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22.04.2020 | Composites & nanocomposites

Vertically aligned dopamine-reduced graphene oxide with high thermal conductivity for epoxy nanocomposites

verfasst von: Yingchun Liu, Kun Wu, Maoping Lu, Shibin Nie, Weilong Chen, Enxiang Jiao, Bingfei Nan, Liyan Liang, Mangeng Lu

Erschienen in: Journal of Materials Science | Ausgabe 21/2020

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Abstract

Designing ordered fillers arrangement and superior interfacial adhesion between fillers and matrix can improve the thermal conductivity (TC) of composites. Here, bioinspired dopamine chemistry was firstly used to reduce graphene oxide (GO) and introduce polydopamine nanoparticles on the surface of GO. Then, a well-aligned epoxy/reduced GO films (EP/RGFs) nanocomposites were prepared via the simple vacuum impregnation. Compared with the random distribution of fillers in a traditional blending composite, fillers were selectively distributed in matrix and continuous thermal conductive network structures were constructed in this strategy. As a result, the nanocomposite exhibited a high TC of 0.913 W m⁻¹ K⁻¹ which is 4.8 times higher than pure EP. In addition, curing kinetics showed that RGFs were similar to an amine-type curing agent that reacted with EP and bonded them tightly, and its nanocomposites reaction activation energy is lower than that of pure EP. These results indicated RGFs possessed excellent interface compatibility with EP and suppressing effectively the phonon scattering at the EP–RGFs interface. Cooling experiments showed that nanocomposites can reduce by about 10 °C for a hot source (80 °C), demonstrating it can transfer efficiently heat energy from the heat source. This study provides an effective method for the preparation of high-performance thermal management composites.

Vorheriger Artikel Effect of water on the breakdown and dielectric response of polypropylene/nano-aluminium nitride composites

Nächster Artikel Global and local conductivity in percolating crosslinked carbon black/epoxy–amine composites

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Titel: Vertically aligned dopamine-reduced graphene oxide with high thermal conductivity for epoxy nanocomposites
verfasst von: Yingchun Liu
Kun Wu
Maoping Lu
Shibin Nie
Weilong Chen
Enxiang Jiao
Bingfei Nan
Liyan Liang
Mangeng Lu
Publikationsdatum: 22.04.2020
Verlag: Springer US
Erschienen in: Journal of Materials Science / Ausgabe 21/2020
Print ISSN: 0022-2461
Elektronische ISSN: 1573-4803
DOI: https://doi.org/10.1007/s10853-020-04639-x

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