Terahertz plasmonic composites

Syrus C. Nemat-Nasser, Alireza V. Amirkhizi, Willie J. Padilla, Dimitri N. Basov, Sia Nemat-Nasser, Derek Bruzewicz, and George Whitesides
Phys. Rev. E 75, 036614 – Published 27 March 2007

Abstract

The dielectric response of a polymer matrix composite can be substantially modified and tuned within a broad frequency band by integrating within the material an artificial plasmon medium composed of periodically distributed, very thin, electrically conducting wires. In the microwave regime, such plasmon/polymer composites have been studied analytically, computationally, and experimentally. This work reports the design, fabrication, and characterization of similar composites for operation at terahertz frequencies. Such composites require significant reduction in the thickness and spacing of the wires. We used numerical modeling to design artificial effective plasmonic media with turn-on frequencies in the terahertz range. Prototype samples were produced by lithographically embedding very thin gold strips into a PDMS [poly(dimethylsiloxane)] matrix. These samples were characterized with a Fourier-transform infrared interferometer using the frequency-dependent transmission and Kramers-Kronig relations to determine the electromagnetic properties. We report the characterization results for a sample, demonstrating excellent agreement between theory, computer design, and experiment. To our knowledge this is the first demonstration of the possibility of creating composites with tuned dielectric response at terahertz frequencies.

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  • Received 27 October 2006

DOI:https://doi.org/10.1103/PhysRevE.75.036614

©2007 American Physical Society

Authors & Affiliations

Syrus C. Nemat-Nasser1,*, Alireza V. Amirkhizi1, Willie J. Padilla2,†, Dimitri N. Basov2, Sia Nemat-Nasser1,‡, Derek Bruzewicz3, and George Whitesides3

  • 1Center of Excellence for Advanced Materials, Department of Mechanical and Aerospace Engineering, University of California, San Diego, Mail code: 0416, 9500 Gilman Drive, La Jolla, California 92093-0416, USA
  • 2Department of Physics, University of California, San Diego, Mail code: 0416, 9500 Gilman Drive, La Jolla, California 92093-0416, USA
  • 3Department of Chemistry and Chemical Biology, Harvard University, Cambridge, Massachusetts 02138, USA

  • *Present address: Fair Isaac Corporation, 3661 Valley Centre Drive, San Diego, CA 92130.
  • Present address: Department of Physics, Boston College, Chestnut Hill, MA 02467.
  • Corresponding author. Electronic address: sia@ucsd.edu

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Issue

Vol. 75, Iss. 3 — March 2007

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