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Topics in Catalysis
Published in: Topics in Catalysis 1-4/2019

07-01-2019 | Original Paper

NOx Adsorption Over Ce/Zr-Based Catalysts Doped with Cu and Ba

Authors: J. Giménez-Mañogil, J. C. Martínez-Munuera, R. Matarrese, L. Castoldi, L. Lietti, A. García-García

Published in: Topics in Catalysis | Issue 1-4/2019

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Abstract

In this study, Ce/Zr-based materials without noble metals in their formulation have been prepared, characterized and tested in NOx adsorption at different temperatures. In particular, the effect of the presence of Ba and Cu in the catalytic formulation has been investigated. The catalyst characterization shows that the redox properties of the catalysts are enhanced by Cu and inhibited by Ba. Upon interaction with NO/O2, it is found that NOx are stored at low temperatures (150 °C) in the form of nitrites, without any relevant NO oxidation activity. This suggests a direct NO uptake. At higher temperatures (300 °C) a significant NO oxidation activity is observed, that is enhanced by Cu and depressed by Ba. In this case, NOx are stored in the form of nitrates; the samples containing both Ba and Cu exhibits the better performances in terms of NOx adsorption capacity.
previous article Selective Catalytic Reduction of NOx with Ammonia and Hydrocarbon Oxidation Over V2O5–MoO3/TiO2 and V2O5–WO3/TiO2 SCR Catalysts
next article Simulation of a NOx Sensor for Model-Based Control of Exhaust Aftertreatment Systems

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Metadata
Title
NOx Adsorption Over Ce/Zr-Based Catalysts Doped with Cu and Ba
Authors
J. Giménez-Mañogil
J. C. Martínez-Munuera
R. Matarrese
L. Castoldi
L. Lietti
A. García-García
Publication date
07-01-2019
Publisher
Springer US
Published in
Topics in Catalysis / Issue 1-4/2019
Print ISSN: 1022-5528
Electronic ISSN: 1572-9028
DOI
https://doi.org/10.1007/s11244-018-1130-z

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