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Erschienen in:
Modelling of Photo-Fenton Solar Reactors for Environmental Applications Kapitel lesen Erstes Kapitel lesen

2015 | OriginalPaper | Buchkapitel

Photocatalytic Splitting of Water

verfasst von : Nathan Skillen, Cathy McCullagh, Morgan Adams

Erschienen in: Environmental Photochemistry Part III

Verlag: Springer Berlin Heidelberg

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Abstract

The use of photocatalysis for the photosplitting of water to generate hydrogen and oxygen has gained interest as a method for the conversion and storage of solar energy. The application of photocatalysis through catalyst engineering, mechanistic studies and photoreactor development has highlighted the potential of this technology, with the number of publications significantly increasing in the past few decades. In 1972 Fujishima and Honda described a photoelectrochemical system capable of generating H2 and O2 using thin-film TiO2. Since this publication, a diverse range of catalysts and platforms have been deployed, along with a varying range of photoreactors coupled with photoelectrochemical and photovoltaic technology. This chapter aims to provide a comprehensive overview of photocatalytic technology applied to overall H2O splitting. An insight into the electronic and geometric structure of catalysts is given based upon the one- and two-step photocatalyst systems. One-step photocatalysts are discussed based upon their d0 and d10 electron configuration and core metal ion including transition metal oxides, typical metal oxides and metal nitrides. The two-step approach, referred to as the Z-scheme, is discussed as an alternative approach to the traditional one-step mechanism, and the potential of the system to utilise visible and solar irradiation. In addition to this the mechanistic procedure of H2O splitting is reviewed to provide the reader with a detailed understanding of the process. Finally, the development of photoreactors and reactor properties are discussed with a view towards the photoelectrochemical splitting of H2O.

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Vorheriges Kapitel Surface-Modified Photocatalysts
Nächstes Kapitel Nonmetal Doping in TiO2 Toward Visible-Light-Induced Photocatalysis
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Metadaten
Titel
Photocatalytic Splitting of Water
verfasst von
Nathan Skillen
Cathy McCullagh
Morgan Adams
Copyright-Jahr
2015
Verlag
Springer Berlin Heidelberg
Buch
Environmental Photochemistry Part III

Print ISBN: 978-3-662-46794-7

Electronic ISBN: 978-3-662-46795-4

Copyright-Jahr: 2015

DOI
https://doi.org/10.1007/698_2014_261