Skip to main content
Disciplines
Automotive Business IT + Informatics Construction + Real Estate Electrical Engineering + Electronics Energy + Sustainability Insurance + Risk Finance + Banking Management + Leadership Marketing + Sales Mechanical Engineering + Materials
Events
DE
EN
Books
Journals
Topic Page
Marketing
Start single access now
Access for companies
EXTENDED SEARCH
Log in
Top
Topics in Catalysis
Published in: Topics in Catalysis 5-7/2016

29-12-2015 | Original Paper

Hydrogen Intercalation of Graphene and Boron Nitride Monolayers Grown on Pt(111)

Authors: Mingming Wei, Qiang Fu, Hao Wu, Aiyi Dong, Xinhe Bao

Published in: Topics in Catalysis | Issue 5-7/2016

Log in

Activate our intelligent search to find suitable subject content or patents.

search-config
loading …

Abstract

H2 atmosphere is often involved in growth and application of two-dimensional (2D) atomic crystals, and it is of great importance to understand interaction of the 2D materials with H2 molecules. Here, a full graphene layer and a full hexagonal boron nitride (h-BN) layer grown on Pt(111) were exposed to H2 atmosphere, which were investigated by in situ near ambient pressure X-ray photoelectron spectroscopy and quasi in situ ultraviolet photoelectron spectroscopy. We confirm the occurrence of hydrogen intercalation of the graphene and h-BN overlayers in ambient pressure H2. The hydrogen intercalation in 0.1 Torr H2 at room temperature and hydrogen desorption in 0.1 Torr H2 at 200 °C are fully reversible on the graphene/Pt(111) and h-BN/Pt(111) surfaces. Furthermore, hydrogen desorption on the graphene/Pt(111) and h-BN/Pt(111) surfaces was found to happen at lower temperature than that on the Pt(111) surface due to the graphene and h-BN cover effect.
previous article A Comparative Ambient Pressure X-ray Photoelectron and Absorption Spectroscopy Study of Various Cobalt-Based Catalysts in Reactive Atmospheres
next article Oxidation of Small Supported Platinum-based Nanoparticles Under Near-Ambient Pressure Exposure to Oxygen

Dont have a licence yet? Then find out more about our products and how to get one now:

Springer Professional "Wirtschaft+Technik"

Online-Abonnement

Mit Springer Professional "Wirtschaft+Technik" erhalten Sie Zugriff auf:

  • über 102.000 Bücher
  • über 537 Zeitschriften

aus folgenden Fachgebieten:

  • Automobil + Motoren
  • Bauwesen + Immobilien
  • Business IT + Informatik
  • Elektrotechnik + Elektronik
  • Energie + Nachhaltigkeit
  • Finance + Banking
  • Management + Führung
  • Marketing + Vertrieb
  • Maschinenbau + Werkstoffe
  • Versicherung + Risiko

Jetzt Wissensvorsprung sichern!

inform now

Springer Professional "Technik"

Online-Abonnement

Mit Springer Professional "Technik" erhalten Sie Zugriff auf:

  • über 67.000 Bücher
  • über 390 Zeitschriften

aus folgenden Fachgebieten:

  • Automobil + Motoren
  • Bauwesen + Immobilien
  • Business IT + Informatik
  • Elektrotechnik + Elektronik
  • Energie + Nachhaltigkeit
  • Maschinenbau + Werkstoffe




 

Jetzt Wissensvorsprung sichern!

