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Journal of Materials Science
Erschienen in: Journal of Materials Science 24/2018

27.08.2018 | Chemical routes to materials

Low-temperature synthesis of manganese oxide–carbon nanotube-enhanced microwave-absorbing nanocomposites

verfasst von: Huifang Pang, Ahmed M. Abdalla, Rakesh P. Sahu, Yuping Duan, Ishwar K. Puri

Erschienen in: Journal of Materials Science | Ausgabe 24/2018

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Abstract

Noting that the dielectric properties of manganese oxide make it a promising microwave-absorbing material, a low-temperature method to deposit crystalline MnO2 over carbon nanotubes (CNTs) is developed. Adjusting the pH of the precursor solution allows control over the phases and morphologies of the synthesized manganese oxides MnO2 and Mn3O4 that have minimum reflection losses of − 11 dB and − 6 dB, respectively. The synthesized CNT–MnO2 and CNT–Mn3O4 nanocomposites are superior microwave absorbers than simpler physical mixtures of CNTs and manganese oxides, with reflection losses as high as − 19 dB at 9.5 GHz and − 34 dB at 4 GHz, and have wider absorption bands than pure manganese oxides. Coating CNTs with manganese oxide not only increases dielectric and magnetic losses, but also improves the impedance match between free space and the absorber. The addition of CNTs to pure MnO2 and Mn3O4 improves impedance matching by enhancing the relaxation polarization and conductivity losses, magnetic loss, including contributions form eddy current and natural resonance. This facile, low-cost, scalable, high-yield method produces an enhanced microwave-absorbing nanocomposite.
Vorheriger Artikel Ultrafast room-temperature synthesis of hierarchically porous metal–organic frameworks by a versatile cooperative template strategy
Nächster Artikel One-pot strategy for covalent construction of POSS-modified silane layer on carbon fiber to enhance interfacial properties and anti-hydrothermal aging behaviors of PPBES composites

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Metadaten
Titel
Low-temperature synthesis of manganese oxide–carbon nanotube-enhanced microwave-absorbing nanocomposites
verfasst von
Huifang Pang
Ahmed M. Abdalla
Rakesh P. Sahu
Yuping Duan
Ishwar K. Puri
Publikationsdatum
27.08.2018
Verlag
Springer US
Erschienen in
Journal of Materials Science / Ausgabe 24/2018
Print ISSN: 0022-2461
Elektronische ISSN: 1573-4803
DOI
https://doi.org/10.1007/s10853-018-2807-1

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