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Published in: Hydrogeology Journal 3/2012

01-05-2012 | Report

Modelling groundwater contamination above a nuclear waste repository at Gorleben, Germany

Author: Michael O. Schwartz

Published in: Hydrogeology Journal | Issue 3/2012

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Abstract

The candidate repository for high-level nuclear waste in the Gorleben salt dome, Germany, is expected to host 8,550 tonnes of uranium in burnt fuel. It has been proposed that 5,440 waste containers be deposited at a depth of about 800 m. There is 260–280 m of siliciclastic cover sediments above the proposed repository. The potential groundwater contamination in the siliciclastic aquifer is simulated with the TOUGHREACT and TOUGH2-MP codes for a three-dimensional model with 290,435 elements. Two deterministic cases are simulated. The single-phase case considers the transport of radionuclides in the liquid phase only. The two-phase case accounts for hydrogen gas generated by the corrosion of waste containers and release of gaseous C-14. The gas release via a backfilled shaft is assumed to be steady (non-explosive). The simulation period is 2,000,000 years for the single-phase case and 7,000 years for the two-phase case. Only the radioactive dose in the two-phase case is higher than the regulatory limit (0.1 mSv/a).

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Literature
go back to reference Beushausen M, Ludwig R (1990) Hydrogeologische Gliederung der oberoligozänen und miozänen Schichten [Hydrogeological classification of the upper Oligocene and Miocene strata]. Report archive no. 106036, Bundesanstalt für Geowissenschaften und Rohstoffe, Hannover, Germany Beushausen M, Ludwig R (1990) Hydrogeologische Gliederung der oberoligozänen und miozänen Schichten [Hydrogeological classification of the upper Oligocene and Miocene strata]. Report archive no. 106036, Bundesanstalt für Geowissenschaften und Rohstoffe, Hannover, Germany
go back to reference Bornemann O, Behlau J, Fischbeck R, Hammer J, Jaritz W, Keller S, Mingerzahn G, Schramm M (2008) Standortbeschreibung Gorleben, Teil 3: Ergebnisse der über- und untertägigen Erkundung des Salinars [Description of the Gorleben site, part 3: results of the surface and underground exploration of the salt formation]. Geol Jahrb C73:5–211 Bornemann O, Behlau J, Fischbeck R, Hammer J, Jaritz W, Keller S, Mingerzahn G, Schramm M (2008) Standortbeschreibung Gorleben, Teil 3: Ergebnisse der über- und untertägigen Erkundung des Salinars [Description of the Gorleben site, part 3: results of the surface and underground exploration of the salt formation]. Geol Jahrb C73:5–211
go back to reference Brooks RH, Corey AT (1964) Hydraulic properties of porous media. Hydrology Papers 3, Colorado State University, Fort Collins, CO, pp 1–27 Brooks RH, Corey AT (1964) Hydraulic properties of porous media. Hydrology Papers 3, Colorado State University, Fort Collins, CO, pp 1–27
go back to reference Corey AT (1954) The interrelation between gas and oil relative permeabilities. Producer’s Monthly, vol 19, no. 1, November 1954 (quoted by Brooks and Corey 1964) Corey AT (1954) The interrelation between gas and oil relative permeabilities. Producer’s Monthly, vol 19, no. 1, November 1954 (quoted by Brooks and Corey 1964)
go back to reference GSF (2006) Deckgebirgsmodellierung Phase IV: Grundwasserbewegungen im Deckgebirge des Standortes Asse [Cover rock modelling phase IV: Groundwater movements in the cover rock of the Asse site]. GSF Forschungszentrum für Umwelt und Gesundheit, München, Germany GSF (2006) Deckgebirgsmodellierung Phase IV: Grundwasserbewegungen im Deckgebirge des Standortes Asse [Cover rock modelling phase IV: Groundwater movements in the cover rock of the Asse site]. GSF Forschungszentrum für Umwelt und Gesundheit, München, Germany
go back to reference Hughes JD, Sanford WE (2004) SUTRA-MS: a version of SUTRA modified to simulate heat and multiple-solute transport. US Geol Surv Open-File Rep 2004–1207, 141 pp Hughes JD, Sanford WE (2004) SUTRA-MS: a version of SUTRA modified to simulate heat and multiple-solute transport. US Geol Surv Open-File Rep 2004–1207, 141 pp
