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Journal of Materials Science: Materials in Electronics
Published in: Journal of Materials Science: Materials in Electronics 7/2019

20-02-2019

Effects of Bi2O3–ZnO–B2O3–SiO2 glass addition on the sintering and microwave dielectric properties of ZnZrNb2O8 ceramics for LTCC applications

Authors: Shishun Qi, Huarong Cheng, Kuiyong Yang, Beibei Song, Shuying Sun, Yong Zhang

Published in: Journal of Materials Science: Materials in Electronics | Issue 7/2019

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Abstract

A novel low-temperature sinterable microwave dielectric ceramic was successfully developed by adding low-melting-point Bi2O3–ZnO–B2O3–SiO2 (BBSZ) glass to ZnZrNb2O8 (ZZN) ceramic. The influence of BBSZ glass on the densification behavior and microwave dielectric properties of ZZN ceramic was systematically investigated by means of an X-ray diffractometer, a scanning electron microscope and a network analyzer. By adding an appropriate amount of BBSZ glass into ZZN ceramic, the sintering temperature was lowered to 950 °C, indicating that BBSZ glass was an effective firing agent for ZZN ceramic. Furthermore, favorable microwave dielectric properties of ɛr = 32.5, Q×f = 38,400 GHz and τf = − 51 ppm/°C were yielded in the ZZN sample with 6 wt% BBSZ glass addition, simultaneously maintaining uniform and compact microstructure. The chemical compatibility between the present composite and Ag electrode was also investigated for commercial applications.
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Literature
1.
M.T. Sbeastian, H. Jantunen, Low loss dielectric materials for LTCC applications: a review. Int. Mater. Rev. 53(2), 57–90 (2008)CrossRef
2.
D.W. Kim, K.S. Hong, C.S. Yoon, C.K. Kim, Low-temperature sintering and microwave dielectric properties of Ba5Nb4O15-BaNb2O6 mixtures for LTCC applications. J. Eur. Ceram. Soc. 23(14), 2597–2601 (2003)CrossRef
3.
K.C. Li, H. Wang, H.F. Zhou, M.H. Zhang, X. Yao, Silver co-firable ZnTiNb2O8 microwave dielectric ceramics with Li2O-ZnO-B2O3 glass additive. Int. J. Appl. Ceram. Technol. 7(S1), 144–150 (2010)CrossRef
4.
A. Mohanram, S.H. Lee, G.L. Messing, D.J. Green, Constrained sintering of low-temperature co-fired ceramics. J. Am. Ceram. Soc. 89(6), 1923–1929 (2006)CrossRef
5.
Q.L. Zhang, H. Yang, H.P. Sun, A new microwave ceramic with low-permittivity for LTCC applications. J. Eur. Ceram. Soc. 28(3), 605–609 (2008)CrossRef
6.
Q.L. Zhang, D. Zou, H. Yang, Microwave dielectric properties of Ba3Ti4–x(Zn 1/3Nb2/3)xNb4O21 for low temperature co-fired ceramics. J. Eur. Ceram. Soc. 31(3), 265–272 (2011)CrossRef
7.
Y.Z. Hao, Q.L. Zhang, J. Zhang, C.R. Xin, H. Yang, Enhanced sintering characteristics and microwave dielectric properties of Li2TiO3 due to nano-size and nonstoichiometry effect. J. Mater. Chem. 22(45), 23885–23892 (2012)CrossRef
8.
C. Zhang, R.Z. Zuo, Q. Sun, Z.W. Hu, J.J. Zhang, Microwave dielectric properties and low temperature sintering of the ZnO-V2O5 doped Ba3Ti2(Mg1/3Nb2/3)2Nb4O21 ceramics. Ceram. Int. 39, 5675–5679 (2013)CrossRef
