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Radiation effects in crystalline ceramics for the immobilization of high-level nuclear waste and plutonium

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Abstract

This review provides a comprehensive evaluation of the state-of-knowledge of radiation effects in crystalline ceramics that may be used for the immobilization of high-level nuclear waste and plutonium. The current understanding of radiation damage processes, defect generation, microstructure development, theoretical methods, and experimental methods are reviewed. Fundamental scientific and technological issues that offer opportunities for research are identified. The most important issue is the need for an understanding of the radiation-induced structural changes at the atomic, microscopic, and macroscopic levels, and the effect of these changes on the release rates of radionuclides during corrosion.

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Authors and Affiliations

  1. Pacific Northwest National Laboratory, P.O. Box 999, M.S. K2–44, 99352, Richland, Washington, USA

    W. J. Weber

  2. Nuclear Engineering and Radiological Sciences, The University of Michigan, 48109, Ann Arbor, Michigan, USA

    R. C. Ewing

  3. The Royal Institution, 21 Albemarle Street, W1X 4BS, London, UK

    C. R. A. Catlow

  4. Lawrence Livermore National Laboratory, P.O. Box 808, 94550, Livermore, California, USA

    T. Diaz de la Rubia

  5. Department of Materials Science and Engineering, Massachusetts Institute of Technology, 02139, Cambridge, Massachusetts, USA

    L. W. Hobbs

  6. Department of Nuclear Engineering, Kyushu University, 812, Fukoka, Japan

    C. Kinoshita

  7. European Commission, Joint Research Center, Institute for Transuranium Elements, Postfach 2340, 76125, Karlsruhe, Germany

    Hj. Matzke

  8. Department of Nuclear Engineering, Pennsylvania State University, 16802, University Park, Pennsylvania, USA

    A. T. Motta

  9. Los Alamos National Laboratory, P.O. Box 1663, 87545, Los Alamos, Mexico

    M. Nastasi

  10. Department of Earth Sciences, University of Cambridge, CB2 3EQ, Cambridge, UK

    E. K. H. Salje

  11. Materials Division, ANSTO, 2234, Menai, NSW, Australia

    E. R. Vance

  12. Oak Ridge National Laboratory, P.O. Box 2008, 37831, Oak Ridge, Tennessee, USA

    S. J. Zinkle

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Weber, W.J., Ewing, R.C., Catlow, C.R.A. et al. Radiation effects in crystalline ceramics for the immobilization of high-level nuclear waste and plutonium. Journal of Materials Research 13, 1434–1484 (1998). https://doi.org/10.1557/JMR.1998.0205

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