go back to reference Javeri V (2006) Three-dimensional analyses of coupled gas, heat and nuclide transport in a repository including rock salt convergence. Proceedings, TOUGH Symposium 2006, 15–17 May 2006, Lawrence Berkeley National Laboratory, Berkeley, CA, 9 pp Javeri V (2006) Three-dimensional analyses of coupled gas, heat and nuclide transport in a repository including rock salt convergence. Proceedings, TOUGH Symposium 2006, 15–17 May 2006, Lawrence Berkeley National Laboratory, Berkeley, CA, 9 pp
go back to reference Johns RT, Rivera A (1996) Comment on “Dispersive transport dynamics in a strongly coupled groundwater-brine flow system” by Curtis M. Oldenburg and Karsten Pruess. Water Resour Res 32:3405–3410CrossRef Johns RT, Rivera A (1996) Comment on “Dispersive transport dynamics in a strongly coupled groundwater-brine flow system” by Curtis M. Oldenburg and Karsten Pruess. Water Resour Res 32:3405–3410CrossRef
go back to reference Keesmann S, Nosek U, Buhrmann D, Fein E, Schneider A (2005) Modellrechnungen zur Langzeitsicherheit von Endlagern in Salz- and Granit-Formationen [Model calculations for the long-term safety of repositories in salt and granite formations]. Report GRS-206, GRS, Braunschweig, Germany Keesmann S, Nosek U, Buhrmann D, Fein E, Schneider A (2005) Modellrechnungen zur Langzeitsicherheit von Endlagern in Salz- and Granit-Formationen [Model calculations for the long-term safety of repositories in salt and granite formations]. Report GRS-206, GRS, Braunschweig, Germany
go back to reference Klemenz W, Rivera A, Wollrath J, Genter M (1998) Three-dimensional coupled groundwater movement and salt transport calculations as part of the safety assessment of the Gorleben repository, Germany. Proceedings DisTec’98, 9–11 September 1998, Hamburg, Germany, pp 591–596 Klemenz W, Rivera A, Wollrath J, Genter M (1998) Three-dimensional coupled groundwater movement and salt transport calculations as part of the safety assessment of the Gorleben repository, Germany. Proceedings DisTec’98, 9–11 September 1998, Hamburg, Germany, pp 591–596
go back to reference Klinge H (1994) Zusammenfassende Bearbeitung der chemischen und isotopengeochemischen Zusammensetzung der Grundwässer im Deckgebirge des Salzstocks Gorleben [Summary of the investigations on the chemical and isotopic composition of the groundwater in the cover rock of the Gorleben salt dome]. Report archive no. 0111699, Bundesanstalt für Geowissenschaften und Rohstoffe, Hannover, Germany Klinge H (1994) Zusammenfassende Bearbeitung der chemischen und isotopengeochemischen Zusammensetzung der Grundwässer im Deckgebirge des Salzstocks Gorleben [Summary of the investigations on the chemical and isotopic composition of the groundwater in the cover rock of the Gorleben salt dome]. Report archive no. 0111699, Bundesanstalt für Geowissenschaften und Rohstoffe, Hannover, Germany
go back to reference Klinge H, Margane A, Mrugalla S, Schelkes K, Söfner B (2001) Hydrogeologie des Untersuchungsgebietes Dömitz-Lenzen [Hydrogeology of the Dömitz-Lenzen exploration area]. Report archive no. 0121207, Bundesanstalt für Geowissenschaften und Rohstoffe, Hannover, Germany Klinge H, Margane A, Mrugalla S, Schelkes K, Söfner B (2001) Hydrogeologie des Untersuchungsgebietes Dömitz-Lenzen [Hydrogeology of the Dömitz-Lenzen exploration area]. Report archive no. 0121207, Bundesanstalt für Geowissenschaften und Rohstoffe, Hannover, Germany
go back to reference Klinge H, Boehme J, Grissemann C, Houben G, Ludwig R, Rübel A, Schelkes K, Schildknecht F, Suckow A (2007) Standortbeschreibung Gorleben, Teil 1: Die Hydrogeologie des Deckgebirges des Salzstocks Gorleben [Description of the Gorleben site, part 1: hydrogeology of the cover rock of the Gorleben salt dome]. Geol Jahrb C71:5–147 Klinge H, Boehme J, Grissemann C, Houben G, Ludwig R, Rübel A, Schelkes K, Schildknecht F, Suckow A (2007) Standortbeschreibung Gorleben, Teil 1: Die Hydrogeologie des Deckgebirges des Salzstocks Gorleben [Description of the Gorleben site, part 1: hydrogeology of the cover rock of the Gorleben salt dome]. Geol Jahrb C71:5–147
