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Journal of Materials Science: Materials in Electronics
Published in: Journal of Materials Science: Materials in Electronics 9/2021

24-04-2021

Simultaneously achieved high energy-storage and superior charge–discharge performance in K0.5Bi0.5TiO3-based lead-free ceramics by A-site defect engineering

Authors: Pengfei Chen, Tianyu Li, Wenjun Cao, Chao Cheng, Chunchang Wang

Published in: Journal of Materials Science: Materials in Electronics | Issue 9/2021

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Abstract

Simultaneously possessed high energy-storage and power density dielectric ceramics are promising materials for pulsed power capacitor applications. In this work, the (1 − x)K0.5Bi0.5TiO3–xCa0.7La0.2TiO3 ((1 − x)KBT–xCLT, x = 0, 0.24, 0.29, and 0.34) ceramics were prepared by conventional solid-state reaction method. The structural, dielectric, and energy storage properties of the ceramics were systematically studied. All ceramics exhibit a main perovskite phase with dense microstructure accompanied by little secondary phase. With the increasing of CLT content, relaxor behavior appears and gradually becomes notable in the samples. A high recoverable energy storage density of 2.57 J/cm3 together with outstanding power density of 47 MW/cm3 can be achieved simultaneously in the 0.66KBT–0.34CLT ceramic. In addition, the ceramic also shows a rapid discharge time of 41 ns. This study provides a strategy for achieving high recoverable energy storage and power density simultaneously for pulsed capacitor applications.
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Appendix
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Metadata
Title
Simultaneously achieved high energy-storage and superior charge–discharge performance in K0.5Bi0.5TiO3-based lead-free ceramics by A-site defect engineering
Authors
Pengfei Chen
Tianyu Li
Wenjun Cao
Chao Cheng
Chunchang Wang
Publication date
24-04-2021
Publisher
Springer US
Published in
Journal of Materials Science: Materials in Electronics / Issue 9/2021
Print ISSN: 0957-4522
Electronic ISSN: 1573-482X
DOI
https://doi.org/10.1007/s10854-021-05840-7

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