Skip to main content
Top
Published in: Rheologica Acta 4/2009

01-05-2009 | Original Contribution

Droplet dynamics in sub-critical complex flows

Authors: Elia Boonen, Peter Van Puyvelde, Paula Moldenaers

Published in: Rheologica Acta | Issue 4/2009

Log in

Activate our intelligent search to find suitable subject content or patents.

search-config
loading …

Abstract

A newly designed eccentric cylinder device has been used to study the deformation and orientation of single Newtonian droplets immersed in an immiscible Newtonian liquid in a controlled complex flow field. Optical microscopy coupled with image acquisition analysis allows monitoring the dynamics of droplets flowing in the gap between the eccentric cylinders. Throughout the experiments, the flow intensity was kept below the critical conditions for droplet break-up. The experimental results are compared with predictions which are obtained using the transient form of the phenomenological model of Maffettone and Minale (J Non-Newtonian Fluid Mech 78:227–241, 1998; J Non-Newtonian Fluid Mech 84:105–106, 1999), incorporating a flow type parameter that accounts for the relative amount of elongational effects in the flow field and adapting the capillary number to mixed flows. For all the sub-critical flows studied here, good agreement was found between model predictions and experimental data, providing, for the first time, a quantitative assessment of drop shape predictions in complex flows.

Dont have a licence yet? Then find out more about our products and how to get one now:

Springer Professional "Technik"

Online-Abonnement

Mit Springer Professional "Technik" erhalten Sie Zugriff auf:

  • über 67.000 Bücher
  • über 390 Zeitschriften

aus folgenden Fachgebieten:

  • Automobil + Motoren
  • Bauwesen + Immobilien
  • Business IT + Informatik
  • Elektrotechnik + Elektronik
  • Energie + Nachhaltigkeit
  • Maschinenbau + Werkstoffe




 

Jetzt Wissensvorsprung sichern!

Springer Professional "Wirtschaft+Technik"

Online-Abonnement

Mit Springer Professional "Wirtschaft+Technik" erhalten Sie Zugriff auf:

  • über 102.000 Bücher
  • über 537 Zeitschriften

aus folgenden Fachgebieten:

  • Automobil + Motoren
  • Bauwesen + Immobilien
  • Business IT + Informatik
  • Elektrotechnik + Elektronik
  • Energie + Nachhaltigkeit
  • Finance + Banking
  • Management + Führung
  • Marketing + Vertrieb
  • Maschinenbau + Werkstoffe
  • Versicherung + Risiko

Jetzt Wissensvorsprung sichern!

