intensity dependence and single-exponential behavior in single colloidal quantum dot fluorescence lifetimes. J. Phys. Chem. B 108, 143–148 (2004)
Wang, R., Wang, X.-H., Gu, B.-Y. & Yang, G.-Z. Local density of states in three-dimensional photonic crystals: Calculation and enhancement effects. Phys. Rev. B 67, 155114 (2003)
Koenderink, A. F., Bechger, L., Schriemer, H. P., Lagendijk, A. & Vos, W. L. Broadband fivefold reduction of vacuum fluctuations probed by dye in photonic crystals. Phys. Rev. Lett. 88, 143903 (2002)
Li, Z. Y. & Zhang, Z. Q. Weak photonic band gap effect on the fluorescence lifetime in three-dimensional colloidal photonic crystals. Phys. Rev. B 63, 125106 (2001)
Gérard, J. M. et al. Enhanced spontaneous emission by quantum boxes in a monolithic optical microcavity. Phys. Rev. Lett. 81, 1110–1113 (1998)
Bayer, M. et al. Inhibition and enhancement of the spontaneous emission of quantum dots in structured microresonators. Phys. Rev. Lett. 86, 3168–3171 (2001)
Hood, C. J., Chapman, M. S., Lynn, T. W. & Kimble, H. J. Real-time cavity QED with single atoms. Phys. Rev. Lett. 80, 4157–4160 (1998)
Dabbousi, B. O. et al. (CdSe)ZnS core-shell quantum dots: synthesis and characterization of highly luminescent nanocrystallites. J. Phys. Chem. B 101, 9463–9475 (1997)
Crooker, S. A., Hollingsworth, J. A., Tretiak, S. & Klimov, V. I. Spectrally resolved dynamics of energy transfer in quantum-dot assemblies: towards engineered energy flows in artificial materials. Phys. Rev. Lett. 89, 186802 (2002)
Acknowledgements
We thank L. Woldering for sample preparation, F. Koenderink for DOS calculations, A. Mosk and J. Kelly for discussions, and A. Lagendijk for support. This work is part of the research programme of the Stichting voor Fundamenteel Onderzoek der Materie (FOM), which is financially supported by the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO).
Author information
Authors and Affiliations
Corresponding author
Ethics declarations
Competing interests
The authors declare that they have no competing financial interests.
Rights and permissions
About this article
Cite this article
Lodahl, P., Floris van Driel, A., Nikolaev, I. et al. Controlling the dynamics of spontaneous emission from quantum dots by photonic crystals. Nature 430, 654–657 (2004). https://doi.org/10.1038/nature02772
Received:
Accepted:
Issue Date:
DOI: https://doi.org/10.1038/nature02772
This article is cited by
-
Gigantic suppression of recombination rate in 3D lead-halide perovskites for enhanced photodetector performance
Nature Photonics (2023)
-
A review on photonic crystal materials in food detection
European Food Research and Technology (2023)
-
A giant atom with modulated transition frequency
Frontiers of Physics (2023)
-
Photonic graphene with reconfigurable geometric structures in coherent atomic ensembles
Frontiers of Physics (2023)
-
Three-dimensional photonic topological insulator without spin–orbit coupling
Nature Communications (2022)
Comments
By submitting a comment you agree to abide by our Terms and Community Guidelines. If you find something abusive or that does not comply with our terms or guidelines please flag it as inappropriate.