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Local Jahn-Teller distortion in La1xSrxMnO3 observed by pulsed neutron diffraction

Despina Louca, T. Egami, E. L. Brosha, H. Röder, and A. R. Bishop
Phys. Rev. B 56, R8475(R) – Published 1 October 1997
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Abstract

The atomic pair-density function of La1xSrxMnO3 (0<~x<~0.4) obtained by pulsed neutron diffraction indicates that their local atomic structure significantly deviates from the average structure, and that the local Jahn-Teller (JT) distortion persists even when the crystallographic structure shows no JT distortion. In the paramagnetic insulating phase doped holes form one-site small polarons, represented by the local absence of JT distortion. The polarons become more extended at low temperatures, but local distortions are found even in the metallic phase. The role of polarons in the phase transitions in transport and magnetic properties are discussed.

  • Received 18 July 1997

DOI:https://doi.org/10.1103/PhysRevB.56.R8475

©1997 American Physical Society

Authors & Affiliations

Despina Louca and T. Egami

  • Department of Materials Science and Engineering and Laboratory for Research on the Structure of Matter, University of Pennsylvania, Philadelphia, Pennsylvania 19104

E. L. Brosha, H. Röder, and A. R. Bishop

  • Los Alamos National Laboratory, Los Alamos, New Mexico 87545

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Issue

Vol. 56, Iss. 14 — 1 October 1997

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