Skip to main content
Disciplines
Automotive Business IT + Informatics Construction + Real Estate Electrical Engineering + Electronics Energy + Sustainability Insurance + Risk Finance + Banking Management + Leadership Marketing + Sales Mechanical Engineering + Materials
Events
DE
EN
Books
Journals
Topic Page
Marketing
Start single access now
Access for companies
EXTENDED SEARCH
Log in
Top
Journal of Electroceramics
Published in: Journal of Electroceramics 2-4/2010

01-10-2010

Low-temperature sintering of BaTiO3 with Mn-Si-O glass

Authors: Jerry C. C. Lin, Wen-Cheng J. Wei

Published in: Journal of Electroceramics | Issue 2-4/2010

Log in

Activate our intelligent search to find suitable subject content or patents.

search-config
loading …

Abstract

In order to reduce sintering temperature and prevent adverse dielectric effects, pure BaTiO3 powder with the addition of Mn-Si-O glass was sintered in the temperature range of 1175–1300°C. Microstructural observation showed that BaTiO3 grains of the sintered samples only grew from the initial 400 nm to an average of 430 nm between 1175–1275°C for 1 h, or sintered at 1250°C as long as 27 h. Abnormal BaTiO3 grains are not found in the sintered samples. The microstructure and phase analysis showed that the dielectric properties, tetragonality, and grain growth of BaTiO3 are closely controlled by the formation of the liquid phase, newly formed Ba2TiSi2O8 grains, and Mn solid solution in BaTiO3 grains.
previous article Characterization of Au/Pb(Zr0.96Ti0.04)O3/Al2O3/Si antiferroelectric field-effect transistors for memory application
next article Deep level transient spectroscopy study of the effect of Mn and Bi doping on trap formation in ZnO

Dont have a licence yet? Then find out more about our products and how to get one now:

Springer Professional "Wirtschaft+Technik"

Online-Abonnement

Mit Springer Professional "Wirtschaft+Technik" erhalten Sie Zugriff auf:

  • über 102.000 Bücher
  • über 537 Zeitschriften

aus folgenden Fachgebieten:

  • Automobil + Motoren
  • Bauwesen + Immobilien
  • Business IT + Informatik
  • Elektrotechnik + Elektronik
  • Energie + Nachhaltigkeit
  • Finance + Banking
  • Management + Führung
  • Marketing + Vertrieb
  • Maschinenbau + Werkstoffe
  • Versicherung + Risiko

Jetzt Wissensvorsprung sichern!

inform now

Springer Professional "Technik"

Online-Abonnement

Mit Springer Professional "Technik" erhalten Sie Zugriff auf:

  • über 67.000 Bücher
  • über 390 Zeitschriften

aus folgenden Fachgebieten:

  • Automobil + Motoren
  • Bauwesen + Immobilien
  • Business IT + Informatik
  • Elektrotechnik + Elektronik
  • Energie + Nachhaltigkeit
  • Maschinenbau + Werkstoffe




 

Jetzt Wissensvorsprung sichern!

