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Journal of Materials Science: Materials in Electronics
Erschienen in: Journal of Materials Science: Materials in Electronics 19/2020

14.08.2020

Reinforced supercapacitive behavior of O3-type layer-structured Na3Ni2BiO6 in 1-butyl-3-methylimidazolium tetrafluoroborate (BMIMBF4) electrolyte

verfasst von: Alfred Bekoe Appiagyei, Jeong In Han

Erschienen in: Journal of Materials Science: Materials in Electronics | Ausgabe 19/2020

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Abstract

Sodium-ion-based energy storage devices in which the electrochemical properties are influenced by excess Na ions are very important as an alternative energy storage system. In this study, O3-type multi-metal-oxide layers of Na3Ni2BiO6 were synthesized via a simple solid-state method. Their electrochemical properties were examined while employing them as a supercapacitor electrode material with four different electrolytes: H2SO4, Na2SO4, KOH, and 1-butyl-3-methylimidazolium tetrafluoroborate (BMIMBF4). Among these, BMIMBF4 ionic liquid electrolyte in a symmetric Na3Ni2BiO6 supercapacitor demonstrated the highest specific capacitance performance of 780.49 F g−1 at 0.5 A g−1 with 95.2% capacitance retention after 10,000 cycles. Moreover, a maximum energy density of 67.16 Wh·kg−1 was recorded at 349.87 W·kg−1. The enhanced electrochemical performance is a result of the reinforced fast intercalation/deintercalation of Na+ ions in the Na3Ni2BiO6 crystal structure due to high solvation and association mechanism of Na3Ni2BiO6 in BMIMBF4 ionic liquid media. These results indicate that the developed Na3Ni2BiO6-based supercapacitor with BMIMBF4 ionic liquid electrolyte could be used in the high-performance energy storage devices for smart electrical and electronic units.
Vorheriger Artikel Spectroscopic, optical, magnetic and dielectric investigation of the orthoborate Ba2Co(BO3)2 nanopowder
Nächster Artikel Cost-effective synthesis of NiCo2O4@nitrogen-doped carbon nanocomposite using waste PET plastics for high-performance supercapacitor

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Metadaten
Titel
Reinforced supercapacitive behavior of O3-type layer-structured Na3Ni2BiO6 in 1-butyl-3-methylimidazolium tetrafluoroborate (BMIMBF4) electrolyte
verfasst von
Alfred Bekoe Appiagyei
Jeong In Han
Publikationsdatum
14.08.2020
Verlag
Springer US
Erschienen in
Journal of Materials Science: Materials in Electronics / Ausgabe 19/2020
Print ISSN: 0957-4522
Elektronische ISSN: 1573-482X
DOI
https://doi.org/10.1007/s10854-020-04223-8

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