9.
X.P. Lu, Y. Zheng, B. Zhou, Z.W. Dong, P. Cheng, Microwave dielectric properties of Li2ZnTi3O8 ceramics doped with Bi2O3. Ceram. Int. 39, 9829–9833 (2013)CrossRef
10.
Y.J. Chu, J.H. Jean, Low-fire processing of microwave BaTi4O9 dielectric with crystalline CuB2O4 and BaCuB2O5 additives. Ceram. Int. 39, 5151–5158 (2013)CrossRef
11.
S.X. Duan, E.Z. Li, H.T. Chen, B. Tang, Y. Yuan, S.R. Zhang, Influence of Li2O-B2O3-SiO2 glass on the sintering behavior and microwave dielectric properties of BaO-0.15ZnO-4TiO2 ceramics. Ceram. Int. 42, 7943–7949 (2016)CrossRef
12.
Q.W. Liao, L.X. Li, X. Ren, X.X. Yu, D. Guo, M.J. Wang, A low sintering temperature low loss microwave dielectric material ZnZrNb2O8. J. Am. Ceram. Soc. 95(11), 3363–3365 (2012)CrossRef
13.
S.D. Ramarao, V.R.K. Murthy, Crystal structure refinement and microwave dielectric properties of new low dielectric loss AZrNb2O8 (A: Mn, Zn, Mg and Co) ceramics. Scr. Mater. 69, 274–277 (2013)CrossRef
14.
H.T. Wu, E.S. Kim, Characterization of crystal structure and microwave dielectric properties of AZrNb2O8 (A = Zn, Co, Mg, Mn) ceramics based on complex bond theory. Ceram. Int. 42, 5785–5791 (2016)CrossRef
15.
L.X. Li, H. Sun, H.C. Cai, X.S. Lv, Microstructure and microwave dielectric characteristics of ZnZrNb2O8 and (Zn0.95M0.05)ZrNb2O8 (M = Ni, Mg, Co and Mn) ceramics. J. Alloys Compd. 639, 516–519 (2015)CrossRef
16.
X.S. Lyu, L.X. Li, S. Zhang, H. Sun, B.W. Zhang, J.T. Li, M.K. Du, Crystal structure and microwave dielectric properties of novel (1-x)ZnZrNb2O8-xTiO2 ceramics. Mater. Lett. 171, 129–132 (2016)CrossRef
17.
L.X. Li, S. Zhang, J. Ye, X.S. Lv, H. Sun, S. Li, Crystal structure and microwave dielectric properties of the low dielectric loss ZnZr1–xSnxNb2O8 ceramics. Ceram. Int. 42, 9157–9161 (2016)CrossRef
18.
H.T. Wu, Z.B. Feng, Q.J. Mei, J.D. Guo, J.X. Bi, Correlations of crystal structure, bond energy and microwave dielectric properties of AZrNb2O8 (A = Zn, Co, Mg, Mn) ceramics. J. Alloys Compd. 648, 368–373 (2015)CrossRef
19.
H.T. Wu, J.X. Bi, H.J. Wang, X.S. Jiang, Y.X. Mao, Sintering characteristics and microwave dielectric properties of low loss ZnZrNb2O8 ceramics achieved by reaction sintering process. J. Mater. Sci.: Mater. Electron. 27, 5670–5675 (2016)
20.
Y.G. Zhao, P. Zhang, Preparation for ultra-low loss dielectric ceramics of ZnZrNb2O8 by reaction-sintering process. J. Alloys Compd. 672, 630–635 (2016)CrossRef
21.
J.X. Bi, C.F. Xing, Y.H. Zhang, C.H. Yang, H.T. Wu, Correlation of crystal structure and microwave dielectric properties of Zn1–xNixZrNb2O8 (0 ≤ x ≤ 0.1) ceramics. J. Alloys Compd. 727, 123–134 (2017)CrossRef
22.
J.X. Bi, C.F. Xing, Y.H. Zhang, C.H. Yang, H.T. Wu, Correlation of crystal structure and microwave dielectric characteristics of temperature stable Zn1–xMnxZrNb2O8 (0.02 ≤ x ≤ 0.1) ceramics. Ceram. Int. 43, 92–98 (2017)CrossRef
23.