inform now
Literature
1.
Prasai D, Tuberquia JC, Harl RR, Jennings GK, Bolotin KI (2012) ACS Nano 6:1102CrossRef
2.
Chen SS, Brown L, Levendorf M, Cai WW, Ju SY, Edgeworth J, Li XS, Magnuson CW, Velamakanni A, Piner RD, Kang JY, Park J, Ruoff RS (2011) ACS Nano 5:1321CrossRef
3.
Kang D, Kwon JY, Cho H, Sim JH, Hwang HS, Kim CS, Kim YJ, Ruoff RS, Shin HS (2012) ACS Nano 6:7763CrossRef
4.
Raman RKS, Banerjee PC, Lobo DE, Gullapalli H, Sumandasa M, Kumar A, Choudhary L, Tkacz R, Ajayan PM, Majumder M (2012) Carbon 50:4040CrossRef
5.
6.
7.
Yao YX, Fu Q, Zhang YY, Weng XF, Li H, Chen MS, Jin L, Dong AY, Mu RT, Jiang P, Liu L, Bluhm H, Liu Z, Zhang SB, Bao XH (2014) Proc Natl Acad Sci USA 111:17023CrossRef
8.
9.
Dong AY, Fu Q, Wei MM, Liu Y, Ning YX, Yang F, Bluhm H, Bao XH (2015) Surf Sci 634:37CrossRef
10.
11.
Grånäs E, Knudsen J, Schröder UA, Gerber T, Busse C, Arman MA, Schulte K, Andersen JN, Michely T (2012) ACS Nano 6:9951CrossRef
12.
Grånäs E, Andersen M, Arman MA, Gerber T, Hammer B, Schnadt J, Andersen JN, Michely T, Knudsen J (2013) J Phys Chem C 117:16438CrossRef
13.
Mu RT, Fu Q, Jin L, Yu L, Fang GZ, Tan DL, Bao XH (2012) Angew Chem Int Ed 51:4856CrossRef
14.
Jin L, Fu Q, Dong AY, Ning YX, Wang ZJ, Bluhm H, Bao XH (2014) J Phys Chem C 118:12391CrossRef
15.
16.
Ng ML, Shavorskiy A, Rameshan C, Mikkelsen A, Lundgren E, Preobrajenski A, Bluhm H (2015) ChemPhysChem 16:923CrossRef
17.
Lizzit S, Larciprete R, Lacovig P, Dalmiglio M, Orlando F, Baraldi A, Gammelgaard L, Barreto L, Bianchi M, Perkins E, Hofmann P (2012) Nano Lett 12:4503CrossRef
18.
Larciprete R, Ulstrup S, Lacovig P, Dalmiglio M, Bianchi M, Mazzola F, Hornekær L, Orlando F, Baraldi A, Hofmann P, Lizzit S (2012) ACS Nano 6:9551CrossRef
19.
Zhang YH, Weng XF, Li H, Li HB, Wei MM, Xiao JP, Liu Z, Chen MS, Fu Q, Bao XH (2015) Nano Lett 15:3616CrossRef
20.
Blume R, Kidambi PR, Bayer BC, Weatherup RS, Wang ZJ, Weinberg G, Willinger MG, Greiner M, Hofmann S, Knop-Gericke A, Schlögl R (2014) Phys Chem Chem Phys 16:25989CrossRef
21.
Zhao W, Gebhardt J, Späth F, Gotterbarm K, Gleichweit C, Steinrück HP, Görling A, Papp C (2015) Chem Eur J 21:3347CrossRef
22.
Hornekær L, Šljivančanin Ž, Xu W, Otero R, Rauls E, Stensgaard I, Lægsgaard E, Hammer B, Besenbacher F (2006) Phys Rev Lett 96:156104CrossRef
23.
24.
Elias DC, Nair RR, Mohiuddin TMG, Morozov SV, Blake P, Halsall MP, Ferrari AC, Boukhvalov DW, Katsnelson MI, Geim AK, Novoselov KS (2009) Science 323:610CrossRef
25.
26.
Koswattage KR, Shimoyama I, Baba Y, Sekiguchi T, Nakagawa K (2011) J Chem Phys 135:014706CrossRef
27.
Ng ML, Balog R, Hornekær L, Preobrajenski AB, Vinogradov NA, Mårtensson N, Schulte K (2010) J Phys Chem C 114:18559CrossRef
28.
Balog R, Jørgensen B, Nilsson L, Andersen M, Rienks E, Bianchi M, Fanetti M, Lægsgaard E, Baraldi A, Lizzit S, Sljivancanin Z, Besenbacher F, Hammer B, Pedersen TG, Hofmann P, Hornekær L (2010) Nat Mater 9:315CrossRef
29.
Riedl C, Coletti C, Iwasaki T, Zakharov AA, Starke U (2009) Phys Rev Lett 103:246804CrossRef
30.
Brugger T, Ma HF, Iannuzzi M, Berner S, Winkler A, Hutter J, Osterwalder J, Greber T (2010) Angew Chem Int Ed 49:6120CrossRef
