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Journal of Iron and Steel Research International
Published in: Journal of Iron and Steel Research International 10/2020

14-08-2020 | Original Paper

Highly improved hydrogen storage dynamics of nanocrystalline and amorphous NdMg12-type alloys by mechanical milling

Authors: Ying-chun Liu, Yan Qi, Wei Zhang, Jin-liang Gao, Yang-huan Zhang

Published in: Journal of Iron and Steel Research International | Issue 10/2020

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Abstract

To improve the hydrogenation and dehydrogenation dynamics of NdMg12-type alloy, we replaced part of Mg with Ni in the samples and used the ball milling method to prepare NdMg11Ni + x wt.% Ni (x = 100, 200) samples. The influences of milling duration and Ni content on the electrochemical and gaseous dynamics of the samples were studied in detail. Dehydrogenation activation energies of samples were calculated by using Kissinger and Arrhenius methods. The conclusions show that the dynamic properties of samples are significantly enhanced with the increase in Ni content. With the change of the milling duration, the gaseous hydrogenation rate and high rate discharging capability reach the maximal values. However, the dehydrogenation dynamics of sample alloys are always enhanced with the prolonging of milling duration. More concretely, prolonging milling duration from 5 to 60 h improves the dehydrogenation ratio of NdMg11Ni + 100 wt.% Ni alloy from 58.03% to 64.81% and that of NdMg11Ni + 200 wt.% Ni alloy from 62.20% to 71.59%. Besides, the enhancement of gaseous hydrogen storage dynamics of the samples is believed to be the result of the declined dehydrogenation activation energy resulted from the increase in milling duration and Ni content.
previous article Cyclic oxidation behavior of NiCoCrAlY/YSZ@Ni composite coatings fabricated by laser cladding
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Metadata
Title
Highly improved hydrogen storage dynamics of nanocrystalline and amorphous NdMg12-type alloys by mechanical milling
Authors
Ying-chun Liu
Yan Qi
Wei Zhang
Jin-liang Gao
Yang-huan Zhang
Publication date
14-08-2020
Publisher
Springer Singapore
Published in
Journal of Iron and Steel Research International / Issue 10/2020
Print ISSN: 1006-706X
Electronic ISSN: 2210-3988
DOI
https://doi.org/10.1007/s42243-020-00473-2

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