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Published in: Adsorption 2/2012

01-10-2012

Sorption equilibria of CO2 on silica-gels in the presence of water

Authors: Juanjuan Zheng, Yaping Zhou, Yong Ting Zhi, Wei Su, Yan Sun

Published in: Adsorption | Issue 2/2012

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Abstract

The sorption equilibria of carbon dioxide on three types of silica gel (SG) with different pore size distributions in the presence of water were studied experimentally using a volumetric method at 275 K with pressures from 0 to 3.7 MPa. Both the pore size distribution of the silica gel and the quantity of pre-sorbed water impact the formation of the CO2 hydrates. For wet silicon gel A(SG-A) with water loading ratio of 0.75, the highest CO2 sorption was about 2.5 mmol of CO2 per gram of dry sorbent at 275 K. Similarly, the highest sorption was about 2.7 mmol for wet SG-B with R w =0.81. However, CO2 hydrate did not form on the wet surface of SG-C due to its large pore sizes.

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Metadata
Title
Sorption equilibria of CO2 on silica-gels in the presence of water
Authors
Juanjuan Zheng
Yaping Zhou
Yong Ting Zhi
Wei Su
Yan Sun
Publication date
01-10-2012
Publisher
Springer US
Published in
Adsorption / Issue 2/2012
Print ISSN: 0929-5607
Electronic ISSN: 1572-8757
DOI
https://doi.org/10.1007/s10450-012-9387-1

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