31.
Balog R, Andersen M, Jørgensen B, Sljivancanin Z, Hammer B, Baraldi A, Larciprete R, Hofmann P, Hornekær L, Lizzit S (2013) ACS Nano 7:3823CrossRef
32.
Starr DE, Liu Z, Hävecker M, Knop-Gericke A, Bluhm H (2013) Chem Soc Rev 42:5833CrossRef
33.
Ogletree DF, Bluhm H, Hebenstreit ED, Salmeron M (2009) Nucl Instrum Methods Phys Res Sect A 601:151CrossRef
34.
35.
36.
Preobrajenski AB, Vinogradov AS, Ng ML, Ćavar E, Westerström R, Mikkelsen A, Lundgren E, Mårtensson N (2007) Phys Rev B 75:245412CrossRef
37.
Ćavar E, Westerström R, Mikkelsen A, Lundgren E, Vinogradov AS, Ng ML, Preobrajenski AB, Zakharov AA, Mårtensson N (2008) Surf Sci 602:1722CrossRef
38.
Gao M, Pan Y, Huang L, Hu H, Zhang LZ, Guo HM, Du SX, Gao HJ (2011) Appl Phys Lett 98:033101CrossRef
39.
Otero G, González C, Pinardi AL, Merino P, Gardonio S, Lizzit S, Blanco-Rey M, Van de Ruit K, Flipse CFJ, Méndez J, de Andrés PL, Martín-Gago JA (2010) Phys Rev Lett 105:216102CrossRef
40.
Tao F, Dag S, Wang LW, Liu Z, Butcher DR, Bluhm H, Salmeron M, Somorjai GA (2010) Science 327:850CrossRef
41.
Ogasawara H, Brena B, Nordlund D, Nyberg M, Pelmenschikov A, Pettersson LGM, Nilsson A (2002) Phys Rev Lett 89:276102CrossRef
42.
43.
Koeleman BJJ, Dezwart ST, Boers AL, Poelsema B, Verheij LK (1986) Phys Rev Lett 56:1152CrossRef
44.
45.
46.
47.
Zhu JF, Kinne M, Fuhrmann T, Denecke R, Steinrück HP (2003) Surf Sci 529:384CrossRef
48.
Zhu ZW, Tao F, Zheng F, Chang R, Li YM, Heinke L, Liu Z, Salmeron M, Somorjai GA (2012) Nano Lett 12:1491CrossRef
49.
Preobrajenski AB, Nesterov MA, Ng ML, Vinogradov AS, Mårtensson N (2007) Chem Phys Lett 446:119CrossRef
50.
Preobrajenski AB, Ng ML, Vinogradov AS, Mårtensson N (2008) Phys Rev B 78:073401CrossRef
51.
Rajasekaran S, Kaya S, Abild-Pedersen F, Anniyev T, Yang F, Stacchiola D, Ogasawara H, Nilsson A (2012) Phys Rev B 86:075417CrossRef
52.
Nagashima A, Tejima N, Gamou Y, Kawai T, Oshima C (1995) Phys Rev B 51:4606CrossRef
Metadata
Title
Hydrogen Intercalation of Graphene and Boron Nitride Monolayers Grown on Pt(111)
Authors
Mingming Wei
Qiang Fu
Hao Wu
Aiyi Dong
Xinhe Bao
Publication date
29-12-2015
Publisher
Springer US
Published in
Topics in Catalysis / Issue 5-7/2016
Print ISSN: 1022-5528
Electronic ISSN: 1572-9028
DOI
https://doi.org/10.1007/s11244-015-0516-4

Other articles of this Issue 5-7/2016

Topics in Catalysis 5-7/2016 Go to the issue

Original Paper

Real-Time Observation of Reaction Processes of CO2 on Cu(997) by Ambient-Pressure X-ray Photoelectron Spectroscopy

Original Paper

Comparison of AP-XPS and PLIF Measurements During CO Oxidation Over Pd Single Crystals

Original Paper

Recent Approaches for Bridging the Pressure Gap in Photoelectron Microspectroscopy

Original Paper

Oxidation of Ultrathin FeO(111) Grown on Pt(111): Spectroscopic Evidence for Hydroxylation

Original Paper

Are Au Nanoparticles on Oxygen-Free Supports Catalytically Active?

Original Paper

In-Situ Probing of H2O Effects on a Ru-Complex Adsorbed on TiO2 Using Ambient Pressure Photoelectron Spectroscopy

Premium Partners

    Image Credits