Issue 30, 2014

The enhanced photoelectrochemical performance of CdS quantum dots sensitized TiO2 nanotube/nanowire/nanoparticle arrays hybrid nanostructures

Abstract

This study aims at improving the photoelectrochemical performance mainly from two aspects: the increased number of heterojunctions and the advantages of nanotube/nanowire/nanoparticle arrays hybrid nanostructures. TiO2 nanoparticles porous layer was sensitized by CdS quantum dots (QDs), and coated on the top of the material, hydrogen-treated TiO2 nanotubes with nanowires, which was also sensitized by CdS QDs (This nanostructure is defined as CdS/H:TTWP). CdS/H:TTWP was successfully fabricated by the methods of electrochemical anodization, successive ionic layer adsorption and reaction (SILAR) and sol–gel. The data from the photoelectrochemical (PEC) performance test shows that the photocurrent density of CdS/H:TTWP is 7.6 mA cm−2 at −0.43 V vs. Ag–AgCl under AM 1.5 G illuminations.

Graphical abstract: The enhanced photoelectrochemical performance of CdS quantum dots sensitized TiO2 nanotube/nanowire/nanoparticle arrays hybrid nanostructures

Article information

Article type
Paper
Submitted
17 Jan 2014
Accepted
06 May 2014
First published
07 May 2014

CrystEngComm, 2014,16, 6955-6962

Author version available

The enhanced photoelectrochemical performance of CdS quantum dots sensitized TiO2 nanotube/nanowire/nanoparticle arrays hybrid nanostructures

P. Lv, H. Yang, W. Fu, H. Sun, W. Zhang, M. Li, H. Yao, Y. Chen, Y. Mu, L. Yang, J. Ma, M. Sun, Q. Li and S. Su, CrystEngComm, 2014, 16, 6955 DOI: 10.1039/C4CE00122B

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