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Erschienen in: Journal of Materials Science: Materials in Electronics 11/2016

22.07.2016

Structural evolution, relaxation behaviors and dielectric properties of BaTiO3–BiAlO3 perovskite solid solutions

verfasst von: Yaru Wang, Yongping Pu, Xin Li, Hanyu Zheng

Erschienen in: Journal of Materials Science: Materials in Electronics | Ausgabe 11/2016

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Abstract

The polycrystalline (1 − x)BaTiO3xBiAlO3 ((1 − x)BT–xBA) (x = 0–0.15) ceramics are fabricated via a conventional solid state reaction method. X-ray diffraction and Raman results show a structural evolution from a tetragonal phase to a cubic one with increasing x. Dielectric studies exhibit a diffuse phase transition characterized by a strong temperature and frequency dispersion of permittivity. The dielectric maxima temperature T m decrease, due to the strong interaction of Bi3+ and Al3+ with Ba2+ and Ti4+. (1 − x)BT–xBA ceramics underwent a ferroelectric to relaxor transition at x = 0.06. Activation energy with dozens meV is obtained using the Vogel-Fulcher relationship, which is attributed to thermally activated off-center ion hopping. Raman spectra of the (1 − x)BT–xBA ceramics at 264 cm−1, the paraelectric and cubic phase exist in the ceramics, so the polarization-electric plots are in the form of narrow ellipsoids with the elevation of x. Meanwhile, the discharged energy density of 0.85BT–0.15BA is 0.16 J/cm3.

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Metadaten
Titel
Structural evolution, relaxation behaviors and dielectric properties of BaTiO3–BiAlO3 perovskite solid solutions
verfasst von
Yaru Wang
Yongping Pu
Xin Li
Hanyu Zheng
Publikationsdatum
22.07.2016
Verlag
Springer US
Erschienen in
Journal of Materials Science: Materials in Electronics / Ausgabe 11/2016
Print ISSN: 0957-4522
Elektronische ISSN: 1573-482X
DOI
https://doi.org/10.1007/s10854-016-5287-6

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