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Journal of Materials Science: Materials in Electronics

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24-08-2020

Enhanced dielectric and tunable properties of Ba-doped (Pb,La)(Zr,Sn,Ti)O₃ antiferroelectric ceramics

Authors: Xiucai Wang, Weiqiang Cai, Ze Xiao, Xinmei Yu, Jianwen Chen, Tongqing Yang

Published in: Journal of Materials Science: Materials in Electronics | Issue 19/2020

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Abstract

In this work, a simple method to improve the dielectric tunability of antiferroelectric ceramics was introduced, and (Pb_0.97−xLa_0.02Ba_x)(Zr_0.50Sn_0.40Ti_0.10)O₃ (x = 0.08, 0.09, 0.10) antiferroelectric ceramics were prepared by conventional solid-state route. The effect of Ba-modification on phase structure and electric properties was systematically investigated. The results revealed that the barium content contributed to the decline of the Curie temperature and enhanced dielectric tunable performance. All compositions exhibited butterfly curve, and a high tunability of 48.89% at E_AF and 53.02% at E_FA was obtained in (Pb_0.87La_0.02Ba_0.10)(Zr_0.50Sn_0.40Ti_0.10)O₃. In addition, the ε_max/ε_min ratio was up to 25.32, making it a promising candidate for nonlinear tunable devices.

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Title: Enhanced dielectric and tunable properties of Ba-doped (Pb,La)(Zr,Sn,Ti)O3 antiferroelectric ceramics
Authors: Xiucai Wang
Weiqiang Cai
Ze Xiao
Xinmei Yu
Jianwen Chen
Tongqing Yang
Publication date: 24-08-2020
Publisher: Springer US
Published in: Journal of Materials Science: Materials in Electronics / Issue 19/2020
Print ISSN: 0957-4522
Electronic ISSN: 1573-482X
DOI: https://doi.org/10.1007/s10854-020-04258-x

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