inform now
Literature
1.
S. Sumita, M. Ikeda, Y. Nakano, K. Nishiyama, T. Nomura, Degradation of multilayer ceramic capacitors with nickel electrodes. J. Am. Ceram. Soc. 74(ll), 2739–46 (1991)CrossRef
2.
C.A. Randall, S.F. Wang, D. Laubscher, J.P. Dougherty, W. Huebner, Structure property relationship in core-shell BaTiO3-LiF ceramics. J. Mater. Res. 8(4), 871–9 (1993)CrossRefADS
3.
L. Zhou, Z. Jiang, S. Zhang, Electrical properties of Sr0.7Ba0.3TiO3 ceramics doped with Nb2O5, 3Li2O-2SiO2, and Bi2O3. J. Am. Ceram. Soc. 74(11), 2925–7 (1991)CrossRef
4.
R.Z. Chen, A. Cui, X.H. Wang, Z.L. Gui, L.T. Li, Structure, sintering behavior and dielectric properties of silica-coated BaTiO3. Mater. Lett. 54, 314–7 (2002)CrossRef
5.
M. Valant, D. Suvorov, R.C. Pullar, K. Sarma, N.M. Alford, A mechanism for low-temperature sintering. J. Europ. Ceram. Soc. 26, 2777–83 (2006)CrossRef
6.
C. Metzmacher, K. Albertsen, Microstructural investigations of Barium Titanate-Based Material for base metal electrode ceramic multilayer capacitor. J. Am. Ceram. Soc. 84(4), 821–6 (2001)CrossRef
7.
Q. Feng, C.J. McConville, D.D. Edwards, Effect of oxygen partial pressure on the dielectric properties and microstructures of cofired base-metal- electrode multilayer ceramic capacitors. J. Am. Ceram. Soc. 89(3), 894–901 (2006)CrossRef
8.
D.F. Hennings, Dielectric materials for sintering in reducing atmospheres. J. Euro. Ceram. Soc. 21, 1637–42 (2001)CrossRef
9.
M.R. Opitz, K. Albetsen, J.J. Beeson, D.F. Hennings, J.L. Routbort, C.A. Randall, Kinetic process of reoxidation of base metal technology BaTiO3-based multilayer capacitors. J. Am. Ceram. Soc. 86(11), 1879–84 (2003)CrossRef
10.
Y.S. Jung, E.S. Na, U. Paik, J. Lee, J. Kim, A study on the phase transition and characteristics of rare earth elements doped BaTiO3. Mater Res Bull 37, 1633–40 (2002)CrossRef
11.
S. Wang, S. Zhang, X. Zhou, B. Li, Z. Chen, Investigation on dielectric properties of BaTiO3 co-doped with Ni and Nb. Mater. Lett. 60, 909–11 (2006)CrossRef
12.
S. Wang, S. Zhang, X. Zhou, B. Li, Z. Chen, Influence of sintering atmosphere on the microstructure and electrical properties of BaTiO3-based X8R materials. J. Mater. Sci. 41, 1813–7 (2006)CrossRefADS
13.
C.S. Chen, C.C. Chou, I.N. Lin, Microstructure of X7R type base-metal-electroded BaTiO3 capacitor materials prepared by duplex-structured process. J. Europ. Ceram. Soc. 25, 2743–7 (2005)CrossRef
14.
Y. Mizuno, T. Hagiwara, H. Kishi, Microstructural design of dielectrics for Ni-MLCC with ultra-thin active layers. J. Ceram. Soc. Japan 115(6), 360–4 (2007)CrossRef
15.
J.C.C. Lin, W.C.J. Wei, Melting and interface reaction of Mn-Si-O glass on BaTiO3. J. Am. Ceram. Soc. 92(9), 1926–33 (2009)CrossRef
16.
N. Louet, H. Reveron, G. Fantozzi, Sintering behaviour and microstructural evolution of ultrapure-alumina containing low amounts of SiO2. J. Europ. Ceram. Soc. 28, 205–15 (2008)CrossRef
17.
M.F. Yan, R.M. Cannon, H.K. Bower, in Ceramic Microstructures ’76, ed. by R.M. Fulrath, J.A. Pask (Westview, Boulder, 1977), pp. 276–307
18.
C.J. Lin, W.C.J. Wei, Grain boundary pinning of polycrystalline Al2O3 by Mo inclusions. Mater. Chem. & Phys. 111, 82–6 (2008)CrossRef
19.
S.B. Lee, W. Sigle, M. Ruhle, Investigation of grain boundaries in abnormal grain growth structure of TiO2- excess BaTiO3 by TEM and EELs analysis. Acta Mater. 50, 2151–62 (2002)CrossRef
20.
G. Arlt, D. Hennings, G. de With, Dielectric properties of fine-grained barium titanate ceramics. J. Appl. Phys. 58, 1619–25 (1985)CrossRefADS
21.
A. Halliyal, A.S. Bhalla, S.A. Markgraf, L.E. Cross, R.E. Newnham, Unusual pyroelectric and piezoelectric properties of fresnoite (Ba2TiSi2O8) single crystal and polar glass-ceramics. Ferroelectrics 62(1), 27–38 (1985)
22.
X. Wang, M. Gu, B. Yang, S. Zhu, W. Cao, Hall effect and dielectric properties of Mn-doped barium titanate. Microelectron. Eng. 66, 855–9 (2003)CrossRef
23.
M.A. Zubair, C. Leach, The influence of cooling rate and SiO2 additions on the grain boundary structure of Mn-doped PTC thermistor. J. Europ. Ceram. Soc. 28, 1845–55 (2008)CrossRef
Metadata
Title
Low-temperature sintering of BaTiO3 with Mn-Si-O glass
Authors
Jerry C. C. Lin
Wen-Cheng J. Wei
Publication date
01-10-2010
Publisher
Springer US
Published in
Journal of Electroceramics / Issue 2-4/2010
Print ISSN: 1385-3449
Electronic ISSN: 1573-8663
DOI
https://doi.org/10.1007/s10832-010-9613-8

Other articles of this Issue 2-4/2010

Journal of Electroceramics 2-4/2010 Go to the issue

OriginalPaper

The annealing effect on properties of ZnO thin film transistors with Ti/Pt source-drain contact

OriginalPaper

Deep level transient spectroscopy study of the effect of Mn and Bi doping on trap formation in ZnO

OriginalPaper

Characterization of Au/Pb(Zr0.96Ti0.04)O3/Al2O3/Si antiferroelectric field-effect transistors for memory application

OriginalPaper

Structure and physical properties of Eu0.8Y0.2MnO3 ceramics

OriginalPaper

Phase transitions in Pb[(Ni1/3Sb2/3)xTiyZrz]O3 solid solution ceramics studied by piezoelectric measurements

OriginalPaper

Piezoelectric and ferroelectric properties of new Pb9Ce2Ti12O36 and lead-free Ba2NdTi2Nb3O15 ceramics