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Topics in Catalysis
Published in: Topics in Catalysis 1-4/2019

05-12-2018 | Original Article

Ozone as an Enabler for Low Temperature Methane Control Over a Current Production Fe-BEA Catalyst

Authors: M. Keenan, J. Nicole, D. Poojary

Published in: Topics in Catalysis | Issue 1-4/2019

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Abstract

A process has been developed to oxidise methane at low temperatures in an excess oxygen environment using ozone as the oxidant. Ozone being more reactive than oxygen allows low temperature methane control. A range of catalysts have been screened and a commercially available current production Fe-BEA catalyst, from an automotive application has shown excellent potential for methane control with ozone in the feed, leading to a peak conversion efficiency of 81% at 168 °C in the absence of H2O and 60% conversion at 220 °C in the presence of H2O.
previous article In Situ Time-Resolved Redox Dynamics of Pd Catalysts Under Oscillating A/F Conditions
next article N-Doped Carbon–Silica Composite Confined Pd Nanoparticles for Abatement of Methane Emission From Automobiles

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Metadata
Title
Ozone as an Enabler for Low Temperature Methane Control Over a Current Production Fe-BEA Catalyst
Authors
M. Keenan
J. Nicole
D. Poojary
Publication date
05-12-2018
Publisher
Springer US
Published in
Topics in Catalysis / Issue 1-4/2019
Print ISSN: 1022-5528
Electronic ISSN: 1572-9028
DOI
https://doi.org/10.1007/s11244-018-1098-8

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