Causality and Symmetry in Time-Dependent Density-Functional Theory

Robert van Leeuwen
Phys. Rev. Lett. 80, 1280 – Published 9 February 1998
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Abstract

We resolve an existing paradox regarding the causality and symmetry properties of response functions within time-dependent density-functional theory. We do this by defining a new action functional within the Keldysh formalism. By functional differentiation the new functional leads to response functions which are symmetric in the Keldysh time contour parameter, but which become causal when a transition to physical time is made. The new functional is further used to derive the equations of the time-dependent optimized potential method.

  • Received 8 September 1997

DOI:https://doi.org/10.1103/PhysRevLett.80.1280

©1998 American Physical Society

Authors & Affiliations

Robert van Leeuwen

  • Department of Theoretical Physics, University of Lund, Sölvegatan 14A, S-22362 Lund, Sweden

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Vol. 80, Iss. 6 — 9 February 1998

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