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Journal of Materials Science

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23-07-2018 | Composites

Reduced graphene oxide enhanced magnetic nanocomposites for removal of carbamazepine

Authors: Yijie Jiang, Dezhi Chen, Wu Yang, Shaolin Wu, Xubiao Luo

Published in: Journal of Materials Science | Issue 22/2018

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Abstract

Ferrite, as a kind of common magnetic adsorbent, always tend to reuniting and lead to the poor performance for removing contaminant in aqueous. Meanwhile, reduced graphene oxide (rGO), a high-efficiency adsorbent used for water treatment, is hydrophobic and easy to stack because of the Van der Waals force, resulting in the low adsorption capacity. Herein, we prepare the magnetic CoFe₂O₄/rGO nanocomposites to solve the reuniting of CoFe₂O₄ and stacking of rGO simultaneously. The rGO nanosheets can improve the dispersion of CoFe₂O₄ nanoparticles. As sorbent, the adsorption behaviors of carbamazepine on the nanocomposites can be fitted well by the Langmuir and pseudo-second-order kinetic models. In addition, the CoFe₂O₄/rGO nanocomposites show enhanced adsorption performance than that of the pure CoFe₂O₄ nanoparticles, and the loading of rGO can affect their adsorption performance. The adsorption of carbamazepine on CoFe₂O₄/rGO is exothermic and mainly controlled by π–π interaction and hydrogen bond interaction. Furthermore, the CoFe₂O₄/rGO can be used to remove other organic pollutants simultaneously. Finally, the nanocomposites can be collected by external magnet, and the regenerated nanocomposites still showed a high adsorption capacity retention (90%) after five cycles.

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Title: Reduced graphene oxide enhanced magnetic nanocomposites for removal of carbamazepine
Authors: Yijie Jiang
Dezhi Chen
Wu Yang
Shaolin Wu
Xubiao Luo
Publication date: 23-07-2018
Publisher: Springer US
Published in: Journal of Materials Science / Issue 22/2018
Print ISSN: 0022-2461
Electronic ISSN: 1573-4803
DOI: https://doi.org/10.1007/s10853-018-2712-7

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