W.J. Luo, L.X. Li, X.S. Lv, S. Zhang, Z. Sun, J.T. Li, Structure analysis and microwave dielectric properties of germanium ion-doped ZnZrNb2O8 ceramics. J. Mater. Sci.: Mater. Electron. 28, 9755–9762 (2017)
24.
H.T. Wu, J.X. Bi, Synthesis, characterization, and microwave dielectric properties of monoclinal structure ZnZrNb2O8 ceramics through the aqueous sol-gel process. J. Mater. Sci.: Mater. Electron. 27, 3474–3480 (2016)
25.
J.X. Bi, C.F. Xing, X.S. Jiang, C.H. Yang, H.T. Wu, Effect of H3BO3 on sintering behavior and microwave dielectric properties of monoclinal structure ZnZrNb2O8 ceramics. J. Mater. Sci.: Mater. Electron. 27, 8055–8061 (2016)
26.
X. Tang, H. Yang, Q.L. Zhang, J.H. Zhou, Low-temperature sintering and microwave dielectric properties of ZnZrNb2O8 ceramics with BaCu(B2O5) addition. Ceram. Int. 40, 12875–12881 (2014)CrossRef
27.
O. Dernovek, A. Naeini, G. Preu, W. Wersing, M. Eberstein, W.A. Schiller, LTCC glass-ceramic composites for microwave application. J. Eur. Ceram. Soc. 21(10–11), 1693–1697 (2001)CrossRef
28.
M. Chen, J. Juuti, C. Hsi, C. Chia, H. Jantunen, Dielectric BaTiO3-BBSZ glass ceramic composition with ultra-low sintering temperature. J. Eur. Ceram. Soc. 35(1), 139–144 (2015)CrossRef
29.
S. Thomas, M.T. Sebastian, Effect of B2O3-Bi2O3-SiO2-ZnO glass on the sintering and microwave dielectric properties of 0.83ZnAl2O4-0.17TiO2. Mater. Res. Bull. 43(4), 843–851 (2008)CrossRef
30.
I.J. Induja, P. Abhilash, S. Arun, K.P. Surendran, M.T. Sebastian, LTCC tapes based on Al2O3-BBSZ glass with improved thermal conductivity. Ceram. Int. 41, 13572–13581 (2015)CrossRef
31.
M.Y. Chen, J. Juuti, C.S. Hsi, C.T. Chia, H. Jantunen, Dielectric properties of ultra-low sintering temperature Al2O3-BBSZ glass composite. J. Am. Ceram. Soc. 98(4), 1133–1136 (2015)CrossRef
32.
H. Hsiang, T. Chen, Dielectric and magnetic properties of low-temperature fired ferrite-dielectric composites. J. Am. Ceram. Soc. 91(6), 2043–2046 (2010)CrossRef
33.
H.S. Ren, T.Y. Xie, M.Z. Dang, S.H. Jiang, H.X. Lin, L. Luo, Sintering mechanism and microwave dielectric properties of BaTi4O9-BBZ composite for LTCC technology. Ceram. Int. 43, 11286–12863 (2017)
34.
M.C. Wu, S. Kamba, V. Bovtun, W.F. Su, Comparison of microwave dielectric behavior between Bi1.5Zn0.92Nb1.5O6.92 and Bi1.5ZnNb1.5O7. J. Eur. Ceram. Soc. 26, 1889–1893 (2006)CrossRef
35.
E.S. Kim, W. Choi, Effect of phase transition on the microwave dielectric properties of BiNbO4. J. Eur. Ceram. Soc. 26(10–11), 1761–1766 (2006)CrossRef
Metadata
Title
Effects of Bi2O3–ZnO–B2O3–SiO2 glass addition on the sintering and microwave dielectric properties of ZnZrNb2O8 ceramics for LTCC applications
Authors
Shishun Qi
Huarong Cheng
Kuiyong Yang
Beibei Song
Shuying Sun
Yong Zhang
Publication date
20-02-2019
Publisher
Springer US
Published in
Journal of Materials Science: Materials in Electronics / Issue 7/2019
Print ISSN: 0957-4522
Electronic ISSN: 1573-482X
DOI
https://doi.org/10.1007/s10854-019-00944-7

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