Literature
go back to reference Almusallam AS, Larson RG, Solomon MJ (2000) A constrained volume model for the prediction of droplet shapes and stresses in immiscible blends. J Rheol 44:1055–1083CrossRefADS Almusallam AS, Larson RG, Solomon MJ (2000) A constrained volume model for the prediction of droplet shapes and stresses in immiscible blends. J Rheol 44:1055–1083CrossRefADS
go back to reference Ballal BY, Rivlin RS (1976) Flow of a Newtonian fluid between eccentric rotating cylinders—inertial effects. Arch Rat Mech Anal 62:237–294MATHCrossRefMathSciNet Ballal BY, Rivlin RS (1976) Flow of a Newtonian fluid between eccentric rotating cylinders—inertial effects. Arch Rat Mech Anal 62:237–294MATHCrossRefMathSciNet
go back to reference Bentley BL, Leal LG (1986) An experimental investigation of drop deformation and break-up in steady two-dimensional linear flows. J Fluid Mech 167:241–283MATHCrossRefADS Bentley BL, Leal LG (1986) An experimental investigation of drop deformation and break-up in steady two-dimensional linear flows. J Fluid Mech 167:241–283MATHCrossRefADS
go back to reference Chin HB, Han CD (1980) Studies on droplet deformation and break-up. 2. Break-up of a droplet in a nonuniform shear flow. J Rheol 24:1–37MATHCrossRefADS Chin HB, Han CD (1980) Studies on droplet deformation and break-up. 2. Break-up of a droplet in a nonuniform shear flow. J Rheol 24:1–37MATHCrossRefADS
go back to reference Cox RG (1969) The deformation of a drop in a general time-dependent fluid flow. J Fluid Mech 37:601–623MATHCrossRefADS Cox RG (1969) The deformation of a drop in a general time-dependent fluid flow. J Fluid Mech 37:601–623MATHCrossRefADS
go back to reference Cristini V, Hooper RW, Macosko CW, Simeone M, Guido S (2002) A numerical and experimental investigation of lamellar blends morphologies. Ind Eng Chem Res 41:6305–6311CrossRef Cristini V, Hooper RW, Macosko CW, Simeone M, Guido S (2002) A numerical and experimental investigation of lamellar blends morphologies. Ind Eng Chem Res 41:6305–6311CrossRef
go back to reference de Bruijn RA (1989) Deformation and break-up of drops in simple shear flows. Ph.D. thesis, Eindhoven University of Technology, The Netherlands de Bruijn RA (1989) Deformation and break-up of drops in simple shear flows. Ph.D. thesis, Eindhoven University of Technology, The Netherlands
go back to reference Diprima RC, Stuart JT (1972) Flow between eccentric rotating cylinders. ASME J Lubr Tech 94:266–274 Diprima RC, Stuart JT (1972) Flow between eccentric rotating cylinders. ASME J Lubr Tech 94:266–274
go back to reference Feigl K, Kaufmann SFM, Fischer P, Windhab EJ (2003) A numerical procedure for calculating droplet deformation in dispersing flows and experimental verification. Chem Eng Sci 58:2351–2363CrossRef Feigl K, Kaufmann SFM, Fischer P, Windhab EJ (2003) A numerical procedure for calculating droplet deformation in dispersing flows and experimental verification. Chem Eng Sci 58:2351–2363CrossRef
go back to reference Godbille FD, Picot JJC (2000) Drop break-up in combined shear and elongational flow conditions. Adv Polym Tech 19:14–21CrossRef Godbille FD, Picot JJC (2000) Drop break-up in combined shear and elongational flow conditions. Adv Polym Tech 19:14–21CrossRef
go back to reference Grace HP (1982) Dispersion phenomena in high-viscosity immiscible fluid systems and application of static mixers as dispersion devices in such systems. Chem Eng Commun 14:225–277CrossRef Grace HP (1982) Dispersion phenomena in high-viscosity immiscible fluid systems and application of static mixers as dispersion devices in such systems. Chem Eng Commun 14:225–277CrossRef
go back to reference Guido S, Greco F (2004) Dynamics of a liquid drop in a flowing immiscible liquid. Rheology Reviews 2004, The British Society of Rheology: 99–142 Guido S, Greco F (2004) Dynamics of a liquid drop in a flowing immiscible liquid. Rheology Reviews 2004, The British Society of Rheology: 99–142
go back to reference Guido S, Minale M, Maffettone PL (2000) Drop shape dynamics under shear-flow reversal. J Rheol 44:1385–1399CrossRefADS Guido S, Minale M, Maffettone PL (2000) Drop shape dynamics under shear-flow reversal. J Rheol 44:1385–1399CrossRefADS
go back to reference Han CD, Funatsu K (1978) Experimental study of droplet deformation and break-up in pressure driven flows through converging and uniform channels. J Rheol 22:113–133CrossRefADS Han CD, Funatsu K (1978) Experimental study of droplet deformation and break-up in pressure driven flows through converging and uniform channels. J Rheol 22:113–133CrossRefADS
go back to reference Janssen JMH, Meijer HEH (1993) Droplet breakup mechanisms: stepwise equilibrium versus transient dispersion. J Rheol 37:597–608CrossRefADS Janssen JMH, Meijer HEH (1993) Droplet breakup mechanisms: stepwise equilibrium versus transient dispersion. J Rheol 37:597–608CrossRefADS
