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Published in:
Future Air Pollution in Europe from a Multi-physics Ensemble of Climate Change-Air Quality Projections Read chapter Read first chapter

2014 | OriginalPaper | Chapter

88. Assessing Sensitivity Regimes of Secondary Inorganic Aerosol Formation in Europe with the CALIOPE-EU Modelling System

Authors : María Teresa Pay, Pedro Jiménez-Guerrero, José María Baldasano

Published in: Air Pollution Modeling and its Application XXII

Publisher: Springer Netherlands

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Abstract

Sulphur dioxide (SO2) and nitrogen oxides (NOx) form two of the largest contributors to PM2.5 in Europe: ammonium sulphate, (NH4)2SO4, and ammonium nitrate, NH4NO3. Understanding the formation regimes for these components is important for the achievement of the reduction objectives established in the European legislation for PM2.5. The present work uses the CALIOPE air quality forecasting system to investigate the formation of secondary inorganic aerosols (SIAs) and their gaseous precursors over Europe. Results points out that the continental regions in Europe tend to be HNO3 − limited for nitrate formation. Regulatory strategies in such regions should focus on reductions in NOx rather than NH3 to control NH4NO3.

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previous chapter Development and Evaluation of an Air Quality Model for Predicting the Impacts of Prescribed Burns
next chapter Effect of the Turbulence Parameterizations on the Simulation of Pollutant Dispersion with the RMS Modelling System
Literature
1.
Pay MT, Piot M, Jorba O, Basart S, Gassó S, Jiménez-Guerrero P, Gonçalves M, Dabdub D, Baldasano JM (2010) A full year evaluation of the CALIOPE-EU air quality system in Europe for 2004: a model study. Atmos Environ 44:3322–3342CrossRef
2.
Baldasano JM, Pay MT, Jorba O, Gassó S, Jiménez-Guerrero P (2011) An annual assessment of air quality with the CALIOPE modeling system over Spain. Sci Total Environ 409:2163–2178CrossRef
3.
Hass H, van Loon M, Kessler et al (2003) Aerosol modeling: results and intercomparison from European regional scale modeling system. Technical report. EUROTRAC 2 Report, EUREKA Environmental Project, GLOREAM
4.
Ansari AS, Pandis S (1998) Response of inorganic PM to precursor concentrations. Environ Sci Technol 32:2706–2714CrossRef
Metadata
Title
Assessing Sensitivity Regimes of Secondary Inorganic Aerosol Formation in Europe with the CALIOPE-EU Modelling System
Authors
María Teresa Pay
Pedro Jiménez-Guerrero
José María Baldasano
Copyright Year
2014
Publisher
Springer Netherlands
Book
Air Pollution Modeling and its Application XXII

Print ISBN: 978-94-007-5576-5

Electronic ISBN: 978-94-007-5577-2

Copyright Year: 2014

DOI
https://doi.org/10.1007/978-94-007-5577-2_88