Effective dielectric response of polydispersed composites

Rubén G. Barrera, Pedro Villaseñor-González, W. Luis Mochán, and Guillermo Monsivais
Phys. Rev. B 41, 7370 – Published 15 April 1990
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Abstract

We generalize the concept of renormalized polarizability introduced in a recently developed effective-medium theory to the case of polydispersed composites. We deal with a homogeneous and isotropic ensemble of spherical inclusions with a continuous distribution of sizes. The theory accounts for the correlated fluctuations among the induced dipole moments and the induced internal field within the long-wavelength dipolar approximation. The statistical properties of the ensemble enter in the final result through the two- and three-particle distribution functions. Numerical results are presented for a system of silver spheres in gelatin with a log-normal distribution of radii. The roles played by the dipolar fluctuations and by the size-dependent relaxation time, due to the surface scattering of the electrons, are analyzed and compared.

  • Received 11 December 1989

DOI:https://doi.org/10.1103/PhysRevB.41.7370

©1990 American Physical Society

Authors & Affiliations

Rubén G. Barrera

  • Instituto de Física, Universidad Nacional Autónoma de México, Apartado Postal 20-364, 01000 México, Distrito Federal, Mexico

Pedro Villaseñor-González

  • Instituto de Física, Universidad Autónoma de San Luis Potosí, 78000 San Luis Potosí, San Luis Potosí, Mexico

W. Luis Mochán

  • Laboratorio de Cuernavaca, Instituto de Física, Universidad Nacional Autónoma de México, Aparatado Postal 139-8, 62190 Cuernavaca, Morelos, Mexico

Guillermo Monsivais

  • Instituto de Física, Universidad Nacional Autónoma de México, Apartado Postal 20-364, 01000 México, Distrito Federal, Mexico

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Vol. 41, Iss. 11 — 15 April 1990

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