go back to reference Konikow LF, Sanford WE, Campbell PJ (1997) Constant-concentration boundary condition: lessons from the HYDROCOIN variable-density groundwater benchmark problem. Water Resour Res 33:2253–2261CrossRef Konikow LF, Sanford WE, Campbell PJ (1997) Constant-concentration boundary condition: lessons from the HYDROCOIN variable-density groundwater benchmark problem. Water Resour Res 33:2253–2261CrossRef
go back to reference Köthe A, Hoffmann N, Krull P, Zirngast M, Zwirner R (2007) Standortbeschreibung Gorleben, Teil 2: Die Geologie des Deck- und Nebengebirges des Salzstocks Gorleben [Description of the Gorleben site, part 2: the geology of the cover rock and country rock of the Gorleben salt dome]. Geol Jahrb C72:5–201 Köthe A, Hoffmann N, Krull P, Zirngast M, Zwirner R (2007) Standortbeschreibung Gorleben, Teil 2: Die Geologie des Deck- und Nebengebirges des Salzstocks Gorleben [Description of the Gorleben site, part 2: the geology of the cover rock and country rock of the Gorleben salt dome]. Geol Jahrb C72:5–201
go back to reference Lichtner PC (2007) FLOTRAN user’s manual: two-phase nonisothermal coupled thermal-hydrologic-chemical (THC) reactive flow & transport code, version 2.0. Report LA-UR-01-2349, Los Alamos National Laboratory, Los Alamos, NM, pp 1–168 Lichtner PC (2007) FLOTRAN user’s manual: two-phase nonisothermal coupled thermal-hydrologic-chemical (THC) reactive flow & transport code, version 2.0. Report LA-UR-01-2349, Los Alamos National Laboratory, Los Alamos, NM, pp 1–168
go back to reference Ludwig R, Mandl J, Uhlig A (1989) Zwischenbericht über die Diskretisierung hydrogeologischer Strukturen im Bereich Gorleben [Interim report on the discretisation of hydrogeological structures in the Gorleben area]. Report archive no. 0105061, Bundesanstalt für Geowissenschaften und Rohstoffe, Hannover, Germany Ludwig R, Mandl J, Uhlig A (1989) Zwischenbericht über die Diskretisierung hydrogeologischer Strukturen im Bereich Gorleben [Interim report on the discretisation of hydrogeological structures in the Gorleben area]. Report archive no. 0105061, Bundesanstalt für Geowissenschaften und Rohstoffe, Hannover, Germany
go back to reference Ludwig R, Schneider M, Sewing D (1993) Projekt Gorleben: Hydrogeologische Gliederung der quartärzeitlichen Schichtenfolge [Project Gorleben: Hydrogeological classification of the Quaternary strata]. Report archive no. 110256, Bundesanstalt für Geowissenschaften und Rohstoffe, Hannover, Germany Ludwig R, Schneider M, Sewing D (1993) Projekt Gorleben: Hydrogeologische Gliederung der quartärzeitlichen Schichtenfolge [Project Gorleben: Hydrogeological classification of the Quaternary strata]. Report archive no. 110256, Bundesanstalt für Geowissenschaften und Rohstoffe, Hannover, Germany
go back to reference Ludwig R, Schelkes K, Vogel P, Wollrath J (2001) Implications of large-scale heterogeneities for hydraulic model studies at the potential site of a radioactive waste repository at Gorleben, Germany. Eng Geol 61:119–130CrossRef Ludwig R, Schelkes K, Vogel P, Wollrath J (2001) Implications of large-scale heterogeneities for hydraulic model studies at the potential site of a radioactive waste repository at Gorleben, Germany. Eng Geol 61:119–130CrossRef
go back to reference Mills RT, Lu C, Lichtner PC, Hammond GE (2007) Simulating subsurface flow and transport on ultrascale computers using PFLOTRAN. J Phys Conf Ser 78:1–7CrossRef Mills RT, Lu C, Lichtner PC, Hammond GE (2007) Simulating subsurface flow and transport on ultrascale computers using PFLOTRAN. J Phys Conf Ser 78:1–7CrossRef
go back to reference NAGRA (2002) Project Opalinus Clay: safety report. NAGRA technical report 02–05, NAGRA, Wettingen, Switzerland NAGRA (2002) Project Opalinus Clay: safety report. NAGRA technical report 02–05, NAGRA, Wettingen, Switzerland
go back to reference Nykyri M, Nordman H, Marcos N, Löfman J, Poteri A, Hautojärvi A (2008) Radionuclide release and transport - RNT-2008. POSIVA Report 2008–06, Olkiluoto, Finland, 164 pp Nykyri M, Nordman H, Marcos N, Löfman J, Poteri A, Hautojärvi A (2008) Radionuclide release and transport - RNT-2008. POSIVA Report 2008–06, Olkiluoto, Finland, 164 pp
