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Journal of Materials Science

Erschienen in:

17.06.2021 | Chemical routes to materials

Tetraphenylporphyrin-modified perovskite nanocrystals enable ratiometric fluorescent determination of sulfide ion in water samples

verfasst von: Hongbo Wang, Qian Li, Xiaomeng Niu, Jianxiu Du

Erschienen in: Journal of Materials Science | Ausgabe 27/2021

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Abstract

A simple and feasible approach was constructed for preparation of all inorganic cesium lead bromide perovskite nanocrystals (CsPbBr₃ NCs) modified with tetraphenylporphyrin tetrasulfonic acid (TPPS). The CsPbBr₃/TPPS nanocomposite has good water stability and exhibits a dual-emission property. Adopting the CsPbBr₃/TPPS nanocomposite as a nanoprobe, a rapid, selective and sensitive ratiometric fluorescent method was developed for determination of sulfide ion. When sulfide ion was added into the CsPbBr₃/TPPS nanocomposite, the bright green fluorescence of CsPbBr₃ NCs at 520 nm was sharply quenched, whereas the red fluorescence of TPPS at 650 nm was hardly influenced. The quenching is possibly attributed to destruction of CsPbBr₃ NCs via the formation of more stable PbS. This nanoprobe can determine sulfide ion over the range of 0.2–15.0 nmol·L⁻¹ with a detection limit as low as 0.05 nmol·L⁻¹. The relative standard deviation is 3.3% at 10.0 nmol·L⁻¹ concentration level (n = 11). Sulfide ion content was successfully determined in different water samples by this nanoprobe.

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Vorheriger Artikel Promotion effect of rare earth elements (Ce, Nd, Pr) on physicochemical properties of M-Al mixed oxides (M = Cu, Ni, Co) and their catalytic activity in N2O decomposition

Nächster Artikel Self-lubricating triboactive (Cr,Al)N+Mo:S coatings for fluid-free applications

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Titel: Tetraphenylporphyrin-modified perovskite nanocrystals enable ratiometric fluorescent determination of sulfide ion in water samples
verfasst von: Hongbo Wang
Qian Li
Xiaomeng Niu
Jianxiu Du
Publikationsdatum: 17.06.2021
Verlag: Springer US
Erschienen in: Journal of Materials Science / Ausgabe 27/2021
Print ISSN: 0022-2461
Elektronische ISSN: 1573-4803
DOI: https://doi.org/10.1007/s10853-021-06253-x

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