Abstract
Measurements of photoelectron-photofragment angular correlation and energy partitioning in the dissociative photodetachment of at 532 nm are reported. Using photofragment translational energy and photoelectron spectroscopy in coincidence, vibrationally resolved product translational energy distributions and a pronounced angular correlation between the photoelectron and photofragment recoil directions are observed. These results provide insights into the molecule-fixed photoelectron angular distribution of a negative ion and structural information on in the gas phase.
- Received 10 June 1996
DOI:https://doi.org/10.1103/PhysRevLett.77.3335
©1996 American Physical Society