go back to reference Oldenburg CM, Pruess K (1995a) Dispersive transport dynamics in a strongly coupled groundwater-brine flow system. Water Resour Res 31:289–302CrossRef Oldenburg CM, Pruess K (1995a) Dispersive transport dynamics in a strongly coupled groundwater-brine flow system. Water Resour Res 31:289–302CrossRef
go back to reference Oldenburg CM, Pruess K (1995b) Strongly coupled single-phase flow problems: effects of density variation, hydrodynamic dispersion, and first order decay. Paper presented at the TOUGH Workshop ’95, 20–22 March 1995, Earth Sciences Division, Lawrence Berkeley Laboratory, University of California, Berkeley, CA, 6 pp Oldenburg CM, Pruess K (1995b) Strongly coupled single-phase flow problems: effects of density variation, hydrodynamic dispersion, and first order decay. Paper presented at the TOUGH Workshop ’95, 20–22 March 1995, Earth Sciences Division, Lawrence Berkeley Laboratory, University of California, Berkeley, CA, 6 pp
go back to reference Oldenburg CM, Pruess K, Travis BJ (1996) Reply to Comment on “Dispersive transport dynamics in a strongly coupled groundwater-brine flow system”. Water Resour Res 32:3411–3412CrossRef Oldenburg CM, Pruess K, Travis BJ (1996) Reply to Comment on “Dispersive transport dynamics in a strongly coupled groundwater-brine flow system”. Water Resour Res 32:3411–3412CrossRef
go back to reference Pruess K, Oldenburg C, Moridis G (1999) TOUGH2 user’s guide, version 2.0. Earth Sciences Division, Lawrence Berkeley National Laboratory, University of California, Berkeley, CA, 198 pp Pruess K, Oldenburg C, Moridis G (1999) TOUGH2 user’s guide, version 2.0. Earth Sciences Division, Lawrence Berkeley National Laboratory, University of California, Berkeley, CA, 198 pp
go back to reference Rasmussen TC (2001) Pressure wave vs. tracer velocities through unsaturated fractured rock. In: Evans DD, Nicholson TF, Rasmussen TC (eds) Flow and transport through unsaturated fractured rock, 2nd edn. AGU Geophysical Monograph 42, AGU, Washington, DC, pp 45–52CrossRef Rasmussen TC (2001) Pressure wave vs. tracer velocities through unsaturated fractured rock. In: Evans DD, Nicholson TF, Rasmussen TC (eds) Flow and transport through unsaturated fractured rock, 2nd edn. AGU Geophysical Monograph 42, AGU, Washington, DC, pp 45–52CrossRef
go back to reference Roedder E (1984) The fluids in salt. Am Mineral 69:413–439 Roedder E (1984) The fluids in salt. Am Mineral 69:413–439
go back to reference Roedder E (1990) Formation, handling, storage and disposal of nuclear wastes. J Geol Educ 38:360–392 Roedder E (1990) Formation, handling, storage and disposal of nuclear wastes. J Geol Educ 38:360–392
go back to reference Saripalli KP, Serne RJ, Meyer PD, McGrail BP (2002) Prediction of diffusion coefficients in porous media using tortuosity factors based on interfacial areas. Ground Water 40:346–352CrossRef Saripalli KP, Serne RJ, Meyer PD, McGrail BP (2002) Prediction of diffusion coefficients in porous media using tortuosity factors based on interfacial areas. Ground Water 40:346–352CrossRef
go back to reference Schulze O (2002) Auswirkung der Gasentwicklung auf die Integrität geringdurchlässiger Barrieregesteine [Gas generation affecting the integrity of low-permeability barrier rocks]. Report archive no. 0122442, Bundesanstalt für Geowissenschaften und Rohstoffe, Hannover, Germany, 142 pp Schulze O (2002) Auswirkung der Gasentwicklung auf die Integrität geringdurchlässiger Barrieregesteine [Gas generation affecting the integrity of low-permeability barrier rocks]. Report archive no. 0122442, Bundesanstalt für Geowissenschaften und Rohstoffe, Hannover, Germany, 142 pp
go back to reference Schwartz MO (2009) Modelling groundwater contamination above the Asse 2 medium-level waste repository, Germany. Environ Earth Sci 59:277–286CrossRef Schwartz MO (2009) Modelling groundwater contamination above the Asse 2 medium-level waste repository, Germany. Environ Earth Sci 59:277–286CrossRef
