Ion-induced damage accumulation and electron-beam-enhanced recrystallization in SrTiO3

Y. Zhang, J. Lian, C. M. Wang, W. Jiang, R. C. Ewing, and W. J. Weber
Phys. Rev. B 72, 094112 – Published 21 September 2005

Abstract

Damage accumulation in strontium titanate (SrTiO3) from 1.0MeV Au irradiation has been investigated at temperatures from 150to400K. The relative disorder on the Sr and Ti sublattices at the damage peak has been determined as a function of local dose and temperature. A disorder accumulation model has been fit to data from this study and from the literature, indicating that defect-stimulated amorphization is the primary amorphization mechanism up to 360K. High-dose irradiation at 400K leads to formation of an amorphous surface layer. Analyses of the temperature dependence for amorphization indicate that the amorphization kinetics are consistent with irradiation-enhanced and thermal recovery processes with activation energies of 0.1±0.05eV and 0.7±0.1eV, respectively. Under 200keV electron-beam irradiation, the epitaxial recrystallization rates are orders of magnitude higher than thermal rates, and an activation energy of 0.1±0.05eV is determined for the e-beam enhanced recrystallization processes.

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  • Received 8 June 2005

DOI:https://doi.org/10.1103/PhysRevB.72.094112

©2005 American Physical Society

Authors & Affiliations

Y. Zhang1,*, J. Lian2, C. M. Wang1, W. Jiang1, R. C. Ewing2, and W. J. Weber1

  • 1Pacific Northwest National Laboratory, P.O. Box 999, Richland, Washington 99352, USA
  • 2Department of Geological Sciences, University of Michigan, Ann Arbor, Michigan 48109, USA

  • *Author to whom correspondence should be addressed. Mailing address: Pacific Northwest National Laboratory, P.O. Box 999/MS K8-93, Richland, Washington 99352. Electronic address: Yanwen.Zhang@pnl.gov

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Vol. 72, Iss. 9 — 1 September 2005

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