Compensation of phonon-induced renormalization of vacuum Rabi splitting in large quantum dots: Towards temperature-stable strong coupling in the solid state with quantum dot-micropillars

C. Hopfmann, A. Musiał, M. Strauß, A. M. Barth, M. Glässl, A. Vagov, M. Strauß, C. Schneider, S. Höfling, M. Kamp, V. M. Axt, and S. Reitzenstein
Phys. Rev. B 92, 245403 – Published 3 December 2015

Abstract

We study experimentally the influence of temperature on the emission characteristics of quantum dot-micropillars in the strong coupling regime of cavity quantum electrodynamics (cQED). In particular, we investigate its impact on the vacuum Rabi splitting (VRS) and we address the important question of the temperature stability of the coherent coupling regime in a semiconductor system, which is relevant in view of both fundamental study and future applications. To study the temperature dependence we investigate an unprecedentedly large number of strong coupling cases (89) in a wide temperature range from 10 up to 50 K, which constitutes a good basis for statistical analysis. The experiment indicates a statistically significant increase of the VRS with temperature in contrast to an expected decrease of the VRS due to the dephasing induced by acoustic phonons. From the theoretical point of view, the phonon-induced renormalization of the VRS is calculated using a real-time path-integral approach for strongly confined quantum dots (QDs), which allows for a numerical exact treatment of the coupling between the QD and a continuum of longitudinal acoustic phonons. The absence of the expected decrease of the VRS with temperature in our experimental data can be attributed to a unique optical property of laterally extended In0.4Ga0.6As QDs used in this study. Their electronic structure facilitates an effective temperature-driven increase of the oscillator strength of the excitonic state by up to 40% in the given temperature range. This leads to enhanced light-matter interaction and overcompensates the phonon-related decrease of the VRS. The observed persistence of strong coupling in the presence of phonon-induced decoherence demonstrates the appealing possibility to counteract detrimental phonon effects in the cQED regime via engineering the electronic structure of QDs.

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  • Received 1 September 2015

DOI:https://doi.org/10.1103/PhysRevB.92.245403

©2015 American Physical Society

Authors & Affiliations

C. Hopfmann1, A. Musiał1,2,*, M. Strauß1, A. M. Barth3, M. Glässl3, A. Vagov3, M. Strauß4, C. Schneider4, S. Höfling4,5, M. Kamp4, V. M. Axt3, and S. Reitzenstein1

  • 1Institut für Festkörperphysik, Technische Universität Berlin, Hardenbergstraße 36, 10623 Berlin, Germany
  • 2Laboratory for Optical Spectroscopy of Nanostructures, Department of Experimental Physics, Faculty of Fundamental Problems of Technology, Wrocław University of Technology, Wybrzeże Wyspiańskiego 27, 50-370 Wrocław, Poland
  • 3Institut für Theoretische Physik III, Universität Bayreuth, 95440 Bayreuth, Germany
  • 4Technische Physik, Physikalisches Institut and Wilhelm-Conrad-Röntgen-Research Center for Complex Material Systems, Universität Würzburg, Am Hubland, D-97074 Würzburg, Germany
  • 5SUPA, School of Physics and Astronomy, University of St. Andrews, St. Andrews, KY16 9SS, United Kingdom

  • *anna.musial@physik.tu-berlin.de

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Vol. 92, Iss. 24 — 15 December 2015

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