Nonlinear Dielectric Response at the Excess Wing of Glass-Forming Liquids

Th. Bauer, P. Lunkenheimer, S. Kastner, and A. Loidl
Phys. Rev. Lett. 110, 107603 – Published 8 March 2013
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Abstract

We present nonlinear dielectric measurements of glass-forming glycerol and propylene carbonate applying electrical fields up to 671kV/cm. The measurements extend to sufficiently high frequencies to allow for the investigation of the nonlinear behavior in the regime of the so-far mysterious excess wing, showing up in the loss spectra of many glass formers as a second power law at high frequencies. Surprisingly, we find a complete lack of nonlinear behavior in the excess wing, in marked contrast to the α relaxation where, in agreement with previous reports, a strong increase of dielectric constant and loss is found.

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  • Received 10 August 2012

DOI:https://doi.org/10.1103/PhysRevLett.110.107603

© 2013 American Physical Society

Authors & Affiliations

Th. Bauer, P. Lunkenheimer*, S. Kastner, and A. Loidl

  • Experimental Physics V, Center for Electronic Correlations and Magnetism, University of Augsburg, 86135 Augsburg, Germany

  • *Corresponding author. Peter.Lunkenheimer@Physik.Uni-Augsburg.de

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Issue

Vol. 110, Iss. 10 — 8 March 2013

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