go back to reference Kamal MM (1966) Separation in the flow between eccentric rotating cylinders. ASME J Basic Eng 88:717–724 Kamal MM (1966) Separation in the flow between eccentric rotating cylinders. ASME J Basic Eng 88:717–724
go back to reference Kaufmann SFM, Fischer P, Windhab EJ (2000) Investigation of droplet dispersing processes in shear and elongational flow. In: Fischer P, Marti I, Windhab EJ (eds) Second international symposium on food rheology and structure. Laboratory of Food Process Engineering, Zurich, Switzerland, pp 404–405 Kaufmann SFM, Fischer P, Windhab EJ (2000) Investigation of droplet dispersing processes in shear and elongational flow. In: Fischer P, Marti I, Windhab EJ (eds) Second international symposium on food rheology and structure. Laboratory of Food Process Engineering, Zurich, Switzerland, pp 404–405
go back to reference Khayat RE, Luciani A, Utracki LA, Godbille FD, Picot JJC (2000) Influence of shear and elongation on drop deformation in convergent–divergent flows. Int J Multiphase Flow 26:17–44MATHCrossRef Khayat RE, Luciani A, Utracki LA, Godbille FD, Picot JJC (2000) Influence of shear and elongation on drop deformation in convergent–divergent flows. Int J Multiphase Flow 26:17–44MATHCrossRef
go back to reference Maffettone PL, Minale M (1998) Equation of change for ellipsoidal drops in viscous flow. J Non-Newtonian Fluid Mech 78:227–241MATHCrossRef Maffettone PL, Minale M (1998) Equation of change for ellipsoidal drops in viscous flow. J Non-Newtonian Fluid Mech 78:227–241MATHCrossRef
go back to reference Maffettone PL, Minale M (1999) Equation of change for ellipsoidal drops in viscous flows (vol 78, p 227, 1998). J Non-Newtonian Fluid Mech 84:105–106CrossRef Maffettone PL, Minale M (1999) Equation of change for ellipsoidal drops in viscous flows (vol 78, p 227, 1998). J Non-Newtonian Fluid Mech 84:105–106CrossRef
go back to reference Mietus WGP, Matar OK, Lawrence CJ, Briscoe BJ (2002) Droplet deformation in confined shear and extensional. Chem Eng Sci 57:1217–1230CrossRef Mietus WGP, Matar OK, Lawrence CJ, Briscoe BJ (2002) Droplet deformation in confined shear and extensional. Chem Eng Sci 57:1217–1230CrossRef
go back to reference Minale M (2004) Deformation of a non-Newtonian ellipsoidal drop in a non-Newtonian matrix: extension of the Maffettone–Minale model. J Non-Newtonian Fluid Mech 123:151–160MATHCrossRef Minale M (2004) Deformation of a non-Newtonian ellipsoidal drop in a non-Newtonian matrix: extension of the Maffettone–Minale model. J Non-Newtonian Fluid Mech 123:151–160MATHCrossRef
go back to reference Okamoto K, Takahashi M, Yamane H, Kashihara H, Watanabe H, Masuda T (1999) Shape recovery of dispersed droplet phase and stress relaxation after application of step shear strains in a polystyrene/polycarbonate blend melt. J Rheol 43:951–965CrossRefADS Okamoto K, Takahashi M, Yamane H, Kashihara H, Watanabe H, Masuda T (1999) Shape recovery of dispersed droplet phase and stress relaxation after application of step shear strains in a polystyrene/polycarbonate blend melt. J Rheol 43:951–965CrossRefADS
go back to reference Ottino JM, Leong CW, Rising H, Swanson PD (1988) Morphological structures produced by mixing in chaotic flows. Nature 333:419–425CrossRefADS Ottino JM, Leong CW, Rising H, Swanson PD (1988) Morphological structures produced by mixing in chaotic flows. Nature 333:419–425CrossRefADS
go back to reference Ottino JM, De Roussel P, Hansen S, Khakhar DV (1999) Mixing and dispersion of viscous liquids and powdered solids. Adv Chem Eng 25:105–204CrossRef Ottino JM, De Roussel P, Hansen S, Khakhar DV (1999) Mixing and dispersion of viscous liquids and powdered solids. Adv Chem Eng 25:105–204CrossRef
go back to reference Priore BE, Walker LM (2001) Small angle light scattering analysis of morphology development of a model immiscible polymer blend in transient slit-contraction flows. J Rheol 45:383–402CrossRefADS Priore BE, Walker LM (2001) Small angle light scattering analysis of morphology development of a model immiscible polymer blend in transient slit-contraction flows. J Rheol 45:383–402CrossRefADS
go back to reference Rasband WS (1997–2007) Image J. U. S. National Institutes of Health, Bethesda, Maryland, USA Rasband WS (1997–2007) Image J. U. S. National Institutes of Health, Bethesda, Maryland, USA
go back to reference Stone HA (1994) Dynamics of drop deformation in viscous liquids. Annu Rev Fluid Mech 26:65–102CrossRefADS Stone HA (1994) Dynamics of drop deformation in viscous liquids. Annu Rev Fluid Mech 26:65–102CrossRefADS
