Comptes Rendus
no. 3-4
Displacement damage and transmutations in metals under neutron and proton irradiation
[Dommage de déplacements et transmutations dans les métaux sous irradiation de neutrons et de protons]
Pavel Vladimirov1  ; Serge Bouffard2
1 FZK, Institute of Materials Research I, P.O. Box 3640, 76021 Karlsruhe, Germany
2 CEA/DRECAM, Centre interdisciplinaire de recherche ions lasers (CIRIL), BP 5133, 14070 Caen cedex 5, France
Comptes Rendus. Physique, Volume 9 (2008) no. 3-4, pp. 303-322.

Connaître le taux de génération de défauts et d'impuretés ainsi que la distribution spatiale des défauts est la base de la compréhension de l'évolution des propriétés des matériaux sous irradiation. Cette compréhension est aussi essentielle à une définition exhaustive des simulations expérimentales du comportement des matériaux sous irradiation.

Dans ce papier on discute l'interaction des neutrons et des protons avec les métaux, et, la production de dommage de déplacements qui en résultent. On illustre aussi brièvement les irradiations par particules chargées. Après avoir discuté l'interaction initiale de la particule incidente (neutrons, particules chargées en général, et, plus particulièrement protons) avec les atomes et les noyaux cibles, nous décrivons l'interaction de l'atome de recul avec les autres atomes, qui a pour conséquence le ralentissement du projectile, la création de dommage par déplacements, la production d'impuretés par réactions nucléaires et la création de cascades de déplacements atomiques. On discute alors l'évolution ultérieure de la structure des défauts. La section suivante dévolue à la formation de cascades comprend deux parties. On présente d'abord les évidences expérimentales de formation de sous-cascades provoquées par l'irradiation de neutrons et de particules chargées, puis, les modèles de formation de sous-cascades. Finalement nous analysons les modèles de calculs de dommage de déplacements et nous montrons comment ces modèles peuvent être appliqués au calcul du dommage de déplacements sous irradiation de neutrons. L'application de ces méthodes au cas réel de plusieurs installations nucléaires est finalement présentée.

The knowledge of the defect and impurity generation rates, as well as the defect spatial distribution, is the corner stone for the understanding of the evolution of material properties under irradiation. This knowledge is also an essential element for comprehensive experimental simulations of the behavior of irradiated materials.

In this article the interaction of neutron and proton irradiation with metals is discussed with respect to displacement damage production. Charged particle irradiation is also briefly illustrated. After discussion of the primary interaction of projectiles (neutrons, charged particles in general, and protons in particular) with target atoms/nuclei, we describe the interaction of a recoil atom with other target atoms resulting in the slowing down of the projectile, displacement damage, impurity atom production due to nuclear reactions, and the creation of atomic displacement cascades. Then the further evolution of defect structure is discussed. The next section, devoted to subcascade formation, is divided into two parts. The first experimental evidence of subcascade formation under neutron and charged particle irradiation is presented. Then the models of subcascade formation are described. Finally we review the models for the calculation of displacement damage and show how these models can be applied to displacement damage calculation under neutron irradiation with a demonstration of a real application of the methods discussed to several nuclear facilities.

Publié le :
DOI : 10.1016/j.crhy.2008.02.004
Keywords: Neutron irradiation, Displacement damage, Atomic collision cascades
Mot clés : Irradiation de neutrons, Dommage de déplacements, Cascades de collisions atomiques
Pavel Vladimirov 1 ; Serge Bouffard 2

1 FZK, Institute of Materials Research I, P.O. Box 3640, 76021 Karlsruhe, Germany
2 CEA/DRECAM, Centre interdisciplinaire de recherche ions lasers (CIRIL), BP 5133, 14070 Caen cedex 5, France 
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Pavel Vladimirov; Serge Bouffard. Displacement damage and transmutations in metals under neutron and proton irradiation. Comptes Rendus. Physique, Volume 9 (2008) no. 3-4, pp. 303-322. doi : 10.1016/j.crhy.2008.02.004. https://comptes-rendus.academie-sciences.fr/physique/articles/10.1016/j.crhy.2008.02.004/

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