go back to reference Serco (2003) NAMMU 7.2 user guide. Serco, Didcot, UK, 262 pp Serco (2003) NAMMU 7.2 user guide. Serco, Didcot, UK, 262 pp
go back to reference SKB (2006) Long-term safety for KBS-3 repositories at Forsmark and Laxemar: a first evaluation. SKB technical report TR-06-09, Stockholm, Sweden, 620 pp SKB (2006) Long-term safety for KBS-3 repositories at Forsmark and Laxemar: a first evaluation. SKB technical report TR-06-09, Stockholm, Sweden, 620 pp
go back to reference Storck R, Aschenbach J, Hirsekorn RP, Nies A, Stelte N (1988) PAGIS performance assessment of geological isolation systems for radioactive waste: disposal in salt formations. Office for Official Publications of the European Communities, Luxembourg, 788 pp Storck R, Aschenbach J, Hirsekorn RP, Nies A, Stelte N (1988) PAGIS performance assessment of geological isolation systems for radioactive waste: disposal in salt formations. Office for Official Publications of the European Communities, Luxembourg, 788 pp
go back to reference Suter D, Biehler D, Blasser P, Hollmann A (1998) Derivation of a sorption data set for the Gorleben overburden. Proceedings DisTec ’98, 9–11 September 1998, Hamburg, Germany, pp 581–584 Suter D, Biehler D, Blasser P, Hollmann A (1998) Derivation of a sorption data set for the Gorleben overburden. Proceedings DisTec ’98, 9–11 September 1998, Hamburg, Germany, pp 581–584
go back to reference van Genuchten MT (1980) A closed-form equation for predicting the hydraulic conductivity of unsaturated soils. Soil Sci Soc Am J 44:892–898CrossRef van Genuchten MT (1980) A closed-form equation for predicting the hydraulic conductivity of unsaturated soils. Soil Sci Soc Am J 44:892–898CrossRef
go back to reference Vogel P (2005) Orientierende 3-D-Grundwassermodellrechnungen auf den Strukturen eines hydrogeologischen Modells Gorleben [Scoping calculations for a hydrogeological 3-D model structure of the Gorleben area]. Report archive No. 0125865, Bundesanstalt für Geowissenschaften und Rohstoffe, Hannover, Germany, 70 pp Vogel P (2005) Orientierende 3-D-Grundwassermodellrechnungen auf den Strukturen eines hydrogeologischen Modells Gorleben [Scoping calculations for a hydrogeological 3-D model structure of the Gorleben area]. Report archive No. 0125865, Bundesanstalt für Geowissenschaften und Rohstoffe, Hannover, Germany, 70 pp
go back to reference Vogel P, Schelkes K (1996) Influence of initial conditions and hydrogeological setting on variable density flow in an aquifer above a salt dome. Proceedings ModelCARE 96 Conference, Golden, CO, September 1996, IAHS Pub no. 237, IAHS, Wallingford, UK pp 373–381 Vogel P, Schelkes K (1996) Influence of initial conditions and hydrogeological setting on variable density flow in an aquifer above a salt dome. Proceedings ModelCARE 96 Conference, Golden, CO, September 1996, IAHS Pub no. 237, IAHS, Wallingford, UK pp 373–381
go back to reference Xu T, Sonnenthal E, Spycher N, Pruess K (2005) TOUGHREACT user’s guide: a simulation program for non-isothermal multiphase reactive geochemical transport in variably saturated geologic media. Earth Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, 195 pp Xu T, Sonnenthal E, Spycher N, Pruess K (2005) TOUGHREACT user’s guide: a simulation program for non-isothermal multiphase reactive geochemical transport in variably saturated geologic media. Earth Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, 195 pp
go back to reference Zhang K, Wu Y, Pruess K (2008) User’s guide for TOUGH2-MP: a massively parallel version of the TOUGH2 code. Earth Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, USA, 108 pp Zhang K, Wu Y, Pruess K (2008) User’s guide for TOUGH2-MP: a massively parallel version of the TOUGH2 code. Earth Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, USA, 108 pp
Metadata
Title
Modelling groundwater contamination above a nuclear waste repository at Gorleben, Germany
Author
Michael O. Schwartz
Publication date
01-05-2012
Publisher
Springer-Verlag
Published in
Hydrogeology Journal / Issue 3/2012
Print ISSN: 1431-2174
Electronic ISSN: 1435-0157
DOI
https://doi.org/10.1007/s10040-011-0825-z

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