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18-03-2019 | Issue 8/2019

Journal of Materials Science: Materials in Electronics 8/2019

Preparation of high density garnet electrolytes by impregnation sintering for lithium-ion batteries

Journal:
Journal of Materials Science: Materials in Electronics > Issue 8/2019
Authors:
Shuai Yang, Yike Lei, Jinjin Ai, Yu Chen, Chunyan Lai
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Electronic supplementary material

The online version of this article (https://​doi.​org/​10.​1007/​s10854-019-01131-4) contains supplementary material, which is available to authorized users.

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Abstract

The conductivity of solid state electrolyte is closely connected with its chemical composition, crystal structure and density. High density Ta-doped Li7La3Zr2O12 (LLZTO) plates were synthesized by impregnation sintering. The density of electrolyte plates increased when the impregnating solution concentration increased from 5 to 35%. The LLZTO electrolyte plates showed a highest ionic conductivity of 6.47 × 10−4 S/cm when the impregnating solution concentration was 35%. The LLZTO electrolyte plates presented a highest relative density of 97% when the impregnating solution concentration was 40%, meanwhile, the activation energy of this electrolyte plate was calculated to be 0.35 eV, lower than the other samples.

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Supplementary Material
Supplementary material 1 (DOC 326 KB)
10854_2019_1131_MOESM1_ESM.doc
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