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Journal of Materials Science
Published in: Journal of Materials Science 8/2020

08-11-2019 | Chemical routes to materials

Efficient removal of formaldehyde with ZIF-8 growth on TiO2-coated activated carbon fiber felts prepared via atomic layer deposition

Authors: Lipei Ren, Yan Yu, Yuan Yang, Qian Zhang, Xingfang Xiao, Ruina Liu, Weilin Xu

Published in: Journal of Materials Science | Issue 8/2020

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Abstract

Zeolitic imidazolate framework-8 (ZIF-8) is regarded as an excellent adsorbent material for removing diverse toxic or hazardous gases. However, its milli- to nanoscale size typically restricts its applications. In this study, we demonstrate the ZIF-8 nanocrystals assembled on TiO2-coated activated carbon fiber felts via atomic layer deposition (ZIF-8@ALD-ACF felts), which can be used as a highly efficient adsorbent for HCHO removal. Using the TiO2-coated ACF felts as substrates via ALD can provide large number of growth sites for ZIF-8 nanocrystals, which results in fast and highly efficient removal of HCHO. Furthermore, ZIF-8@ALD-ACF felts achieve a highly efficient removal of HCHO under ultraviolet (UV) light. HCHO can be completely removed at high concentration within 110 min. Moreover, under UV light, it can be completely removed at low concentration within 6 min. The micropores in ACF and nanocages in ZIF-8 are suitable for small molecular HCHO uptaking and provide sufficient contact time for photocatalysis by TiO2. The ALD technology provides a useful methodology for the practical application of MOF-based materials.
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Metadata
Title
Efficient removal of formaldehyde with ZIF-8 growth on TiO2-coated activated carbon fiber felts prepared via atomic layer deposition
Authors
Lipei Ren
Yan Yu
Yuan Yang
Qian Zhang
Xingfang Xiao
Ruina Liu
Weilin Xu
Publication date
08-11-2019
Publisher
Springer US
Published in
Journal of Materials Science / Issue 8/2020
Print ISSN: 0022-2461
Electronic ISSN: 1573-4803
DOI
https://doi.org/10.1007/s10853-019-04142-y

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