go back to reference Stone HA, Leal LG (1989) The influence of initial deformation on drop break-up in sub-critical time-dependent flows at low Reynolds numbers. J Fluid Mech 206:223–263CrossRefADS Stone HA, Leal LG (1989) The influence of initial deformation on drop break-up in sub-critical time-dependent flows at low Reynolds numbers. J Fluid Mech 206:223–263CrossRefADS
go back to reference Stone HA, Bentley BL, Leal LG (1986) An experimental study of transient effects in the break-up of viscous drops. J Fluid Mech 173:131–158CrossRefADS Stone HA, Bentley BL, Leal LG (1986) An experimental study of transient effects in the break-up of viscous drops. J Fluid Mech 173:131–158CrossRefADS
go back to reference Taylor GI (1932) The viscosity of a fluid containing small drops of another fluid. Proc Roy Soc Lond Math Phys Sci 138:41–48MATHCrossRefADS Taylor GI (1932) The viscosity of a fluid containing small drops of another fluid. Proc Roy Soc Lond Math Phys Sci 138:41–48MATHCrossRefADS
go back to reference Taylor GI (1934) The formation of emulsions in definable fields of flow. Proc Roy Soc Lond Math Phys Sci 146:501–523CrossRefADS Taylor GI (1934) The formation of emulsions in definable fields of flow. Proc Roy Soc Lond Math Phys Sci 146:501–523CrossRefADS
go back to reference Testa C, Sigillo I, Grizzuti N (2001) Morphology evolution of immiscible polymer blends in complex flow fields. Polymer 42:5651–5659CrossRef Testa C, Sigillo I, Grizzuti N (2001) Morphology evolution of immiscible polymer blends in complex flow fields. Polymer 42:5651–5659CrossRef
go back to reference Utracki LA (1989) Polymer alloys and blends. Hanser, Munich Utracki LA (1989) Polymer alloys and blends. Hanser, Munich
go back to reference Van der Reijden-Stolk C, Sara A (1986) A study on polymer blending microrheology. 3. Deformation of Newtonian drops submerged in another Newtonian fluid flowing through a converging cone. Polym Eng Sci 26:1229–1239CrossRef Van der Reijden-Stolk C, Sara A (1986) A study on polymer blending microrheology. 3. Deformation of Newtonian drops submerged in another Newtonian fluid flowing through a converging cone. Polym Eng Sci 26:1229–1239CrossRef
go back to reference Van Puyvelde P, Yang H, Mewis J, Moldenaers P (2000) Break-up of filaments in blends during simple shear flow. J Rheol 44:1401–1415CrossRefADS Van Puyvelde P, Yang H, Mewis J, Moldenaers P (2000) Break-up of filaments in blends during simple shear flow. J Rheol 44:1401–1415CrossRefADS
go back to reference Vananroye A, Van Puyvelde P, Moldenaers P (2006) Structure development in confined polymer blends: Steady-state shear flow and relaxation. Langmuir 22:2273–2280PubMedCrossRef Vananroye A, Van Puyvelde P, Moldenaers P (2006) Structure development in confined polymer blends: Steady-state shear flow and relaxation. Langmuir 22:2273–2280PubMedCrossRef
go back to reference Vananroye A, Van Puyvelde P, Moldenaers P (2007) Effect of confinement on the steady-state behavior of single droplets during shear flow. J Rheol 51:139–153CrossRefADS Vananroye A, Van Puyvelde P, Moldenaers P (2007) Effect of confinement on the steady-state behavior of single droplets during shear flow. J Rheol 51:139–153CrossRefADS
go back to reference Windhab EJ, Dressler M, Feigl K, Fischer P, Megias-Alguacil D (2005) Emulsion processing—from single-drop deformation to design of complex processes and products. Chem Eng Sci 60:2101–2113CrossRef Windhab EJ, Dressler M, Feigl K, Fischer P, Megias-Alguacil D (2005) Emulsion processing—from single-drop deformation to design of complex processes and products. Chem Eng Sci 60:2101–2113CrossRef
go back to reference Yamane H, Takahashi M, Hayashi R, Okamoto K, Kashihara H, Masuda T (1998) Observation of deformation and recovery of poly(isobutylene) droplet in a poly(isobutylene)/ poly(dimethyl siloxane) blend after application of step shear strain. J Rheol 42:567–579CrossRefADS Yamane H, Takahashi M, Hayashi R, Okamoto K, Kashihara H, Masuda T (1998) Observation of deformation and recovery of poly(isobutylene) droplet in a poly(isobutylene)/ poly(dimethyl siloxane) blend after application of step shear strain. J Rheol 42:567–579CrossRefADS
go back to reference Yu W, Bousmina M (2003) Ellipsoidal model for droplet deformation in emulsions. J Rheol 47:1001–1039CrossRef Yu W, Bousmina M (2003) Ellipsoidal model for droplet deformation in emulsions. J Rheol 47:1001–1039CrossRef
Metadata
Title
Droplet dynamics in sub-critical complex flows
Authors
Elia Boonen
Peter Van Puyvelde
Paula Moldenaers
Publication date
01-05-2009
Publisher
Springer-Verlag
Published in
Rheologica Acta / Issue 4/2009
Print ISSN: 0035-4511
Electronic ISSN: 1435-1528
DOI
https://doi.org/10.1007/s00397-008-0322-z

Other articles of this Issue 4/2009

Rheologica Acta 4/2009 Go to the issue

Premium Partners